Molecular electrocatalysis at soft interfaces

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In recent years, many efforts have been made to find alternative renewable energy sources that can ideally replace the use of fossil fuels in all aspects. One of the new emerging energy technologies is the bioelectrochemical system, of which two types are ...

The present invention relates to a compound of the general formula (I), and (II)wherein one of R11 and R12 is hydrogen and the other is -CH2-R70, and one of R13 and R14 is hydrogen and the other is -CH2-R71, or wherein one of R11 and R12 is hydrogen and th ...

The present invention relates to a compound of the general formula (I), (II) and (III), more specifically of formula (Ia), (Ib), (Ic)wherein R11 and R12 or R21 and R22 or R31 and R32 are both hydrogen or form together with CHR50 a cyclic moiety or one of R ...

Pt(II)-based molecular catalysts stand as a prototypical system in hydrogen evolution reactions (HER) owing to their consistently elevated activity levels. Their integration into heterogeneous systems thus provides an ideal platform to develop catalytic ma ...

Renewable energy sources offer a promising solution for mitigating sustainability and CO2 emissions-related issues due to their vast energy generation capacity. They enable hydrogen production via water electrolysis, as well as carbon capture and utilizati ...

Frustrated Lewis pairs (FLPs), featuring reactive combinations of Lewis acids and Lewis bases, have been utilized for myriad metal-free homogeneous catalytic processes. Immobilizing the active Lewis sites to a solid support, especially to porous scaffolds, ...

Hydrogen storage and utilization are the technologies to achieve carbon-neutral energy systems with renewable energy sources. Among the various materials that have been investigated, complex hydrides are a material exhibiting high gravimetric hydrogen dens ...

The coevolution of hydrogen and oxygen during photocatalytic water splitting presents a challenge for efficient product separation. Here, we demonstrate membrane-free, drop-based photocatalytic water splitting with inherent product separation and competiti ...

Plasma-molecular interactions generate molecular ions which react with the plasma and contribute to detachment through molecular activated recombination (MAR), reducing the ion target flux, and molecular activated dissociation (MAD), both of which create e ...

In this account, we discuss the use of genetic algorithms in the inverse design process of homogeneous catalysts for chemical transformations. We describe the main components of evolutionary experiments, specifically the nature of the fitness function to o ...

Hydrogen fuel cells are an essential component of hydrogen economy, which have been advocated as a major path towards the decarbonization of the energy sector. Within the two main types of low-temperature hydrogen fuel cells, anion-exchange membrane fuel c ...

In my thesis, I present an investigation of the dissociation reactions of gas phase molecules on single crystal metal surfaces studied by a molecular beam in combination with Reflection Absorption Infrared Spectroscopy (RAIRS). Two gas/surface systems were ...

Clean energy is highly needed at this time when the energy requirements are rapidly increasing. The observed increasing energy requirement are largely due to continued industrialization and global population explosion. The current means of energy source is ...

Energy conversion through sustainable means is essential to counter global warming and an urgent solution through a multidisciplinary approach is required. The temperature change stems from the emission of greenhouse gases largely contributed by burning fo ...

The energy transition towards a carbon-neutral and sustainable economy is one of the greatest challenges of the 21st century to combat global warming and pollution. The decarbonization process is affecting every sector of the economy (electricity, transpor ...

Cu-based bimetallic catalysts have attracted great attention for the reverse water gas shift (RWGS) reaction due to their high activity and selectivity. This work reports the application of Cu-In bimetallic catalysts for the RWGS reaction and demonstrates ...

The contact nature when monolayer blue phosphorus (blueP) interfaces with three transition metal electrodes (i. e., Pd, Ir, and Pt) was unraveled by the ab initio density functional theory calculations. Specifically, n-type Schottky contact is observed for ...

Molecular surface functionalization of metallic catalysts is emerging as an ever-developing approach to tuning their catalytic performance. Here, we report the synthesis of hybrid catalysts comprising copper nanocrystals (CuNCs) and an imidazolium ligand f ...

The conversion of intermittent renewable energy resources in the form of chemical bond, such as hydrogen production from electrochemical water splitting, is a promising way to satisfy the future global energy demand and address the environmental issues. Th ...

During electrochemical carbon dioxide (CO2) reduction on copper electrodes in an aqueous electrolyte, one of the key challenges is the competition between hydrogen evolution and CO2 reduction, especially under large current density. Here, micro-electrodes ...

Molecular electrocatalysis at soft interfaces

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Green hydrogen production using Shewanella oneidensis MR-1 bioanode and cuprous oxide-based photocathode

Biobased surfactant

Biobased surfactant

Photogeneration of Hydrogen: Insights from a Pt(II)-Complex Incorporated into a Covalent Organic Framework

Tailoring nanocatalysts and reaction interfaces for water- and CO2-electrolysis

Engineering Frustrated Lewis Pair Active Sites in Porous Organic Scaffolds for Catalytic CO2 Hydrogenation

Using Complex Hydrides for Hydrogen Storage and Direct Borohydride Fuel Cells for Electricity Production

Single emulsion drops for photocatalytic water splitting as a membrane-free approach to product separation

Investigating the impact of the molecular charge-exchange rate on detached SOLPS-ITER simulations

Genetic Algorithms for the Discovery of Homogeneous Catalysts

The design and development of anion exchange membranes for hydrogen fuel cells

Gas/Surface reactions probed by reflection absorption infrared spectroscopy

Solid-state synthesis of CdFe2O4 binary catalyst for potential application in renewable hydrogen fuel generation

Strategic factors to design the next generation of molecular water oxidation catalysts: Lesson learned from ruthenium complexes

Redox dual-flow battery for combined electricity storage and hydrogen production

Support-Dependent Cu-In Bimetallic Catalysts for Tailoring the Activity of Reverse Water Gas Shift Reaction

Electric metal contacts to monolayer blue phosphorus: electronic and chemical properties

Copper Nanocrystal Morphology Determines the Viability of Molecular Surface Functionalization in Tuning Electrocatalytic Behavior in CO2 Reduction

Atomic Level Insights of Non-Noble Metal Catalysts for the Oxygen Evolution Reaction

Micro-Electrode with Fast Mass Transport for Enhancing Selectivity of Carbonaceous Products in Electrochemical CO2 Reduction