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Jacques-Edouard Moser

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Publications associées (137)

Lateral Intermolecular Electronic Interactions of Diketopyrrolopyrrole D−π–A Solar Dye Sensitizers Adsorbed on Mesoporous Alumina

Jacques-Edouard Moser, Ulf Anders Hagfeldt, Heewon Bahng

The development of push−pull organic dyes utilizing the donor−(π-conjugated bridge)−acceptor (D−π−A) motif has induced a paradigm shift in the design of efficient nanocrystalline dye-sensitized solar cells (DSSCs), offering control over the aesthetic prope ...

2018

Donor Effect on the Photoinduced Interfacial Charge Transfer Dynamics of D−π–A Diketopyrrolopyrrole Dye Sensitizers Adsorbed on Titanium Dioxide

Jacques-Edouard Moser, Ulf Anders Hagfeldt, Heewon Bahng

In this report, we investigate the effects of a strong electron-donating group on the electron injection and recombination processes of diketopyrrolopyrrole (DPP)-sensitized TiO2 films by comparing the dynamics of triphenylamine donor-installed DPP_A and d ...

2018

Comprehensive control of voltage loss enables 11.7% efficient solid-state dye-sensitized solar cells

Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Ladislav Kavan, Ulf Anders Hagfeldt, Chenyi Yi, Yiming Cao, Jingshan Luo, Yasemin Saygili, Heewon Bahng, Weiwei Zhang, Yuhang Liu, Yinghui Wu

The relatively large voltage loss (Vloss) in excitonic type solar cells severely limits their power conversion efficiencies (PCEs). Here, we report a comprehensive control of Vloss through efficacious engineering of the sensitizer and redox mediator, makin ...

2018

Inter-Domain Charge Transfer as a Rationale for Superior Photovoltaic Performances of Mixed Halide Lead Perovskites

Jacques-Edouard Moser, Joël Teuscher, Eric Vauthey, Marine Eva Fedora Bouduban, Fabrizio Giordano

Organic-inorganic lead halide perovskites containing a mixture of iodide and bromide anions consistently perform better in donor-acceptor heterojunction solar cells than the standard methylammonium lead triiodide material. This observation is counterintuit ...

2018

Direct Synthesis of Selenium Nanowire Mesh on a Solid Substrate and Insights into Ultrafast Photocarrier Dynamics

Jacques-Edouard Moser, Fabien Sorin, Wei Yan, Andrés Burgos Caminal

Selenium (Se) nanowires have generated much interest both for the fundamental understanding of crystal formation and growth and for technological applications in optoelectronics, imaging, piezoelectricity, catalysis, and energy harvesting and storage. Seve ...

2018

11% efficiency solid-state dye-sensitized solar cells with copper(II/I) hole transport materials

Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Joël Teuscher, Ulf Anders Hagfeldt, Norman Pellet, Yiming Cao, Amita Ummadisingu, Fabrizio Giordano, Jingshan Luo, Yasemin Saygili, Marina Freitag

Solid-state dye-sensitized solar cells currently suffer from issues such as inadequate nanopore filling, low conductivity and crystallization of hole-transport materials infiltrated in the mesoscopic TiO2 scaffolds, leading to low performances. Here we rep ...

Nature Publishing Group2017

Energy and Charge Transfer Cascade in Methylammonium Lead Bromide Perovskite Nanoparticle Aggregates

Jacques-Edouard Moser, Joël Teuscher, Marine Eva Fedora Bouduban, Andrés Burgos Caminal, Rachele Ossola

Highly photoluminescent hybrid lead halide perovskite nanoparticles have recently attracted a wide interest in the context of high-stake applications, such as light emitting diodes (LEDs), light emitting transistors and lasers. In addition, they constitute ...

Royal Soc Chemistry2017

Charge separation and carrier dynamics in donor-acceptor heterojunction photovoltaic systems

Jacques-Edouard Moser, Majed Chergui, Joël Teuscher, Jean-Pierre Wolf, Ursula Röthlisberger, Jan Cornelius Brauer, Alicia Solano, Natalie Renuka Banerji, Ariadni Boziki

Electron transfer and subsequent charge separation across donor-acceptor heterojunctions remain the most important areas of study in the field of third-generation photovoltaics. In this context, it is particularly important to unravel the dynamics of indiv ...

2017

Charge migration and charge transfer in molecular systems

Jacques-Edouard Moser, Majed Chergui, Joël Teuscher, Ursula Röthlisberger, Christopher Alexander Arrell, Andrea Cannizzo, Pablo Lopez Tarifa, Natalie Renuka Banerji, Elisa Liberatore

The transfer of charge at the molecular level plays a fundamental role in many areas of chemistry, physics, biology and materials science. Today, more than 60 years after the seminal work of R. A. Marcus, charge transfer is still a very active field of res ...

2017

Dye-sensitized solar cells for efficient power generation under ambient lighting

Paul Liska, Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Joël Teuscher, Ulf Anders Hagfeldt, Fabrizio Giordano, Yasemin Saygili, Xiaoyu Zhang, Marina Freitag

Solar cells that operate efficiently under indoor lighting are of great practical interest as they can serve as electric power sources for portable electronics and devices for wireless sensor networks or the Internet of Things. Here, we demonstrate a dye-s ...

Nature Publishing Group2017

Unveiling the Nature of Charge Carrier Interactions by Electroabsorption Spectroscopy: An Illustration with Lead-Halide Perovskites

Jacques-Edouard Moser, Joël Teuscher, Marine Eva Fedora Bouduban, Andrés Burgos Caminal

Unravelling the nature of the interactions between photogenerated charge carriers in solar energy conversion devices is key to enhance performance. In this perspective, we discuss electroabsorption spectroscopy (EAS), as the spectral bandshape of the elect ...

Schweizerische Chemische Gesellschaft2017

Synthesis and optoelectronic properties of chemically modified bi-fluorenylidenes

Michael Graetzel, Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Robin Humphry-Baker, Magdalena Anna Marszalek, Mateusz Barnaba Wielopolski

The development of new light harvesting materials is a key issue for the progress of the research on organic & hybrid photovoltaics. Here, we report a new class of organic sensitizers based on the bi-fluorenylidene moiety as p-linker within the donor–p-lin ...

Royal Society of Chemistry2016

Self-Tracking Solar Concentrator Device

Jacques-Edouard Moser, Volker Günter Zagolla, Christophe Moser

A device for self-tracking a light source, including a focusing optical device configured to focus incoming light to a focal spot, an adaptive device configured to reflect the light of the focal spot and arranged to provide for a phase change at an area of ...

2016

Dynamics of Photocarrier Separation in MAPbI3 Perovskite Multigrain Films under a Quasistatic Electric Field

Jacques-Edouard Moser, Joël Teuscher, Jelissa Risse, Arun Aby Paraecattil, Vytenis Pranculis

Applying time-resolved electroabsorption spectroscopy for the first time to methylammonium lead triiodide perovskite (MAPbI3) thin films under reverse bias, we monitored optically the ultrafast evolution of the local counter-electric field produced by the ...

American Chemical Society2016

The Fate of Electron–Hole Pairs in Polymer:Fullerene Blends for Organic Photovoltaics

Jacques-Edouard Moser, Natalie Stingelin, Jan Cornelius Brauer, Jelissa Risse, Mariateresa Scarongella, Natalie Renuka Banerji, Martina Causa'

There has been long-standing debate on how free charges are generated in donor:acceptor blends that are used in organic solar cells, and which are generally comprised of a complex phase morphology, where intermixed and neat phases of the donor and acceptor ...

Nature Publishing Group2016

Copper Bipyridyl Redox Mediators for Dye-Sensitized Solar Cells with High Photovoltage

Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Nikolaos Vlachopoulos, Ladislav Kavan, Ulf Anders Hagfeldt, Norman Pellet, Yiming Cao, Fabrizio Giordano, Yasemin Saygili, Marina Freitag, Magnus Söderberg

Redox mediators play a major role determining the photocurrent and the photovoltage in dye-sensitized solar cells (DSCs). To maintain the photocurrent, the reduction of oxidized dye by the redox mediator should be significantly faster than the electron bac ...

American Chemical Society2016

Unreacted PbI2 as a Double-Edged Sword for Enhancing the Performance of Perovskite Solar Cells

Jacques-Edouard Moser, Joël Teuscher, Kurt Schenk, Ulf Anders Hagfeldt, Marine Eva Fedora Bouduban, Wolfgang Richard Tress, Juan-Pablo Correa-Baena, Tor Jesper Jacobsson, Elham Halvani Anaraki

Lead halide perovskites have over the past few years attracted considerable interest as photo absorbers in PV applications with record efficiencies now reaching 22%. It has recently been found that not only the composition but also the precise stoichiometr ...

American Chemical Society2016

Unraveling the Dual Character of Sulfur Atoms on Sensitizers in Dye-Sensitized Solar Cells

Jacques-Edouard Moser, Mohammad Khaja Nazeeruddin, Joël Teuscher, Thomas Moehl, Aswani Yella, Peng Gao, Sadig Aghazada

Cyclometalated ruthenium sensitizers have been synthesized that differ with number of thiophene units on the auxiliary ligands. Sensitizers possessing four (SA25, SA246, and SA285) or none (SA282) sulfur atoms in their structures, were tested in solar cell ...

Amer Chemical Soc2016

Dynamics of Interfacial Charge Transfer States and Carriers Separation in Dye-Sensitized Solar Cells: A Time-Resolved Terahertz Spectroscopy Study

Jacques-Edouard Moser, Jan Cornelius Brauer, Arianna Marchioro, Ahmad Ajdar Zadeh Oskouei, Arun Aby Paraecattil

Electron injection from a photoexcited molecular sensitizer into a wide-bandgap semiconductor is the primary step toward charge separation in dye-sensitized solar cells (DSSCs). According to the current understanding of DSSCs functioning mechanism, charges ...

American Chemical Society2015

Using the Stark effect to understand charge generation in organic solar cells

Jacques-Edouard Moser, Natalie Stingelin, Jelissa Risse, Natalie Renuka Banerji

We have used a femtosecond-resolved spectroscopic technique based on the Stark effect (electromodulated differential absorption) in order to investigate free charge generation and charge drift in solar cell devices of neat conjugated polymer pBTTT and in i ...

Spie-Int Soc Optical Engineering2015

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