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Michael Graetzel

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Publications associées (1 223)

Unravelling the Potential for Dithienopyrrole Sensitizers in Dye-Sensitized Solar Cells

Michael Graetzel, Jacques-Edouard Moser, Mohammad Khaja Nazeeruddin, Robin Humphry-Baker, Joël Teuscher, Ursula Röthlisberger, Ivano Tavernelli, Basile Curchod, Negar Ashari Astani, Aswani Yella, Julien Edouard Frey, Peng Gao, Lauren Elizabeth Polander

Two D−π−A dyes based on the dithieno[3,2-b:2′,3′-d]pyrrole π-bridge (DTP) were synthesized, characterized using UV−vis absorption spectroscopy and electrochemistry, modeled using quantum chemical calculations, and used as sensitizers in dye-sensitized sola ...

Amer Chemical Soc2013

First-Principles Modeling of Mixed Halide Organometal Perovskites for Photovoltaic Applications

Michael Graetzel, Mohammad Khaja Nazeeruddin, Filippo de Angelis

We computationally investigate organometal CH3NH3PbX3 and mixed halide CH3NH3PbI2X perovskites (X = Cl, Br, I), which are key materials for high efficiency solid-state solar cells. CH3NH3PbX3 perovskites exhibited the expected absorption blue shift along t ...

American Chemical Society2013

Bodipy dyes as a potential sentisizer for dye sensitized solar cells

Michael Graetzel, Mohammad Khaja Nazeeruddin, Shaik Mohammed Zakeeruddin, Jun Ho Yum, Magdalena Anna Marszalek

Amer Chemical Soc2013

Pulsed-current versus constant-voltage light-emitting electrochemical cells with trifluoromethyl-substituted cationic iridium(III) complexes

Michael Graetzel, Mohammad Khaja Nazeeruddin, Rosario Scopelliti, Cristina Roldán Carmona

We report on five cationic iridium(III) complexes with cyclometalating 2-(3'-trifluoromethylphenyl)pyridine and a diimine, (C boolean AND N)(2)Ir(N boolean AND N), N boolean AND N = 4,4'-R-2-2,2'-dipyridyl or 4,7-R-2-1,10-phenanthroline (R = H, Me, ...

Royal Society of Chemistry2013

Solid-State Dye-Sensitized Solar Cells Using a Novel Class of Ullazine Dyes as Sensitizers

Michael Graetzel, Mohammad Khaja Nazeeruddin, Robin Humphry-Baker, Amalie Dualeh

Here we present the photovoltaic performance of solid-state dye-sensitized solar cells (DSCs) using a series of ullazine-based metal-free organic sensitizers and spiro-MeOTAD as a hole-transport material. A maximum of 4.95% power conversion efficiency meas ...

Wiley-VCH Verlag Berlin2013

Synthesis and Characterization of High-Photoactivity Electrodeposited Cu2O solar absorber by photoelectrochemistry and ultrafast spectroscopy

Michael Graetzel, Jacques-Edouard Moser, Jan Cornelius Brauer, Adriana Paracchino

We present a systematic study on the effects of electrodeposition parameters on the photoelectrochemical properties of Cu2O. The influence of deposition variables (temperature, pH, and deposition current density) on conductivity has been widely explored in ...

2012

Solid-State Dye-Sensitized Solar Cells using Ordered TiO2 Nanorods on Transparent Conductive Oxide as Photoanodes

Michael Graetzel, Shaik Mohammed Zakeeruddin, Carole Graetzel, Robin Humphry-Baker, Soo-Jin Moon, Mingkui Wang, Florian Le Formal

TiO2 nanorod arrays were prepared on top of a transparent conductive glass substrate covered with a thin TiO2 compact layer. Solid-state dye-sensitized solar cells (SSDSCs) were fabricated using these structured TiO2 films sensitized with C106 dye as a pho ...

American Chemical Society2012

Towards high-performance DPP-based sensitizers for DSC applications

Michael Graetzel, Mohammad Khaja Nazeeruddin, Jun Ho Yum, Thomas Wesley Holcombe, Junghyun Yoon, Kasparas Rakstys, Yongjoo Kim

A novel, asymmetric DPP bridge/core was synthesized and tested in DSC devices. By desymmetrising the DPP core/bridge, a remarkable IPCE of >80% and a maximum power conversion efficiency of 7.7% were achieved. With the use of a wide-bandgap co-sensitizer, 8 ...

Royal Society of Chemistry2012

A New Heteroleptic Ruthenium Sensitizer for Transparent Dye-Sensitized Solar Cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Nuttapol Pootrakulchote, Thomas Moehl, Miao Chen

A new heteroleptic ruthenium complex, coded CYC-B19, incorporating an ancillary ligand endowed with hexylthio-bithiophene segments and a conjugated anchoring ligand with vinyl groups was prepared. This new sensitizer exhibits a lower energy MLCT band centr ...

Wiley-VCH Verlag Berlin2012

Voltage enhancement in dye-sensitized solar cell using (001)-oriented anatase TiO2 nanosheets

Michael Graetzel, Paul Liska, Jacques-Edouard Moser, Ladislav Kavan, Elham Ghadiri

A nanocrystalline TiO2 (anatase) nanosheet ex- posing mainly the (001) crystal faces was tested as photo- anode material in dye-sensitized solar cells. The nanosheets were prepared by hydrothermal growth in HF medium. Good-quality thin films were deposited ...

Springer2012

Donor-p-Acceptors Containing the 10-(1,3-Dithiol-2-ylidene)anthracene Unit for Dye-Sensitized Solar Cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Robin Humphry-Baker, Magdalena Anna Marszalek

Two donoracceptor molecular tweezers incorporating the 10-(1,3-dithiol-2-ylidene)anthracene unit as donor group and two cyanoacrylic units as accepting/anchoring groups are reported as metal-free sensitizers for dye-sensitized solar cells. By changing the ...

Wiley-Blackwell2012

Colorants, pile solaire sensibilisée aux colorants et son procédé de fabrication

Michael Graetzel, Mohammad Khaja Nazeeruddin

A dyestuff shown by the formula (1), ML 1 L 2 L 3 (1) wherein M represents an element belonging to Group 8 to Group 10 of the long format Periodic Table, L 1 and L 2 individually represent a bidentate ligand shown by the formula (2), L 3 represents a biden ...

2012

Modulating dye E(S+/S*) with efficient heterocyclic nitrogen containing acceptors for DSCs

Michael Graetzel, Mohammad Khaja Nazeeruddin, Aswani Yella

Acceptor motifs based on nitrogen containing heterocycles have been synthesized for use in dye-sensitized solar cells (DSCs). Through the selective addition of nitrogen atoms and increased conjugation of the nitrogen containing heterocycles the excited-sta ...

Royal Society of Chemistry2012

Sub-nanometer Ga2O3 tunnelling layer by atomic layer deposition to achieve 1.1V open-circuit potential in dye-sensitized solar cells

Michael Graetzel, Mohammad Khaja Nazeeruddin, Robin Humphry-Baker, Nicolas Tétreault, Aravind Kumar Chandiran, Chenyi Yi

Herein, we present the first use of a gallium oxide tunnelling layer to significantly reduce electron recombination in dye-sensitized solar cells (DSC). The sub-nanometer coating is achieved using atomic layer deposition (ALD) and leading to a new DSC reco ...

American Chemical Society2012

Symmetric vs. asymmetric squaraines as photosensitisers in mesoscopic injection solar cells: a structure-property relationship study

Michael Graetzel, Mohammad Khaja Nazeeruddin, Guido Viscardi, Davide Di Censo

A symmetric squaraine and its related non-symmetric structure are shown to have comparable efficiencies in DSCs, but with undoubtedly advantages in the low cost and casiness of synthesis for the symmetrical structure. ...

Royal Society of Chemistry2012

Influence of cations of the electrolyte on the performance and stability of dye sensitized solar cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Philippe Wyss, Thomas Moehl

The electrolyte is one of the key components for DSC and its properties have great influence on the photo-conversion efficiency and stability of the devices. Five new low volatile electrolytes containing 3-methoxypropionitrile (MPN) as solvent were prepare ...

Royal Society of Chemistry2012

Influence of the counter electrode on the photovoltaic performance of dye-sensitized solar cells using a disulfide/thiolate redox electrolyte

Michael Graetzel, Mohammad Khaja Nazeeruddin, Shaik Mohammed Zakeeruddin, Julian Burschka

Strong scientific interests focus on the investigation of iodine-free redox couples for their application in dye-sensitized solar cells (DSCs). Recently, a disulfide/thiolate-based redox electrolyte has been proposed as a valuable alternative to the conven ...

2012

Time-Resolved Indirect Nanoplasmonic Sensing Spectroscopy of Dye Molecule Interactions with Dense and Mesoporous TiO2 Films

Michael Graetzel, Bengt Kasemo, Leo-Philipp Heiniger

Indirect nanoplasmonic sensing (INPS) is an experimental platform exploiting localized surface plasmon resonance (LSPR) detection of processes in nanomaterials, molecular assemblies, and films at the nanoscale. Here we have for the first time applied INPS ...

American Chemical Society2012

Nanocomposites containing neutral blue emitting cyclometalated iridium(III) emitters for oxygen sensing

Michael Graetzel, Mohammad Khaja Nazeeruddin, Davide Di Censo, Rosario Scopelliti, Ursula Röthlisberger, Ivano Tavernelli, Basile Curchod, Il Jung

The behavior toward oxygen sensing of nanocomposites made of the aluminum oxide-hydroxide nanostructured solid support (AP200/19) and neutral blue emitting cyclometalated iridium(III) complexes was studied. The results are compared with the same dyes immob ...

2012

Cobalt Electrolyte/Dye Interactions in Dye-Sensitized Solar Cells: A Combined Computational and Experimental Study

Michael Graetzel, Mohammad Khaja Nazeeruddin, Jun Ho Yum, Filippo de Angelis

We report a combined experimental and computational investigation to understand the nature of the interactions between cobalt redox mediators and TiO2 surfaces sensitized by :ruthenium and organic dyes, and their impact on. the performance of the correspon ...

American Chemical Society2012

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