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Michael Graetzel

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Publications associées (1 223)

Co(III) Complexes as p-Dopants in Solid-State Dye-Sensitized Solar Cells

Michael Graetzel, Mohammad Khaja Nazeeruddin, Julian Burschka

Following our recent work on the use of Co(III) complexes as p-type dopants for triarylamine-based organic hole-conductors, we herein report on two new Co(III) complexes for doping applications. With the aim of ameliorating the dopant's suitability for its ...

American Chemical Society2013

Between photocatalysis and photosynthesis: Synchrotron spectroscopy methods on molecules and materials for solar hydrogen generation

Michael Graetzel, Yelin Hu, Artur Braun, Jin Guo

Energy research is to a large extent materials research, encompassing the physics and chemistry of materials, including their synthesis, processing toward components and design toward architectures, allowing for their functionality as energy devices, exten ...

Elsevier2013

Investigation of the role of anions in hydrotalcite for quasi-solid state dye-sensitized solar cells application

Michael Graetzel, Xiaoyan Wang

In recent research in clean energy applications, clay has gained significant interest, especially as a gelator in dye-sensitized solar cells (DSSCs), for its capability to resolve the leakage issue of liquid electrolyte. In this paper, anionic hydrotalcite ...

Royal Society of Chemistry2013

Evaluating the critical thickness of TiO2 layer on insulating mesoporous templates for efficient current collection in dye-sensitized solar cells

Pascal Comte, Michael Graetzel, Mohammad Khaja Nazeeruddin, Robin Humphry-Baker, Aravind Kumar Chandiran, Chenyi Yi

In this paper, we present a way of utilizing thin and conformal overlayer of titanium dioxide on insulating mesoporous template as a photoanode for dye-sensitized solar cells (DSC). Different thicknesses of TiO2 ranging from 1 nm to 15 nm are deposited on ...

Wiley-Blackwell2013

The Influence of the Ammonolysis Temperature on the Photocatalytic Activity of beta-TaON

Michael Graetzel, Takashi Hisatomi

Phase-pure tantalum oxynitride (beta-TaON) powders were synthesized by thermal ammonolysis of Ta2O5 powders. X-ray diffraction revealed an enlargement of the unit cell and an increase of the crystallite size with increasing ammonolysis temperature. Scannin ...

Hindawi Publishing Corporation2013

Facile synthesis of a bulky BPTPA donor group suitable for cobalt electrolyte based dye sensitized solar cells

Michael Graetzel, Mohammad Khaja Nazeeruddin, Jun Ho Yum, Peng Gao, Thomas Wesley Holcombe, Yongjoo Kim

An efficient synthesis of N-(2 ',4 '-bis(hexyloxy)-[1,1 '-biphenyl]-4-yl)-N-(4-bromophenyl)-2 ',4 '-bis(hexyloxy)-[ 1,1 '-biphenyl]-4-amine (BPTPA donor, 5) was developed based on a new 4-step synthetic route. The BPTPA donor is used to quickly access two ...

Royal Society of Chemistry2013

The Application of Electrospun Titania Nanofibers in Dye-sensitized Solar Cells

Michael Graetzel, Mohammad Khaja Nazeeruddin, Ladislav Kavan, Aravind Kumar Chandiran

Titania nanofibers were fabricated using the industrial Nanospider (TM) technology. The preparative protocol was optimized by screening various precursor materials to get pure anatase nanofibers. Composite films were prepared by mixing a commercial paste o ...

Schweizerische Chemische Gesellschaft2013

In situ photo-assisted deposition of MoS2 electrocatalyst onto zinc cadmium sulphide nanoparticle surfaces to construct an efficient photocatalyst for hydrogen generation

Michael Graetzel, Nripan Mathews

We reported herein a facile and scalable preparation process for MoS2-decorated ZnxCd1-xS hybrid photocatalysts for hydrogen generation. ZnxCd1-xS nanopowder was first prepared from commercially available precursors employing a solution based process. MoS2 ...

Royal Society of Chemistry2013

High-performance pure blue phosphorescent OLED using a novel bis-heteroleptic iridium(III) complex with fluorinated bipyridyl ligands

Michael Graetzel, Mohammad Khaja Nazeeruddin

A novel pure blue phosphorescent emitter FK306 with fluorinated bipyridyl ligands was developed. The I-p level was determined to be 6.3 eV by photoelectron yield spectroscopy (PYS) in the solid state. The photophysical properties of a FK306/mCP film were e ...

Royal Society of Chemistry2013

Nanofibrous TiO2 improving performance of mesoporous TiO2 electrode in dye-sensitized solar cell

Michael Graetzel, Ladislav Kavan, Jun Ho Yum

A method of direct coating of conducting glass by electrospinning was developed. Electrospun fibrous TiO2 consisting of closely packed anatase nanocrystals of 40-50 nm in size was incorporated into mesoporous TiO2 thin film stabilized by phosphorus. The me ...

Springer Verlag2013

Effects of ZnO film growth route and nanostructure on electron transport and recombination in dye-sensitized solar cells

Michael Graetzel, Thomas Moehl

The photovoltaic performances of ZnO-based dye-sensitized solar cells (DSSCs) have been studied for ZnO porous films prepared by different techniques. A comparison is made between nanoparticle (NP) films prepared by a sol-gel method and two different elect ...

Royal Society of Chemistry2013

Determining the Conductivities of the Two Charge Transport Phases in Solid-State Dye-Sensitized Solar Cells by Impedance Spectroscopy

Michael Graetzel, Shaik Mohammed Zakeeruddin, Soo-Jin Moon, Nripan Mathews, Feng Li

To apply impedance spectroscopy (IS) for studying charge transport in the mesoporous film of solid-state dye-sensitized solar cells (ss-DSCs), it is necessary to determine the relative conductivities of the electron and hole transporting phases, given the ...

American Chemical Society2013

New sensitizers for dye-sensitized solar cells featuring a carbon-bridged phenylenevinylene

Michael Graetzel, Anne-Sophie Chauvin, Aswani Yella

We demonstrate that a carbon-bridged phenylenevinylene (CPV)-linked dye serves as a novel and efficient sensitizer for dye-sensitized solar cells. The cells show IPCE values of greater than 90%, PCEs of up to 7.12%, and high open circuit voltages reaching ...

Royal Society of Chemistry2013

Diffusion and adsorption of dye molecules in mesoporous TiO2 photoelectrodes studied by indirect nanoplasmonic sensing

Michael Graetzel, Bengt Kasemo, Leo-Philipp Heiniger

In this study, we used Hidden Interface-Indirect Nanoplasmonic Sensing (HI-INPS) for real time monitoring of dye impregnation (adsorption-diffusion process) of mesoporous TiO2 electrodes of the kind used in dye-sensitized solar cells. We measured the dye p ...

Royal Society of Chemistry2013

Electrodes for dye-sensitized solar cells: A case of graphene-based materials

Michael Graetzel, Ladislav Kavan, Jun Ho Yum

Amer Chemical Soc2013

Towards Compatibility between Ruthenium Sensitizers and Cobalt Electrolytes in Dye-Sensitized Solar Cells

Michael Graetzel, Jacques-Edouard Moser, Mohammad Khaja Nazeeruddin, Joël Teuscher, Rosario Scopelliti, Ursula Röthlisberger, Ivano Tavernelli, Basile Curchod, Negar Ashari Astani, Aswani Yella, Julien Edouard Frey, Peng Gao, Simon Mathew, Lauren Elizabeth Polander

Wiley-Blackwell2013

Steric hindrance at metal centre quenches green phosphorescence of cationic iridium(III) complexes with 1-(2-pyridyl)-pyrazoles

Michael Graetzel, Mohammad Khaja Nazeeruddin, Rosario Scopelliti

Cationic cyclometalated iridium(III) complexes (N,C-2'-2-phenylpyridyl)(2)Ir((NN)-N-boolean AND) with alkyl-substituted 1-(2'-pyridyl)-pyrazole (NN)-N-boolean AND ligands exhibit green phosphorescence from a cyclometalating-ligand-centered excited s ...

Elsevier2013

New donor-pi-acceptor sensitizers containing 5H-[1,2,5]thiadiazolo [3,4-f]isoindole-5,7(6H)-dione and 6H-pyrrolo[3,4-g]quinoxaline-6,8(7H)-dione units

Michael Graetzel, Ulf Anders Hagfeldt

Two new D-pi-A sensitizers (L101 and L102) incorporating 5H-[1,2,5]thiadiazolo [3,4-f] isoindole-5,7(6H)-dione and 6H-pyrrolo[3,4-g]quinoxaline-6,8(7H)-dione core structures were synthesized and tested in liquid dye-sensitized solar cells (DSCs). L102 achi ...

Royal Society of Chemistry2013

The Molecular Engineering of Organic Sensitizers for Solar-Cell Applications

Michael Graetzel, Mohammad Khaja Nazeeruddin, Aswani Yella, Thomas Wesley Holcombe

Wiley-Blackwell2013

Decoupling light absorption and charge transport properties in near IR-sensitized Fe2O3 regenerative cells

Michael Graetzel, Satvasheel Powar, Nripan Mathews, Kazuteru Nonomura

We report a regenerative iron oxide nanorod solar cell sensitized with squarine (SQ02) dye, which improves the overall light harvesting due to the dye's complementary absorption. The use of illumination sources which enabled selective excitation of Fe2O3 a ...

Royal Society of Chemistry2013

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