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Jacques-Edouard Moser

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Publications associées (137)

Critical role of H-aggregation for high-efficiency photoinduced charge generation in pristine pentamethine cyanine salts

Jacques-Edouard Moser, Frank Nüesch, George Cameron Fish, Juan Manuel Moreno Naranjo

The mechanism of photoinduced symmetry-breaking charge separation in solid cyanine salts at the base of organic photovoltaic and optoelectronic devices is still debated. Here, we employ femtosecond transient absorption spectroscopy (TAS) to monitor the cha ...

2021

The Role of Alkyl Chain Length and Halide Counter Ion in Layered Dion−Jacobson Perovskites with Aromatic Spacers

Michael Graetzel, Jacques-Edouard Moser, Davide Moia, Joachim Maier, Loï Charles Carbone, Jovana Milic, George Cameron Fish, Algirdas Ducinskas, Michael Allan Hope

Layered hybrid perovskites based on Dion−Jacobson phases are of interest to various optoelectronic applications. However, the understanding of their structure−property relationships remains limited. Here, we present a systematic study of Dion−Jacobson pero ...

2021

Dataset of "Direct Observation of Shallow Trap States in Thermal Equilibrium with Band-Edge Excitons in Strongly Confined CsPbBr3 Perovskite Nanoplatelets""

Jacques-Edouard Moser, Etienne Christophe Socie, Andrés Burgos Caminal, Brener Rodrigo De Carvalho Vale

Dataset underpinning the published article: Direct Observation of Shallow Trap States in Thermal Equilibrium with Band-Edge Excitons in Strongly Confined CsPbBr3 Perovskite Nanoplatelets Adv. Optical Mater. 2021, 9< ...

2021

A molecular photosensitizer achieves a Voc of 1.24 V enabling highly efficient and stable dye-sensitized solar cells with copper(II/I)-based electrolyte

Michael Graetzel, Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Nikolaos Vlachopoulos, Ulf Anders Hagfeldt, Yiming Cao, Marko Stojanovic, Etienne Christophe Socie, Felix Thomas Eickemeyer, Yameng Ren, Dan Zhang

To develop photosensitizers with high open-circuit photovoltage (Voc) is a crucial strategy to enhance the power conversion efficiency (PCE) of co-sensitized solar cells. Here, we show a judiciously tailored organic photosensitizer, coded MS5, featuring th ...

Nature Research2021

Dataset of "Critical role of H-aggregation for high-efficiency photoinduced charge generation in pristine pentamethine cyanine salts"

Jacques-Edouard Moser, Frank Nüesch, George Cameron Fish

Dataset underpinning the published article: Critical role of H-aggregation for high-efficiency photoinduced charge generation in pristine pentamethine cyanine salts Phys. Chem. Chem. Phys. 2021, 23, 23886-23895. DOI: 10.1039/D1CP03251H ...

2021

Naphthalenediimide/Formamidinium-Based Low-Dimensional Perovskites

Michael Graetzel, Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Ursula Röthlisberger, Vincent Henri Guillaume Dufoulon, Marko Mladenovic, Dominik Józef Kubicki, David Lyndon Emsley, Farzaneh Jahanbakhshi, Paramvir Ahlawat, Pascal Alexander Schouwink, Jovana Milic, George Cameron Fish, Marco Alejandro Ruiz Preciado, Masaud Hassan S Almalki, Aditya Mishra, Thomas Schneeberger

Low-dimensional hybrid perovskites have emerged as promising materials for optoelectronic applications. Although these materials have already demonstrated enhanced stability as compared to their three-dimensional perovskite analogues, their functionality h ...

2021

Enhanced Intersystem Crossing and Transient Electron Spin Polarization in a Photoexcited Pentacene–Trityl Radical

Jacques-Edouard Moser, Etienne Christophe Socie, Dominik Józef Kubicki, David Lyndon Emsley, Aaron James Rossini, Claudia Esther Avalos, Gabriele Stevanato, Moreno Lelli

Identifying and characterizing systems that generate well-defined states with large electron spin polarization is of high interest for applications in molecular spintronics, high-energy physics, and magnetic resonance spectroscopy. The generation of electr ...

2020

Revealing Exciton and Metal–Ligand Conduction Band Charge Transfer Absorption Spectra in Cu-Zn-In-S Nanocrystals

Jacques-Edouard Moser, Etienne Christophe Socie, Brener Rodrigo De Carvalho Vale

Copper indium sulfide quantum dots (QDs) have attracted substantial attention in recent years due to environmental issues and diverse applications. We report the synthesis and characterization of copper-zinc-indium-sulfide (CZIS) QDs and CZIS treated with ...

2020

Spatial Charge Separation as the Origin of Anomalous Stark Effect in Fluorous 2D Hybrid Perovskites

Jacques-Edouard Moser, Mohammad Khaja Nazeeruddin, Marine Eva Fedora Bouduban, Valentin Ianis Emmanuel Queloz, Giulia Grancini, Inés Garcia Benito, Alexander Fedorovskiy

2D hybrid perovskites (2DP) are versatile materials, whose electronic and optical properties can be tuned through the nature of the organic cations (even when those are seemingly electronically inert). Here, it is demonstrated that fluorination of the orga ...

2020

Blue Photosensitizer with Copper(II/I) Redox Mediator for Efficient and Stable Dye‐Sensitized Solar Cells

Michael Graetzel, Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Jean-David Décoppet, Ulf Anders Hagfeldt, Yiming Cao, Natalie Flores Diaz, George Cameron Fish, Yameng Ren, Dan Zhang

Dye-sensitized solar cells (DSCs) based on copper(II/I) redox mediators have recently achieved notable performance progress through tailoring the ligand structure of the copper complexes, exploiting cosensitization, and introducing an advanced device struc ...

2020

Exciton and Carrier Dynamics in Two-Dimensional Perovskites

Jacques-Edouard Moser, Marine Eva Fedora Bouduban, Etienne Christophe Socie, Andrés Burgos Caminal

Two-dimensional Ruddlesden−Popper hybrid lead halide perovskites have become a major topic in perovskite optoelectronics. Here, we aim to unravel the ultrafast dynamics governing the evolution of charge carriers and excitons in these materials. Using a com ...

2020

Liquid State and Zombie Dye Sensitized Solar Cells with Copper Bipyridine Complexes Functionalized with Alkoxy Groups

Michael Graetzel, Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Joël Teuscher, Rosario Scopelliti, Ulf Anders Hagfeldt, Marko Stojanovic, Yasemin Saygili, Marina Freitag, Hui-Seon Kim

Copper redox mediators can be employed in dye sensitized solar cells (DSCs) both as liquid electrolytes or as solid state hole transport materials (HTMs). The solid state devices that employ copper complex HTMs can be simply obtained by solvent evaporation ...

2020

Semiclassical Approach to Photophysics Beyond Kasha’s Rule and Vibronic Spectroscopy Beyond the Condon Approximation. The Case of Azulene

Jacques-Edouard Moser, Marius Wehrle, Jiri Vanicek, Tomas Zimmermann, Julien Roulet, Antonio Prlj, Tomislav Begusic, Seonghoon Choi, Zhan Tong Zhang, George Cameron Fish

Azulene is a prototypical molecule with ananomalousfluorescence from the second excited electronic state,thus violating Kasha’s rule, and with an emission spectrum thatcannot be understood within the Condon approximation. To betterunderstand the photophysi ...

2020

Exciton, Biexciton, and Hot Exciton Dynamics in CsPbBr3 Colloidal Nanoplatelets

Jacques-Edouard Moser, Etienne Christophe Socie, Andrés Burgos Caminal, Brener Rodrigo De Carvalho Vale

Lead halide perovskites have emerged as promising materials for light-emitting devices. Here, we report the preparation of colloidal CsPbBr3 nanoplatelets (3 × 4 × 23 nm3) experiencing a strong quasi-one-dimensional quantum confine- ment. Ultrafast transie ...

2020

Phenanthrene-Fused-Quinoxaline as a Key Building Block for Highly Efficient and Stable Sensitizers in Copper-Electrolyte-Based Dye-Sensitized Solar Cells

Michael Graetzel, Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Etienne Christophe Socie, Weiwei Zhang, Brian Irving Carlsen, Yameng Ren, Huiyun Jiang, Yinghui Wu

Dye-sensitized solar cells (DSSCs) based on Cu-II/I bipyridyl or phenanthroline complexes as redox shuttles have achieved very high open-circuit voltages (V-OC, more than 1 V). However, their short-circuit photocurrent density (J(SC)) has remained modest. ...

Wiley-VCH Verlag GmbH2020

Atomic-Level Microstructure of Efficient Formamidinium-Based Perovskite Solar Cells Stabilized by 5-Ammonium Valeric Acid Iodide Revealed by Multinuclear and Two-Dimensional Solid-State NMR

Michael Graetzel, Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Ursula Röthlisberger, Marine Eva Fedora Bouduban, Marko Mladenovic, Fabrizio Giordano, Dominik Józef Kubicki, David Lyndon Emsley, Farzaneh Jahanbakhshi, Essa Awadh R Alharbi, Daniel Prochowicz, Anwar Qasem M Alanazi, Jovana Milic, Dan Ren

Chemical doping of inorganic–organic hybrid perovskites is an effective way of improving the performance and operational stability of perovskite solar cells (PSCs). Here we use 5-ammonium valeric acid iodide (AVAI) to chemically stabilize the structure of ...

2019

Crystal Orientation Drives the Interface Physics at Two/Three-Dimensional Hybrid Perovskites

Jacques-Edouard Moser, Mohammad Khaja Nazeeruddin, Marine Eva Fedora Bouduban, Valentin Ianis Emmanuel Queloz, Kyung Taek Cho, Sanghyun Paek, Cristina Roldán Carmona, Giulia Grancini

Combining halide perovskites with tailored dimensionality into two/three-dimensional (2D/3D) systems has revealed a powerful strategy to boost the performances of perovskite photovoltaics (PVs). Despite recent advances, a clear understanding of the intimat ...

2019

A tandem redox system with a cobalt complex and 2-azaadamantane-N-oxyl for fast dye regeneration and open circuit voltages exceeding 1 V

Michael Graetzel, Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Nikolaos Vlachopoulos, Ulf Anders Hagfeldt, Heewon Bahng, Natalie Flores Diaz

A new tandem electrolyte composed of two redox pairs, the organic radical 2-azaadamantane-N-oxyl (AZ) and the well-known redox pair Co(bpy)(3) was investigated in dye sensitized solar cells. Importantly, an increase in V-OC was achieved using the ...

Royal Society of Chemistry2019

Atomic-level passivation mechanism of ammonium salts enabling highly efficient perovskite solar cells

Michael Graetzel, Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Fabrizio Giordano, Dominik Józef Kubicki, Jingshan Luo, Andrés Burgos Caminal, David Lyndon Emsley, Brennan James Walder, Essa Awadh R Alharbi, Anwar Qasem M Alanazi, Alexander Roland Uhl

The high conversion efficiency has made metal halide perovskite solar cells a real break-through in thin film photovoltaic technology in recent years. Here, we introduce a straight-forward strategy to reduce the level of electronic defects present at the i ...

Nature Research2019

Effect of Coordination Sphere Geometry of Copper Redox Mediators on Regeneration and Recombination Behavior in Dye-Sensitized Solar Cell Applications

Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Joël Teuscher, Ulf Anders Hagfeldt, Marko Stojanovic, Fabrizio Giordano, Yasemin Saygili, Marina Freitag, Jan Tiepelt

The recombination of injected electrons with oxidized redox species and regeneration behavior of copper redox mediators are investigated for four copper complexes, [Cu(dmby)2]2+/1+ (dmby = 6,6′-dimethyl-2,2′- bipyridine), [Cu(tmby)2]2+/1+ (tmby = 4,4′,6,6′ ...

2018

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