Heralded Spectroscopy: a new single-particle probe for nanocrystal photophysics

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Publications associées (32)

Structure-property relationships and mixed conductivity in layered hybrid perovskites based on phenyl-derived spacers

Algirdas Ducinskas

Hybrid halide perovskites are currently one of the most studied semiconductors. However, due to poor intrinsic and extrinsic stability, further developments to commercialize devices based on hybrid halide perovskites are limited. Many different strategies ...

EPFL2022

Exploring the potential of FCC-hh to search for particles from B mesons

Alexey Boyarsky, Lesya Shchutska

The Future Circular Collider (FCC-hh) is a proposed successor of the Large Hadron Collider (LHC). FCC-hh would push both the energy and intensity frontiers of searches for new physics particles. In particular, due to higher energy and luminosity than at th ...

Springer Nature2022

Resolving the Controversy in Biexciton Binding Energy of Cesium Lead Halide Perovskite Nanocrystals through Heralded Single-Particle Spectroscopy

Claudio Bruschini, Edoardo Charbon, Samuel Burri, Ivan Michel Antolovic, Arin Can Ülkü

Understanding exciton-exciton interaction in multiply excited nanocrystals is crucial to their utilization as functional materials. Yet, for lead halide perovskite nanocryst-als, which are promising candidates for nanocrystal-based technologies, numerous c ...

AMER CHEMICAL SOC2021

Defect incorporation in In-containing layers and quantum wells: experimental analysis via deep level profiling and optical spectroscopy

Jean-François Carlin, Nicolas Grandjean, Mauro Mosca, Camille Haller

Recent studies demonstrated that the performance of InGaN/GaN quantum well (QW) light emitting diodes (LEDs) can be significantly improved through the insertion of an InGaN underlayer (UL). The current working hypothesis is that the presence of the UL redu ...

IOP PUBLISHING LTD2021

Direct measurement of key exciton properties: Energy, dynamics, and spatial distribution of the wave function

Martin Wolf, Michele Puppin

Excitons, Coulomb-bound electron-hole pairs, are the fundamental excitations governing the optoelectronic properties of semiconductors. Although optical signatures of excitons have been studied extensively, experimental access to the excitonic wave functio ...

Wiley2021

Integrated photonics enables continuous-beam electron phase modulation

Rui Ning Wang, Tobias Kippenberg, Junqiu Liu, Arslan Sajid Raja, Guanhao Huang, Yujia Yang

Integrated photonics facilitates extensive control over fundamental light-matter interactions in manifold quantum systems including atoms(1), trapped ions(2,3), quantum dots(4) and defect centres(5). Ultrafast electron microscopy has recently made free-ele ...

NATURE PORTFOLIO2021

Heralded Spectroscopy Reveals Exciton-Exciton Correlations in Single Colloidal Quantum Dots

Claudio Bruschini, Edoardo Charbon, Samuel Burri, Ivan Michel Antolovic, Arin Can Ülkü

Multiply excited states in semiconductor quantum dots feature intriguing physics and play a crucial role in nanocrystal-based technologies. While photoluminescence provides a natural probe to investigate these states, room-temperature single-particle spect ...

AMER CHEMICAL SOC2021

Enhanced Room-Temperature Photoluminescence Quantum Yield in Morphology Controlled J-Aggregates

Frank Nüesch, Surendra Babu Anantharaman, Jakob Heier

Supramolecular assemblies from organic dyes forming J-aggregates are known to exhibit narrowband photoluminescence with full-width at half maximum of approximate to 9 nm (260 cm(-1)). Applications of these high color purity emitters, however, are hampered ...

2021

Imaging Nonradiative Point Defects Buried in Quantum Wells Using Cathodoluminescence

Jean-François Carlin, Nicolas Grandjean, Raphaël Butté, Duncan Thomas Lindsay Alexander, Wei Liu, Wei Liu, Thomas Fjord Kjaersgaard Weatherley

Crystallographic point defects (PDs) can dramatically decrease the efficiency of optoelectronic semiconductor devices, many of which are based on quantum well (QW) heterostructures. However, spatially resolving individual nonradiative PDs buried in such QW ...

AMER CHEMICAL SOC2021

Nano-emitting Heterostructures Violate Optical Reciprocity and Enable Efficient Photoluminescence in Halide-Segregated Methylammonium-Free Wide Bandgap Perovskites

Christophe Ballif, Quentin Thomas Jeangros, Peter Joseph Fiala, Chien-Jen Yang, Pietro Caprioglio, Christian Michael Wolff

This work investigates halide segregation in methylammonium-free wide bandgap perovskites by photoluminescence quantum yield (PLQY) and advanced electron microscopy techniques. Our study reveals how the formation of nano-emitting low-energy domains embedde ...

AMER CHEMICAL SOC2021

Resonant Band-Edge Emissive States in Strongly Confined CsPbBr3 Perovskite Nanoplatelets

Jacques-Edouard Moser, Etienne Christophe Socie, Aaron Tomas Terpstra, Brener Rodrigo De Carvalho Vale

Strongly confined, fully inorganic cesium lead halide perovskite nanocrystals are of great promise for light-emitting devices in the blue spectral range owing to their high photoluminescence quantum yields. A combination of broadband fluorescence up-conver ...

2021

Interaction of Confined Polaritons in Microcavity Structures

Morteza Navadeh Toupchi

A polariton is a quasiparticle formed from the coupling of a confined photon in a cavity to electronic excitation, like exciton in a semiconductor. This dissertation reports on series of experiments in confined polariton interaction by design, fabrication, ...

EPFL2021

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