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Tom Theodorus Antonius Lummen

Cette personne a quitté l’EPFL

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Publications associées (61)

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Spontaneously Self-Assembly of a 2D/3D Heterostructure Enhances the Efficiency and Stability in Printed Perovskite Solar Cells

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen, Fei Guo

As perovskite solar cells (PSCs) are highly efficient, demonstration of high-performance printed devices becomes important. 2D/3D heterostructures have recently emerged as an attractive way to relieving the film inhomogeneity and instability in perovskite ...

2020

Azatruxene-Based, Dumbbell-Shaped, Donor-pi-Bridge-Donor Hole-Transporting Materials for Perovskite Solar Cells

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen, Cristina Roldán Carmona, Inés Garcia Benito, Cansu Igci

Three novel donor-pi-bridge-donor (D-pi-D) hole-transporting materials (HTMs) featuring triazatruxene electron-donating units bridged by different 3,4-ethylenedioxythiophene (EDOT) pi-conjugated linkers have been synthesized, characterized, and implemented ...

2020

Controlling PbI2 Stoichiometry during Synthesis to Improve the Performance of Perovskite Photovoltaics

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen

Over the past decade, remarkable progress has advanced the field of perovskite solar cells to the forefront of thin film solar technologies. The stoichiometry of the perovskite material is of paramount importance as it determines the optoelectronic propert ...

2021

An Efficient Approach to Fabricate Air-Stable Perovskite Solar Cells via Addition of a Self-Polymerizing Ionic Liquid

Mohammad Khaja Nazeeruddin, Yi Zhang, Paul Joseph Dyson, Rosario Scopelliti, Zhaofu Fei, Farzaneh Fadaei Tirani, Tom Theodorus Antonius Lummen, Cristina Roldán Carmona, Valentin Ianis Emmanuel Queloz, Zhangjun Huang, Nikita Drigo, Florian Berczy

Despite the excellent photovoltaic properties achieved by perovskite solar cells at the laboratory scale, hybrid perovskites decompose in the presence of air, especially at high temperatures and in humid environments. Consequently, high-efficiency perovski ...

Wiley2020

Universal approach toward high-efficiency two-dimensional perovskite solar cells via a vertical-rotation process

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen, Cristina Roldán Carmona, Pascal Alexander Schouwink, Yong Ding, Mo Li

The emerging 2D perovskites exhibit superior stability and similar optoelectronic attributes compared to the 3D analogues, but their strong exciton-binding energy and inferior interlayer charge-transport reduce dramatically the device performance. Herein, ...

2020

Soft Template-Controlled Growth of High-Quality CsPbI3 Films for Efficient and Stable Solar Cells

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen, Yong Ding

The unfavorable morphology and inefficient utilization of phase transition reversibility have limited the high-temperature-processed inorganic perovskite films in both efficiency and stability. Here, a simple soft template-controlled growth (STCG) method i ...

2020

alpha-CsPbI(3)Bilayers via One-Step Deposition for Efficient and Stable All-Inorganic Perovskite Solar Cells

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen, Yong Ding, Olga Syzgantseva, Xianfu Zhang

The emerging inorganic CsPbI(3)perovskites are promising wide-bandgap materials for application in tandem solar cells, but they tend to transit from a black alpha phase to a yellow delta phase in ambient conditions. Herein, a gradient grain-sized (GGS) CsP ...

Wiley2020

Lead Sequestration from Perovskite Solar Cells Using a Metal-Organic Framework Polymer Composite

Mohammad Khaja Nazeeruddin, Yi Zhang, Wendy Lee Queen, Tom Theodorus Antonius Lummen, Mounir Driss Mensi, Aron Joel Huckaba, Daniel Teav Sun, Albertus Adrian Sutanto, Florian Berczy, Michael Gullberg

Perovskite solar cells (PSCs) have increased in power conversion efficiency in the last 10 years, from approximate to 3% to now over 25%. While the best perovskite photovoltaics have remarkable efficiencies, the Pb-based absorber is likely problematic for ...

2020

Molecular materials as interfacial layers and additives in perovskite solar cells

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen

Solar cells based on organo-metal halide perovskites have gained unprecedented research interest over the last few years due to their low-cost solution processability, high power conversion efficiency, which has recently reached a certified value of 25.2%, ...

Royal Society of Chemistry2020

Lead and HTM Free Stable Two-Dimensional Tin Perovskites with Suitable Band Gap for Solar Cell Applications

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen, Iwan Zimmermann, Sadig Aghazada

Organic-inorganic hybrid perovskites have attracted great attention over the last few years as potential light-harvesting materials for efficient and cost-effective solar cells. However, the use of lead iodide in state-of-the-art perovskite devices may dem ...

Wiley-VCH Verlag GmbH2019

Optoelectronic Properties of Layered Perovskite Solar Cells

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen, Yonghui Lee, Sanghyun Paek, Kyung Taek Cho, Alexandre Vincent Laurent Chenu

Herein, the optoelectronic properties of interface-engineered perovskite 2D|3D-heterojunction structure solar cells are reported. The reciprocity theorem is applied to determine the maximum open-circuit voltage (V-oc) the device can deliver under solar ill ...

2019

Beyond Tolerance Factor: Using Deep Learning for Prediction Formability of ABX3 Perovskite Structures

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen, Valentin Ianis Emmanuel Queloz, Alexander Fedorovskiy

Deep learning (DL) is a modern powerful instrument for multiple purposes, including classification. In this study, this technique is applied to the task of perovskites formability. A commonly known perovskite dataset is used to try to make an instrument su ...

2021

Appraisement of Crystal Expansion in CH3NH3PbI3 on Doping: Improved Photovoltaic Properties

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen

Three-dimensional hybrid perovskite materials (CH3NH3PbI3) suffer from intrinsic instability owing to organic cation evaporation and ion migration. The inclusion of a large organic cation such as guanidinium has been probed to stabilize the structure. This ...

2019

Nanoscale Mass-Spectrometry Imaging of Grain Boundaries in Perovskite Semiconductors

Mohammad Khaja Nazeeruddin, Hiroyuki Kanda, Tom Theodorus Antonius Lummen, Iwan Zimmermann, Paul Gratia

Incorporation of alkali metals such as Cs+, Rb+, and K+ into hybrid organic-inorganic halide lead perovskites (HOIPs) generally improves the optoelectronic properties of HOIPs. However, it is still uncertain how alkali metals interact and distribute within ...

2020

Imaging and controlling plasmonic interference fields at buried interfaces

Fabrizio Carbone, Tom Theodorus Antonius Lummen, Gabriele Berruto, Brett Eugene Barwick

Capturing and controlling plasmons at buried interfaces with nanometre and femtosecond resolution has yet to be achieved and is critical for next generation plasmonic devices. Here we use light to excite plasmonic interference patterns at a buried metal-di ...

Nature Publishing Group2016

High-humidity processed perovskite solar cells

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen

Perovskite solar cells (PSCs) are considered the next-in-line technology in the solar industry. This technology can reduce the cost of solar energy to an unprecedented level given their remarkably high efficiency and ease of manufacturing. Hitherto, many s ...

Royal Society of Chemistry2020

Cation optimization for burn-in loss-free perovskite solar devices

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen, Sanghyun Paek, Cristina Roldán Carmona, Marius Franckevicius, Olga Syzgantseva

Hybrid lead halide perovskites will potentially lead the future energy scenario if highly efficient cells have long-term stability. Here we combine state-of-the art mixed-cation formulations containing formamidinium (FA) and methylammonium (MA), with optim ...

Royal Society of Chemistry2021

Development of an inorganic cesium carbonate-based electron transport material for a 17% power conversion efficiency perovskite solar cell device

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen, Iwan Zimmermann

A low-temperature solution process technique is employed to develop an inorganic cesium carbonate (Cs2CO3) as an electron transport material for inorganic-organic hybrid double cation (FAPbI(3))(0.85)(MAPbBr(3))(0.15) perovskite solar cells, as an alternat ...

2020

Quasi-quantum dot-induced stabilization of alpha-CsPbI3 perovskite for high-efficiency solar cells

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen, Yong Ding, Xin Liu, Yuanlong Li

All-inorganic cesium lead iodide perovskites (CsPbI3) are promising materials for efficient solar cells. However, they suffer from the formation of an undesired yellow delta -phase under ambient conditions. Herein, we provide a novel strategy to in situ pr ...

Royal Society of Chemistry2020

Inorganic and Hybrid Interfacial Materials for Organic and Perovskite Solar Cells

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen

As organic solar cells (OSCs) and perovskite solar cells (PVSCs) move closer to commercialization, further efforts toward optimizing both cell efficiency and stability are needed. As interfaces strongly affect device performance and degradation processes, ...

2020