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Michael Graetzel

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Publications associées (1 223)

Cation Dynamics in Mixed-Cation (MA)(x)(FA)(1-x)PbI3 Hybrid Perovskites from Solid-State NMR

Michael Graetzel, Shaik Mohammed Zakeeruddin, Péter Kalman Péchy, Dominik Józef Kubicki, David Lyndon Emsley, Albert Hofstetter, Daniel Prochowicz

Mixed-cation organic lead halide perovskites attract unfaltering attention owing to their excellent photovoltaic properties. Currently, the best performing perovskite materials contain multiple cations and provide power conversion efficiencies up to around ...

2017

The Role of Rubidium in Multiple-Cation-Based High-Efficiency Perovskite Solar Cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Mohammad Ibrahim Dar, Fabrizio Giordano, Neha Arora, Essa Awadh R Alharbi, Pankaj Kumar Yadav

Perovskite solar cells (PSCs) based on cesium (Cs)- and rubidium (Rb)-containing perovskite films show highly reproducible performance; however, a fundamental understanding of these systems is still emerging. Herein, this study has systematically investiga ...

Wiley-Blackwell2017

Novel highly active Pt/graphene catalyst for cathodes of Cu(II/I)-mediated dye-sensitized solar cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Ladislav Kavan, Ulf Anders Hagfeldt, Yasemin Saygili, Marina Freitag

Novel highly active, optically-transparent electrode catalyst containing Pt, PtOx, graphene oxide and stacked graphene platelet nanofibers is developed for a cathode of Cu(II/I)-mediated dye-sensitized solar cells. The catalyst layer is deposited on a FTO ...

Pergamon-Elsevier Science Ltd2017

Unraveling the Impact of Rubidium Incorporation on the Transport-Recombination Mechanisms in Highly Efficient Perovskite Solar Cells by Small-Perturbation Techniques

Michael Graetzel, Shaik Mohammed Zakeeruddin, Mohammad Ibrahim Dar, Neha Arora, Pankaj Kumar Yadav

We applied intensity-modulated photocurrent spectroscopy (IMPS) and intensity-modulated photovoltage spectroscopy (IMVS) techniques to explore the effect of rubidium (Rb) incorporation into lead halide perovskite films on the photovoltaic parameters of per ...

American Chemical Society2017

Air Processed Inkjet Infiltrated Carbon Based Printed Perovskite Solar Cells with High Stability and Reproducibility

Michael Graetzel, Shaik Mohammed Zakeeruddin, Syed Ghufran Hashmi, Mohammad Ibrahim Dar, Xiong Li

Carbon based perovskite solar cells are fabricated for the first time in a room temperature environment by employing inkjet infiltration of perovskite precursor ink. The fabricated perovskite solar cells exhibit impressive performance reproducibility with ...

Wiley2017

Toward All Room-Temperature, Solution- Processed, High-Performance Planar Perovskite Solar Cells: A New Scheme of Pyridine-Promoted Perovskite Formation

Michael Graetzel, Dan Li

A new, all room-temperature solution process is developed to fabricate efficient, low-cost, and stable perovskite solar cells (PVSCs). The PVSCs show high efficiency of 17.10% and 14.19%, with no hysteresis on rigid and flexible substrates, respectively, w ...

Wiley-V C H Verlag Gmbh2017

Chemical Distribution of Multiple Cation (Rb+, Cs+, MA(+), and FA(+)) Perovskite Materials by Photoelectron Spectroscopy

Michael Graetzel, Ulf Anders Hagfeldt, Juan-Pablo Correa-Baena, Michael Saliba, Silver Hamill Turren Cruz

Lead-based mixed perovskite materials have emerged in the last couple of years as promising photovoltaic materials. Recently, it was shown that improved material stability can be achieved by incorporating small amounts of inorganic cations (Cs+ and Rb+), p ...

American Chemical Society2017

One-Year stable perovskite solar cells by 2D/3D interface engineering

Michael Graetzel, Mohammad Khaja Nazeeruddin, Cristina Roldán Carmona, Iwan Zimmermann, Giulia Grancini, Filippo de Angelis

Despite the impressive photovoltaic performances with power conversion efficiency beyond 22%, perovskite solar cells are poorly stable under operation, failing by far the market requirements. Various technological approaches have been proposed to overcome ...

Nature Publishing Group2017

Approaching truly sustainable solar cells by the use of water and cellulose derivatives

Michael Graetzel, Guido Viscardi

Aqueous dye-sensitized solar cells (DSSCs) are emerging as the first truly safe, cheap and eco-friendly photovoltaic technology, at the same time overcoming the well-known instability upon moisture/water contamination typical of many solar cells. While man ...

Royal Soc Chemistry2017

Organic Dyes Containing Coplanar Dihexyl-Substituted Dithienosilole Groups for Efficient Dye-Sensitised Solar Cells

Michael Graetzel, Ravindranathan Thampi, Aswani Yella

A chromophore containing a coplanar dihexyl-substituted dithienosilole (CL1) synthesised for use in dye-sensitised solar cells displayed an energy conversion efficiency of 6.90% under AM 1.5 sunlight irradiation. The new sensitiser showed a similar fill fa ...

Hindawi Publishing Corporation2017

Effect of Cs-Incorporated NiOx on the Performance of Perovskite Solar Cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Ulf Anders Hagfeldt, Jiyoun Seo, Hui-Seon Kim, Monica Marcela Lira Cantu, Haibing Xie

The effect of Cs-incorporated NiOx on perovskite solar cells with an inverted structure was investigated, where NiOx and PCBM were used as selective contacts for holes and electrons, respectively. It was found that the generation of an Ni phase in an NiOx ...

Amer Chemical Soc2017

Phase Segregation in Cs-, Rb- and K-Doped Mixed-Cation (MA)(x)(FA)(1-x)Pbl(3) Hybrid Perovskites from Solid-State NMR

Michael Graetzel, Shaik Mohammed Zakeeruddin, Dominik Józef Kubicki, David Lyndon Emsley, Albert Hofstetter, Daniel Prochowicz

Hybrid (organic-inorganic) multication lead halide perovskites hold promise for a new generation of easily processable solar cells. Best performing compositions to date are multiple-cation solid alloys of formamidinium (FA), methylammonium (MA), cesium, an ...

American Chemical Society2017

Hill climbing hysteresis of perovskite-based solar cells: a maximum power point tracking investigation

Michael Graetzel, Shaik Mohammed Zakeeruddin, Norman Pellet, Mohammad Ibrahim Dar, Fabrizio Giordano, Joachim Maier

The surge of the power conversion efficiency of metal halide lead perovskite solar cells comes with concerns, such as the long-term ecotoxicity of lead compounds, their sensitivity toward moisture and oxygen, or the scarcity of some of their components. Mo ...

Wiley-Blackwell2017

Charge transporting material for optoelectronic and/or photoelectrochemical devices

Michael Graetzel, Mohammad Khaja Nazeeruddin, Paul Gratia, Iwan Zimmermann, Inés Garcia Benito

The present invention relates to an optoelectronic and/or photoelectrochemical device comprising at least one organic-inorganic perovskite as sensitizer and at least one compound of formula (I) comprising one benzotrithiophene core Q, wherein each thiophen ...

2017

A wire shaped coaxial photovoltaic solar cell

Michael Graetzel, Mohammad Khaja Nazeeruddin, Carlos Perez, Mohammad Ibrahim Dar

A wire shaped coaxial photovoltaic solar cell comprising: a conductive core wire shaped support (401), a nanostructured semiconductor scaffold layer (402), one or more successive perovskite layers (403), an optionally provided hole transporting material la ...

2017

Crystal Structure of DMF-Intermediate Phases Uncovers the Link Between CH3NH3PbI3 Morphology and Precursor Stoichiometry

Michael Graetzel, Andrey Petrov

We found for the first time a new origin of selection of perovskite crystallization pathways from DMF solutions containing MAI and PbI2 to present here a comprehensive study of a full set of essential intermediate phases determining the perovskite's morpho ...

American Chemical Society2017

Light management: porous 1-dimensional nanocolumnar structures as effective photonic crystals for perovskite solar cells

Michael Graetzel, Mohammad Khaja Nazeeruddin, Francisco Javier Ramos Mellado

Hybrid organic-inorganic perovskite solar cells are a topic of increasing interest, as in a short time span they are able to lead in the third generation photovoltaics. Organohalide perovskites possess exceptional optoelectronic and physical properties, th ...

Royal Society of Chemistry2016

High Open-Circuit Voltage: Fabrication of Formamidinium Lead Bromide Perovskite Solar Cells Using Fluorene-Dithiophene Derivatives as Hole-Transporting Materials

Michael Graetzel, Mohammad Khaja Nazeeruddin, Paul Gratia, Gwénolé Jean Jacopin, Mohammad Ibrahim Dar, Sadig Aghazada, Neha Arora, Filippo de Angelis

Four different fluorene dithiophene derivative-based hole-transporting materials (HTMs) (SO7-10) have been synthesized via a facile route and were successfully used in the fabrication of formamidinium lead bromide perovskite solar cells. Detailed character ...

Amer Chemical Soc2016

Branched methoxydiphenylamine-substituted fluorene derivatives as hole transporting materials for high-performance perovskite solar cells

Michael Graetzel, Mohammad Khaja Nazeeruddin, Paul Gratia, Taisuke Matsui, Michael Saliba, Simona Urnikaite

Small-molecule hole transporting materials based on methoxydiphenylamine-substituted fluorene fragments were synthesized and incorporated into a perovskite solar cell, which displayed a power conversion efficiency of up to 19.96%, one of the highest conver ...

Royal Soc Chemistry2016

High-Efficiency Perovskite Solar Cells Employing a S,N-Heteropentacene-based D-A Hole-Transport Material

Michael Graetzel, Mohammad Khaja Nazeeruddin, Shaik Mohammed Zakeeruddin, Ulf Anders Hagfeldt, Peng Gao, Amaresh Mishra, Marius Franckevicius, Dongqin Bi

We developed a new donor--acceptor-type hole-transport material (HTMs) incorporating S,N-heteropentacene as -spacer, triarylamine as donor, and dicyanovinylene as acceptor. In addition to appropriate frontier molecular orbital energies, the new HTM showed ...

Wiley-V C H Verlag Gmbh2016

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