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Michael Graetzel

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Publications associées (1 223)

Template enhanced organic inorganic perovskite heterojunction photovoltaic device

Michael Graetzel, Shaik Mohammed Zakeeruddin, Xiong Li

The present invention relates to a solid state photovoltaic device comprising a absorbing layer containing a light harvester and at least one templating agent, said absorbing layer being prepared in a single step. ...

2017

Nondestructive Probing of Perovskite Silicon Tandem Solar Cells Using Multiwavelength Photoluminescence Mapping

Michael Graetzel, Ulf Anders Hagfeldt, Juan-Pablo Correa-Baena, Michael Saliba, Elham Halvani Anaraki

In this paper, spatially resolved photoluminescence (PL) spectroscopy with various excitation wavelengths is presented as a nondestructive and versatile technique providing access to the individual subcells of multijunction solar cells. This method is demo ...

Ieee-Inst Electrical Electronics Engineers Inc2017

Globularity-Selected Large Molecules for a New Generation of Multication Perovskites

Michael Graetzel, Ulf Anders Hagfeldt, Wolfgang Richard Tress, Juan-Pablo Correa-Baena, Antonio Abate, Michael Saliba, Filippo de Angelis, Silver Hamill Turren Cruz

Perovskite solar cells (PSCs) use perovskites with an APbX(3) structure, where A is a monovalent cation and X is a halide such as Cl, Br, and/or I. Currently, the cations for high-efficiency PSCs are Rb, Cs, methylammonium (MA), and/or formamidinium (FA). ...

Wiley-Blackwell2017

Redox Catalysis for Improved Counter-Electrode Kinetics in Dye-Sensitized Solar Cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Li Fan

Developing high-performance, low-cost electrocatalysts for the reduction reaction at the cathode of dye-sensitized solar cells (DSCs) is important for their commercialization. Here, we introduce the concept of redox catalysis for improving counter-electrod ...

Wiley-V C H Verlag Gmbh2017

Computational Characterization of the Dependence of Halide Perovskite Effective Masses on Chemical Composition and Structure

Michael Graetzel, Ursula Röthlisberger, Amir Hesam Salavati, Negar Ashari Astani, Giulia Palermo, Simone Meloni

Effective masses are calculated for a large variety of perovskites of the form ABX(3) differing in chemical composition (A= Na, Li, Cs; B = Pb, Sn; X= Cl, Br, I) and crystal structure. In addition, the effects of some defects and dopants are assessed. We s ...

2017

The effect of illumination on the formation of metal halide perovskite films

Michael Graetzel, Ludmilla Steier, Amita Ummadisingu, Wolfgang Richard Tress, Antonio Abate, Jiyoun Seo, Taisuke Matsui

Optimizing the morphology of metal halide perovskite films is an important way to improve the performance of solar cells(1) when these materials are used as light harvesters(2), because film homogeneity is correlated with photovoltaic performance(3). Many ...

Nature Publishing Group2017

Interfacial Kinetics of Efficient Perovskite Solar Cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Michael Saliba, Pankaj Kumar Yadav, Daniel Prochowicz

Perovskite solar cells (PSCs) have immense potential for high power conversion efficiency with an ease of fabrication procedure. The fundamental understanding of interfacial kinetics in PSCs is crucial for further improving of their photovoltaic performanc ...

2017

Monovalent Cation Doping of CH3NH3PbI3 for Efficient Perovskite Solar Cells

Michael Graetzel, Mojtaba Abdi Jalebi, Mohammad Ibrahim Dar

Here, we demonstrate the incorporation of monovalent cation additives into CH3NH3PbI3 perovskite in order to adjust the optical, excitonic, and electrical properties. The possibility of doping was investigated by adding monovalent cation halides with simil ...

Journal Of Visualized Experiments2017

A cockspur for the DSS cells: Erythrina crista-galli sensitizers

Michael Graetzel, Jean-David Décoppet

Dye sensitized solar cells were assembled employing a mixture of anthocyanins extracted from red ceibo's flowers. At the literature different extraction procedures are reported to extract anthocyanins from natural products and sensitize the cells. In order ...

Elsevier2017

The rapid evolution of highly efficient perovskite solar cells

Michael Graetzel, Ulf Anders Hagfeldt, Wolfgang Richard Tress, Juan-Pablo Correa-Baena, Antonio Abate, Michael Saliba, Tor Jesper Jacobsson

Perovskite solar cells (PSCs) have attracted much attention because of their rapid rise to 22% efficiencies. Here, we review the rapid evolution of PSCs as they enter a new phase that could revolutionize the photovoltaic industry. In particular, we describ ...

Royal Society of Chemistry2017

Additives, Hole Transporting Materials and Spectroscopic Methods to Characterize the Properties of Perovskite Films

Michael Graetzel, Shaik Mohammed Zakeeruddin, Nikolaos Vlachopoulos, Ulf Anders Hagfeldt, Marko Stojanovic, Amita Ummadisingu, Jiyoun Seo, Michael Saliba

The achievement of high efficiency and high stability in perovskite solar cells (PSCs) requires optimal selection and evaluation of the various components. After a brief introduction to the perovskite materials and their historical evolution, the first par ...

Schweizerische Chemische Gesellschaft2017

Spontaneous crystal coalescence enables highly efficient perovskite solar cells

Michael Graetzel, Ulf Anders Hagfeldt, Amita Ummadisingu, Juan-Pablo Correa-Baena, Antonio Abate, Michael Saliba

Perovskite solar cells have recently reached staggering efficiencies, through efforts focused on reducing grain boundaries, by enlarging the size of the crystalline domains that constitute the perovskite films. Here, we demonstrate that smaller crystallite ...

Elsevier Science Bv2017

The Rise of Highly Efficient and Stable Perovskite Solar Cells

Michael Graetzel

Recently, metal halide perovskite solar cells (PSCs) of the general formular ABX(3) where A is a monovalent cation, that is, methylammonium (MA) CH3NH3+center dot, formamidinium CH2(NH2)(2)(+), Cs+, or Rb+, B stands for Pb(II) or Sn(II), and X for iodide o ...

Amer Chemical Soc2017

Electrochemical Properties of Cu(II/I)-Based Redox Mediators for Dye-Sensitized Solar Cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Ladislav Kavan, Ulf Anders Hagfeldt, Yasemin Saygili, Marina Freitag

Three Cu(II/I)-phenanthroline and Cu(II/I)-bipyridine redox mediators are studied on various electrodes and in variety of electrolyte solutions using cyclic voltammetry and impedance spectroscopy on symmetrical dummy cells. Graphene-based catalysts provide ...

2017

Migration of cations induces reversible performance losses over day/night cycling in perovskite solar cells

Michael Graetzel, Mohammad Khaja Nazeeruddin, Ulf Anders Hagfeldt, Konrad Domanski, Wolfgang Richard Tress, Juan-Pablo Correa-Baena, Antonio Abate, Taisuke Matsui, Michael Saliba, Filippo de Angelis, Silver Hamill Turren Cruz

Perovskites have been demonstrated in solar cells with a power conversion efficiency of well above 20%, which makes them one of the strongest contenders for next generation photovoltaics. While there are no concerns about their efficiency, very little is ...

Royal Soc Chemistry2017

Morphology Engineering: A Route to Highly Reproducible and High Efficiency Perovskite Solar Cells

Michael Graetzel, Arnaud Magrez, Ulf Anders Hagfeldt, Jingshan Luo, Dongqin Bi, Fei Zhang

Despite the rapid increase in the performance of perovskite solar cells (PSC), they still suffer from low lab-to-lab or people-to-people reproducibility. Aiming for a universal condition to high-performance devices, we investigated the morphology evolution ...

Wiley-VCH Verlag Berlin2017

Room-Temperature Formation of Highly Crystalline Multication Perovskites for Efficient, Low-Cost Solar Cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Jiyoun Seo, Taisuke Matsui, Michael Saliba

Wiley-Blackwell2017

High efficiency large area perovskite solar cells and process for producing the same

Michael Graetzel, Shaik Mohammed Zakeeruddin, Ulf Anders Hagfeldt, Chenyi Yi, Xiong Li, Dongqin Bi

The present invention relates to a method for producing a solid state solar cell, comprising the steps of providing a conductive support layer or current collector, applying a metal oxide layer on the conducting support layer, applying at least one sensiti ...

2017

Metal complex used as dopant and other usage

Michael Graetzel, Mohammad Khaja Nazeeruddin, Julian Burschka

The invention relates to electrochemical devices comprising complexes of cobalt comprising at least one ligand with a 5- or six membered, N-containing heteroring. The complex are useful as p- and n-dopants, as over of electrochemical devices, in particular ...

2017

A new formation strategy of hybrid perovskites via room temperature reactive polyiodide melts

Michael Graetzel, Shaik Mohammed Zakeeruddin, Andrey Petrov

Here we introduce a new solvent-free preparation method for hybrid metal halide perovskites involving the direct reaction of metallic lead with polyiodide melts. We discovered new reactive polyiodide melts (RPMs) that can be prepared simply by adding eleme ...

Royal Soc Chemistry2017

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