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Xile Hu

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Publications associées (209)

Tailored water and hydroxide transport at a quasi-two-phase interface of membrane electrode assembly electrolyzer for CO electroreduction

Xile Hu, Wenhao Ren

Electrochemical CO reduction can potentially serve as an intermediate step for the efficient conversion of CO2 to chemical fuels using renewable electricity. Although membrane electrode assembly (MEA) CO electrolyzers are industrially relevant, they curren ...

Cell Press2023

Anion Exchange Ionomers Enable Sustained Pure-Water Electrolysis Using Platinum-Group-Metal-Free Electrocatalysts

Xile Hu, Fang Song, Nanjun Chen, Ariana Serban, Yiwei Zheng

Anion exchange membrane water electrolyzer (AEMWE) is a rising technology that offers potential advantages in cost and scalability over proton exchange membrane water electrolyzer (PEMWE) technology. However, AEMWEs that stably operate in pure water still ...

2023

Robust Piperidinium-Enriched Polystyrene Ionomers for Anion Exchange Membrane Fuel Cells and Water Electrolyzers

Xile Hu, Fang Song, Nanjun Chen

Durable and efficient anion exchange polyelectrolytes (AEPs) are crucial for the long-term operation of cost-effective anion exchange membrane fuel cells (AEMFCs) and water electrolyzers (AEMWEs). Here, we present a new class of ?-amine-piperidinium-functi ...

AMER CHEMICAL SOC2023

Manganese Transfer Hydrogenases Based on the Biotin-Streptavidin Technology

Florence Pojer, Xile Hu, Kelvin Ka Ching Lau, Weijin Wang

Artificial (transfer) hydrogenases have been developed for organic synthesis, but they rely on precious metals. Native hydrogenases use Earth-abundant metals, but these cannot be applied for organic synthesis due, in part, to their substrate specificity. H ...

Wiley-VCH Verlag GmbH2023

Operando identification of a side-on nickel superoxide intermediate and the mechanism of oxygen evolution on nickel oxyhydroxide

Xile Hu, Lichen Bai, Seunghwa Lee

The oxygen evolution reaction (OER) is a key electrochemical reac-tion relevant to energy storage. Ni-containing bimetallic oxyhydrox-ides are among the most active OER catalysts in alkaline medium, but the mechanism of OER on pure Ni oxyhydroxide remains ...

ELSEVIER2023

Copper lattice tension boosts full-cell CO electrolysis to multi-carbon olefins and oxygenates

Xile Hu

Electrocatalytic upgrading of CO to value-added multi-carbon (C2+) compounds is a promising approach to efficient carbon utilization. However, current full-cell systems have low energy conversion effi-ciencies under practical conditions due to the requirem ...

Cell Press2023

Anion Exchange Membranes for Hydrogen Technologies: Challenges and Progress

Xile Hu, Xingyu Wu

Anion exchange membrane fuel cells (AEMFCs) are considered one of the most promising and efficient hydrogen conversion technologies due to their ability to use cost-effective materials. However, AEMFCs are still in an early stage of development and the lac ...

SWISS CHEMICAL SOC2023

Smart chemistry for traceless release of anticancer therapeutics

Xile Hu, Li Tang, Céline Jasmin Prange

In the design of delivery strategies for anticancer therapeutics, the controlled release of intact cargo at the destined tumor and metastasis locations is of particular importance. To this end, stimuli-responsive chemical linkers have been extensively inve ...

Elsevier Sci Ltd2023

Aryl-ether-free polyaromatic polymers with branched structures for anion exchange membranes

Xile Hu, Xingyu Wu

The present invention relates to a polyaromatic polymer that comprises multifunctional aromatic moieties MA, cationic groups CG and bifunctional aromatic moieties BA, wherein one or more CG and one or more BA form a linear unit L, and MA is connected to 3 ...

2023

Synergistic interactions between PtRu catalyst and nitrogen-doped carbon support boost hydrogen oxidation

Andreas Schueler, Jeremy Luterbacher, Xile Hu, Anna Krammer, Weiyan Ni, Lichen Bai, Miyeon Chang, Seunghwa Lee, Songlan Sun, Seongmin Jin, Yiwei Zheng

Hydroxide exchange membrane fuel cell (HEMFC) is a potentially cost-effective energy conversion technology. However, current state-of-the-art HEMFCs require a high loading of platinum-group-metal (PGM) catalysts, especially for the hydrogen oxidation react ...

NATURE PORTFOLIO2023

Enhancement of electrocatalytic oxygen evolution by chiral molecular functionalization of hybrid 2D electrodes

Magalí Alejandra Lingenfelder, Xile Hu, Karla Banjac, Seunghwa Lee, Yunchang Liang

While solar-to-fuel catalysis requires the careful transfer of electrons, there are still challenges understanding how electron spin contributes to reactivity. Here, authors employ chiral fused thiadiazole-helicenes to control spin polarization in oxygen e ...

Nature Portfolio2022

Enhanced rate performance of lithium-ion battery anodes using a cobalt-incorporated carbon conductive agent

Ming Yang, Xile Hu, Albert Claude Jean-Pierre Daubry

Lithium-ion batteries with enhanced rate performance are of crucial importance for practical applications. Extensive studies on the structural design and surface modification of electrode materials with the aim of improving the rate performance have been r ...

ROYAL SOC CHEMISTRY2022

Modulating electric field distribution by alkali cations for CO2 electroreduction in strongly acidic medium

Xile Hu, Sophia Haussener, Weiyan Ni, Shuo Liu, Wenhao Ren

The reaction of carbon dioxide with hydroxide to form carbonate in near-neutral or alkaline medium severely limits the energy and carbon efficiency of CO2 electroreduction. Here we show that by suppression of the otherwise predominant hydrogen evolution us ...

2022

Bronze-Phase TiO2 as Anode Materials in Lithium and Sodium-Ion Batteries

Xile Hu, Xiaoyan Wang

Titanium dioxide of bronze phase (TiO2(B)) has attracted considerable attention as a promising alternative lithium/sodium-ion battery anode due to its excellent operation safety, good reversible capacity, and environmental friendliness. However, several in ...

WILEY-V C H VERLAG GMBH2022

Electronic Regulation of Nickel Single Atoms by Confined Nickel Nanoparticles for Energy-Efficient CO2 Electroreduction

Andreas Schueler, Xile Hu, Anna Krammer, Wenhao Ren

Modulating the electronic structure of atomically dispersed active sites is promising to boost catalytic activity but is challenging to achieve. Here we show a cooperative Ni single-atom-on-nanoparticle catalyst (NiSA/NP) prepared via direct solid-state py ...

Wiley-VCH Verlag GmbH2022

In Vitro Biosynthesis of the [Fe]-Hydrogenase Cofactor Verifies the Proposed Biosynthetic Precursors

Xile Hu, Huijie Pan

In the FeGP cofactor of [Fe]-hydrogenase, low-spin Fe-II is in complex with two CO ligands and a pyridinol derivative; the latter ligates the iron with a 6-acylmethyl substituent and the pyridinol nitrogen. A guanylylpyridinol derivative, 6-carboxymethyl-3 ...

Wiley-VCH Verlag GmbH2022

The Function of Two Radical-SAM Enzymes, HcgA and HcgG, in the Biosynthesis of the [Fe]-Hydrogenase Cofactor

Xile Hu, Huijie Pan, Yiwei Zheng

In the biosynthesis of the iron-guanylylpyridinol (FeGP) cofactor, 6-carboxymethyl-5-methyl-4-hydroxy-2-pyridinol (1) is 3-methylated to form 2, then 4-guanylylated to form 3, and converted into the full cofactor. HcgA-G proteins catalyze the biosynthetic ...

Wiley-VCH Verlag GmbH2022

A Cation Concentration Gradient Approach to Tune the Selectivity and Activity of CO2 Electroreduction

Xile Hu, Wenhao Ren

The linear scaling relationship of the binding energies of different intermediates limits the catalyst performance in CO 2 electroreduction. Here we demonstrate a cation concentration gradient strategy to promote the activity and tune the selectivity of CO ...

Wiley-VCH Verlag GmbH2022

An efficient nickel hydrogen oxidation catalyst for hydroxide exchange membrane fuel cells

Andreas Schueler, Jeremy Luterbacher, Xile Hu, Anna Krammer, Florent Emmanuel Héroguel, Weiyan Ni, Liang Yao, Seunghwa Lee

Hydroxide exchange membrane fuel cells are promising as an energy conversion technology, but require platinum group metal electrocatalysts for their application. A Ni-based hydrogen oxidation reaction catalyst is now shown to exhibit unprecedented electroc ...

2022

Enantio- and diastereoselective construction of vicinal C(sp(3)) centres via nickel-catalysed hydroalkylation of alkenes

Xile Hu, Srikrishna Bera, Chao Fan

In drug discovery, the proportion of aliphatic carbons (C(sp(3))) and the presence of chiral carbons in organic molecules are positively correlated to their chance of clinical success. Although methods exist for the synthesis of chiral C(sp(3))-rich molecu ...

2022

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