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Qian Wang

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Publications associées (225)

A search for new physics in central exclusive production using the missing mass technique with the CMS detector and the CMS-TOTEM precision proton spectrometer

Rakesh Chawla, Arvind Shah, Andrea Rizzi, Matthias Finger, Federica Legger, Matteo Galli, Sun Hee Kim, Jian Zhao, João Miguel das Neves Duarte, Tagir Aushev, Hua Zhang, Alexis Kalogeropoulos, Yixing Chen, Tian Cheng, Ioannis Papadopoulos, Gabriele Grosso, Valérie Scheurer, Meng Xiao, Maren Tabea Meinhard, Qian Wang, Michele Bianco, Varun Sharma, Jessica Prisciandaro, Joao Varela, Sourav Sen, Ashish Sharma, Seungkyu Ha, David Vannerom, Csaba Hajdu, Sanjeev Kumar, Sebastiana Gianì, Kun Shi, Abhisek Datta, Miao Hu, Siyuan Wang, Muhammad Waqas, Anton Petrov, Jian Wang, Yi Zhang, Muhammad Ansar Iqbal, Yong Yang, , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , ,

Organocatalytic Enantioselective Pictet–Spengler Reaction of α‐Ketoesters: Development and Application to the Total Synthesis of (+)‐Alstratine A

Qian Wang, Jieping Zhu, Rémi Julien Sylvain Andres, Fenggang Sun

We report herein an asymmetric Pictet– Spengler reaction of α-ketoesters. In the presence of a catalytic amount of simple alanine-derived squaramide and p-nitrobenzoic acid, reaction of tryptamines with methyl 2-oxoalkanoates afforded the corresponding 1- ...

Wiley-VCH Verlag GmbH2023

Divergent Asymmetric Total Synthesis of (−)‐Voacafricines A and B

Qian Wang, Jieping Zhu, Rémi Julien Sylvain Andres

A divergent asymmetric total synthesis of voacafricines A and B, hexacyclic monoterpene indole alkaloids, has been accomplished featuring the following key steps: a)a catalyst-controlled asymmetric Pictet– Spengler reaction of 6-methoxytryptamine with a ch ...

Wiley-VCH Verlag GmbH2023

Proton reconstruction with the CMS-TOTEM Precision Proton Spectrometer

Rakesh Chawla, Arvind Shah, Andrea Rizzi, Matthias Finger, Federica Legger, Matteo Galli, Sun Hee Kim, Jian Zhao, João Miguel das Neves Duarte, Tagir Aushev, Hua Zhang, Alexis Kalogeropoulos, Yixing Chen, Tian Cheng, Ioannis Papadopoulos, Gabriele Grosso, Valérie Scheurer, Meng Xiao, Maren Tabea Meinhard, Qian Wang, Michele Bianco, Varun Sharma, Jessica Prisciandaro, Joao Varela, Sourav Sen, Ashish Sharma, Seungkyu Ha, David Vannerom, Csaba Hajdu, Sanjeev Kumar, Sebastiana Gianì, Kun Shi, Abhisek Datta, Miao Hu, Siyuan Wang, Muhammad Waqas, Anton Petrov, Jian Wang, Yi Zhang, Muhammad Ansar Iqbal, Yong Yang, Xin Sun, , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , ,

Enantioselective Total Synthesis of (+)-Stephadiamine

Qian Wang, Jieping Zhu, Guang Li, Baochao Yang

An asymmetric synthesis of (+)-stephadiamine has been accomplished featuring (a) an enantioselective dearomatizative Michael addition to generate a quaternary stereocenter; (b) a domino sequence involving reductive generation of nitrone from γ-nitro ketone ...

2023

Enantioselective Total Synthesis of (-)-Artatrovirenol A

Qian Wang, Jieping Zhu, Rémi Hugo Lavernhe

We report herein an enantioselective total synthesis of (-)-artatrovirenol A, a structurally unprecedented cage-like sesquiterpenoid. The synthesis features the following key steps: (a) cationic chiral oxazaborolidinium-catalyzed Diels-Alder reaction betwe ...

Amer Chemical Soc2023

Dual Photoredox and Copper Catalysis: Enantioselective 1,2-Amidocyanation of 1,3-Dienes

Qian Wang, Jieping Zhu, Dan Forster, Weisi Guo

Dual photoredox−transition-metal catalysis has emerged as a powerful tool for the development of chemical transformations. However, its application in the selective difunctionalization of 1,3-dienes remains essentially unexploited. By the synergistic actio ...

2023

Diverting the 5-exo-Trig Oxypalladation to Formally 6-endo-Trig Fluorocycloetherification Product through 1,2-O/Pd(IV) Dyotropic Rearrangement

Qian Wang, Jieping Zhu, Jing Gong

Pd-catalyzed cyclizative functionalization of γ-hydroxyalkenes affords tetrahydrofuran derivatives via a key 5-exo-trig oxypalladation step. Herein, we report a palladium(II)-catalyzed, Selectfluor-mediated formal 6-endo-trig fluorocycloetherification of γ ...

2023

Assessment of idiopathic inflammatory myopathy using a deep learning method for muscle T2 mapping segmentation

Tobias Kober, Tom Hilbert, Qian Wang, Yubo Zhao, Yao Zhang

Objective To investigate the utility of an automatic deep learning (DL) method for segmentation of T2 maps in patients with idiopathic inflammatory myopathy (IIM) against healthy controls, and also the association of quantitative T2 values in patients with ...

SPRINGER2022

Advances in Magnetics Roadmap on Spin-Wave Computing

Xiuwei Zhang, Qian Wang, Dirk Grundler, Yiming Li

Magnonics addresses the physical properties of spin waves and utilizes them for data processing. Scalability down to atomic dimensions, operation in the GHz-to-THz frequency range, utilization of nonlinear and nonreciprocal phenomena, and compatibility wit ...

Institute of Electrical and Electronics Engineers2022

Beam test performance of a prototype module with Short Strip ASICs for the CMS HL-LHC tracker upgrade

François Bianchi, Rakesh Chawla, Albert Perez, François Robert, Andrea Rizzi, Stefano Michelis, Chun Xia, Tian Cheng, Qian Wang, Varun Sharma, Jessica Prisciandaro, Davide Ceresa, Francesco Fiori, Ashish Sharma, David Vannerom, David Parker, Alessandro Caratelli, Simone Scarfì, Yong Yang, Muhammad Ahmad, Kai Yi, Andromachi Tsirou, Georgios Anagnostou, Konstantin Androsov, Ajay Kumar, Werner Lustermann, Davide Di Croce, Hui Wang, Xin Chen, Jing Li

The Short Strip ASIC (SSA) is one of the four front-end chips designed for the upgrade of the CMS Outer Tracker for the High Luminosity LHC. Together with the Macro-Pixel ASIC (MPA) it will instrument modules containing a strip and a macro-pixel sensor sta ...

2022

Two-Carbon Ring Expansion of Cyclobutanols to Cyclohexenones Enabled by Indole Radical Cation Intermediate: Development and Application to a Total Synthesis of Uleine

Qian Wang, Jieping Zhu, Alexandre Julien Florent Leclair

A single-electron transfer (SET) oxidation of indole or benzo[b]thiophene to a radical cation reverses the intrinsic polarity of these pi-excessive bicyclic heteroarenes. Here we report an oxidative two-carbon homologation of cyclobutanols to cyclohexenone ...

AMER CHEMICAL SOC2022

Apparent 6-endo-trig Carbofluorination of Alkenes Enabled by Palladium-Based Dyotropic Rearrangement

Qian Wang, Jieping Zhu, Jing Gong

Alkene difunctionalization featuring an intramolecular carbometallation step has been developed into a powerful transformation in organic synthesis. The 5-exo-trig carbometallation is in general highly favored over the alternative 6-endo-trig cyclization. ...

Wiley-VCH Verlag GmbH2022

Migrative Carbofluorination of Saturated Amides Enabled by Pd-Based Dyotropic Rearrangement

Anne-Clémence Corminboeuf, Qian Wang, Jieping Zhu, Hua Wu, Simone Gallarati, Guoqiang Yang

Directly editing an all-carbon quaternary carbon itself of nonstrained acyclic molecules remains underexploited despite the recent advances in the fields of both C–H and C–C bond activation. Herein, we report a palladium-catalyzed migrative carbofluorinati ...

ACS2022

Organocatalytic Enantioselective Diels-Alder Reaction of 2-Trifluoroacetamido-1,3-dienes with alpha,beta-Unsaturated Ketones

Qian Wang, Jieping Zhu, Xinqi Zhu

We report herein the first examples of chiral phosphoric acid-catalyzed enantioselective Diels-Alder reactions between 2-trifluoroacetamido-1,3-dienes 1 and alpha,beta-unsaturated carbonyl compounds 2. Polysubstituted 1-acetamido cyclohexenes 3 were formed ...

Wiley-VCH Verlag GmbH2023

Synthesis of 3-Acyloxyindolenines by TiCl3-Mediated Reductive Cyclization of 2-(ortho-Nitroaryl)-Substituted Enol Esters

Cyril Piemontesi, Qian Wang, Jieping Zhu, Dina Boyarskaya, Alberto Ongaro

In the presence of TiCl3, the reductive cyclization of tetrasubstituted enol esters bearing a 2-(ortho-nitroaryl) substituent affords 3-acyloxy-2,3-disubstituted indolenines in good yields. A domino process involving the partial reduction of nitro to a nit ...

2022

Modular Synthesis of Benzocyclobutenes via Pd(II)-Catalyzed Oxidative [2+2] Annulation of Arylboronic Acids with Alkenes

Anne-Clémence Corminboeuf, Qian Wang, Jieping Zhu, Simone Gallarati, Takuji Fujii

Benzocyclobutenes (BCBs) are highly valuable compounds in organic synthesis, medicinal chemistry, and materials science. However, catalytic modular synthesis of functionalized BCBs from easily accessible starting materials remains limited. We report herein ...

2022

Search for singly and pair-produced leptoquarks coupling to third-generation fermions in proton-proton collisions at root s=13 TeV

Rakesh Chawla, Arvind Shah, Andrea Rizzi, Matthias Finger, Bandeep Singh, Federica Legger, Bertrand François, Thomas Berger, Jian Zhao, João Miguel das Neves Duarte, Tagir Aushev, Hua Zhang, Quentin Python, Alexis Kalogeropoulos, Chao Wang, Yixing Chen, Tian Cheng, Ioannis Papadopoulos, Valérie Scheurer, Meng Xiao, Wei Sun, Maren Tabea Meinhard, Qian Wang, Michele Bianco, Doohyun Kim, Varun Sharma, Jessica Prisciandaro, Joao Varela, Francesco Fiori, Sourav Sen, Ashish Sharma, Seungkyu Ha, David Vannerom, Csaba Hajdu, Sanjeev Kumar, Sebastiana Gianì, Kun Shi, Abhisek Datta, Miao Hu, Siyuan Wang, Peter Hansen, , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , ,

Search for top squark production in fully hadronic final states in proton-proton collisions at root s=13 TeV

Rakesh Chawla, Arvind Shah, Andrea Rizzi, Matthias Finger, Bandeep Singh, Federica Legger, Bertrand François, Thomas Berger, Jian Zhao, João Miguel das Neves Duarte, Tagir Aushev, Hua Zhang, Alexis Kalogeropoulos, Chao Wang, Yixing Chen, Tian Cheng, Ioannis Papadopoulos, Valérie Scheurer, Meng Xiao, Wei Sun, Maren Tabea Meinhard, Qian Wang, Michele Bianco, Doohyun Kim, Varun Sharma, Jessica Prisciandaro, Joao Varela, Francesco Fiori, Sourav Sen, Ashish Sharma, Seungkyu Ha, David Vannerom, Csaba Hajdu, Sanjeev Kumar, Sebastiana Gianì, Kun Shi, Abhisek Datta, Miao Hu, Siyuan Wang, Peter Hansen, Muhammad Waqas, , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , ,

Search for the rare decay of the W boson into a pion and a photon in proton-proton collisions at root s=13 TeV

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A generic search is presented for the associated production of a Z boson or a photon with an additional unspecified massive particle X, pp -> pp + Z/gamma + X, in proton-tagged events from proton-proton collisions at root s = 13 TeV, recorded in 2017 with ...

Springer2023

The Precision Proton Spectrometer (PPS) of the CMS and TOTEM experiments collected 107.7 fb 1 in proton-proton (pp) collisions at the LHC at 13 TeV(Run 2). This paper describes the key features of the PPS alignment and optics calibrations, the proton recon ...

Iop Publishing Ltd2023

Benjamin William Allen

A search for leptoquarks produced singly and in pairs in proton-proton collisions is presented. We consider the leptoquark (LQ) to be a scalar particle of charge -1/3e coupling to a top quark plus a tau lepton (t tau) or a bottom quark plus a neutrino (b n ...

2021

A search for production of the supersymmetric partners of the top quark, top squarks, is presented. The search is based on proton-proton collision events containing multiple jets, no leptons, and large transverse momentum imbalance. The data were collected ...

American Physical Society2021

Benjamin William Allen

A search is performed for the rare decay W-+/--> pi(+/-)gamma in proton-proton collisions at root s = 13 TeV. Data corresponding to an integrated luminosity of 137 fb(-1) were collected during 2016 to 2018 with the CMS detector. This analysis exploits a no ...

2021