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Michael Graetzel

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Publications associées (1 218)

Page 3 sur 61

Highly active oxide photocathode for photoelectrochemical water reduction

Michael Graetzel, Kevin Sivula, Vincent Laporte, Adriana Paracchino

A clean and efficient way to overcome the limited supply of fossil fuels and the greenhouse effect is the production of hydrogen fuel from sunlight and water through the semiconductor/water junction of a photoelectrochemical cell, where energy collection a ...

Nature Publishing Group2011

Self-assembled photosystem-I biophotovoltaics on nanostructured TiO2 and ZnO

Michael Graetzel, Mohammad Khaja Nazeeruddin

The abundant pigment-protein membrane complex photosystem-I (PS-I) is at the heart of the Earth's energy cycle. It is the central molecule in the "Z-scheme'' of photosynthesis, converting sunlight into the chemical energy of life. Commandeering this intric ...

Nature Publishing Group2012

Significant Improvement of Dye-Sensitized Solar Cell Performance by Small Structural Modification in π-Conjugated Donor-Acceptor Dyes

Michael Graetzel, Shaik Mohammed Zakeeruddin, Robin Humphry-Baker, Jacques-Edouard Moser, Joël Teuscher, Magdalena Anna Marszalek, Mateusz Barnaba Wielopolski

Two donor-π-acceptor (D-π-A) dyes are synthesized for application in dye- sensitized solar cells (DSSC). These D-π-A sensitizers use triphenylamine as donor, oligothiophene as both donor and π-bridge, and benzothiadiazole (BTDA)/cyanoacrylic acid as accept ...

Wiley-Blackwell2012

Selective C-C Coupling in Carbon Dioxide Electroreduction via Efficient Spillover of Intermediates As Supported by Operando Raman Spectroscopy

Michael Graetzel, Shaik Mohammed Zakeeruddin, Jingshan Luo, Dan Ren, Hong Zhang, Jing Gao

Developing efficient systems for the conversion of carbon dioxide to valuable chemicals using solar power is critical for mitigating climate change and ascertaining the worlds future supply of clean fuels. Here, we introduce a mesoscopic cathode consisting ...

AMER CHEMICAL SOC2019

Sequential deposition as a route to high-performance perovskite-sensitized solar cells

Michael Graetzel, Mohammad Khaja Nazeeruddin, Robin Humphry-Baker, Peng Gao, Peng Gao, Soo-Jin Moon, Norman Pellet, Julian Burschka

Following pioneering work(1), solution-processable organic-inorganic hybrid perovskites-such as CH3NH3PbX3 (X = Cl, Br, I)-have attracted attention as light-harvesting materials for mesoscopic solar cells(2-15). So far, the perovskite pigment has been depo ...

Nature Publishing Group2013

New pyrido[3,4-b]pyrazine-based sensitizers for efficient and stable dye-sensitized solar cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Jacques-Edouard Moser, Pascal Comte, Thomas Moehl, Mateusz Barnaba Wielopolski

A series of new pyrido[3,4-b]pyrazine-based organic sensitizers (PP-I and APP-I–IV) containing different donors and p-spacers have been synthesized and employed in dye-sensitized solar cells (DSSCs). The absorption spectra properties of dyes are analysed b ...

Royal Soc Chemistry2014

Combined Vacuum Evaporation and Solution Process for High-Efficiency Large-Area Perovskite Solar Cells with Exceptional Reproducibility

Michael Graetzel

Organic-inorganic hybrid perovskites exhibit outstanding performances in perovskite solar cells (PSCs). However, the complex solution chemistry of perovskites precursors renders it difficult to prepare large-area devices in a reproducible way, which is a p ...

Wiley-V C H Verlag Gmbh2023

NiCuCoS3 chalcogenide as an efficient electrocatalyst for hydrogen and oxygen evolution

Michael Graetzel, Shaik Mohammed Zakeeruddin

Herein, a newly developed non-noble metal water splitting catalyst based on NiCuCoS3 was reported. Water splitting catalysts are largely developed with noble-based transition metals to lower the energy requirement for the overall water splitting reactions. ...

ELSEVIER2021

Monovalent Cation Doping of CH3NH3PbI3 for Efficient Perovskite Solar Cells

Michael Graetzel, Mohammad Ibrahim Dar, Mojtaba Abdi Jalebi

Here, we demonstrate the incorporation of monovalent cation additives into CH3NH3PbI3 perovskite in order to adjust the optical, excitonic, and electrical properties. The possibility of doping was investigated by adding monovalent cation halides with simil ...

Journal Of Visualized Experiments2017

Solid-state synthesis of CdFe2O4 binary catalyst for potential application in renewable hydrogen fuel generation

Michael Graetzel, Shaik Mohammed Zakeeruddin

Clean energy is highly needed at this time when the energy requirements are rapidly increasing. The observed increasing energy requirement are largely due to continued industrialization and global population explosion. The current means of energy source is ...

Nature Portfolio2022

Carbazole Treated Waterproof Perovskite Films with Improved Solar Cell Performance

Michael Graetzel, Paul Joseph Dyson, Ursula Röthlisberger, Felix Thomas Eickemeyer, Lukas Pfeifer, Virginia Carnevali, Nikolaos Lempesis, Vladislav Slama, Yeonju Kim, Haizhou Lu, Jaeki Jeong

Surface passivation has been widely employed to suppress non-radiative charge recombination and prevent interfacial charge accumulation in perovskite photovoltaics. In this report, carbazole modified with ammonium iodide connected via alkyl chains of diffe ...

Wiley-V C H Verlag Gmbh2024

Dual effect of humidity on cesium lead bromide: enhancement and degradation of perovskite films

Michael Graetzel, Mohammad Ibrahim Dar, Simone Meloni

CsPbBr3 perovskite is highly desired to fabricate many optoelectronic devices: high photovoltage solar cells, tandem solar cells, light-emitting diodes, lasers, photodetectors, field effect transistors etc. However, to realize these applications, resistanc ...

Royal Society of Chemistry2019

Lead immobilization for environmentally sustainable perovskite solar cells

Michael Graetzel, Antonio Abate, Hui Zhang

Lead halide perovskites are promising semiconducting materials for solar energy harvesting. However, the presence of heavy-metal lead ions is problematic when considering potential harmful leakage into the environment from broken cells and also from a publ ...

NATURE PORTFOLIO2023

Near-UV to red-emitting charged bis-cyclometallated iridium(III) complexes for light-emitting electrochemical cells

Michael Graetzel, Mohammad Khaja Nazeeruddin, Rosario Scopelliti, Davide Di Censo

Herein we report a series of charged iridium complexes emitting from near-UV to red using carbene-based (NC)-C-boolean AND: ancillary ligands. Synthesis, photophysical and electrochemical properties of this series are described in detail together with X-ra ...

Royal Society of Chemistry2012

Bis(pyrazol-1-yl)methane as Non-Chromophoric Ancillary Ligand for Charged Bis-Cyclometalated Iridium(III) Complexes

Michael Graetzel, Mohammad Khaja Nazeeruddin, Rosario Scopelliti, Davide Di Censo, Sheng Meng, Il Jung

New charged cyclometalated iridium(III) complexes Ir(ppy)2(L) [ppy = 2-phenylpyridine; L = bis(pyrazol-1-yl)methane (for 1); L = bis(3,5-dimethylpyrazol-1-yl)methane (for 2)] were synthesized and their electrochemical and photophysical properties st ...

Wiley-Blackwell2012

Crystal-Size-Induced Band Gap Tuning in Perovskite Films

Michael Graetzel, Simone Meloni, Wolfgang Richard Tress, Amita Ummadisingu

A comprehensive picture explaining the effect of the crystal size in metal halide perovskite films on their opto-electronic characteristics is currently lacking. We report that perovskite nanocrystallites exhibit a wider band gap due to concurrent quantum ...

Wiley-VCH Verlag GmbH2021

Ionic polarization-induced current–voltage hysteresis in CH3NH3PbX3 perovskite solar cells

Michael Graetzel, Mohammad Khaja Nazeeruddin, Shaik Mohammed Zakeeruddin, Ursula Röthlisberger, Peng Gao, Wolfgang Richard Tress, Thomas Moehl, Michael Saliba, Peng Gao, Yonghui Lee, Simone Meloni, Marius Franckevicius

CH3NH3PbX3 (MAPbX(3)) perovskites have attracted considerable attention as absorber materials for solar light harvesting, reaching solar to power conversion efficiencies above 20%. In spite of the rapid evolution of the efficiencies, the understanding of b ...

Nature Research2016

Spatial Conformation Engineering of Aromatic Ketones for Highly Efficient and Stable Perovskite Solar Cells

Minhuan Wang, Michael Graetzel, Shaik Mohammed Zakeeruddin, Likai Zheng, Xiaoqing Jiang

Carbonyl-containing materials employed in state-of-the-art hybrid lead halide perovskite solar cells (PSCs) exhibit a strong structure-dependent electron donor effect that predominates in defect passivation. However, the impact of the molecular spatial con ...

AMER CHEMICAL SOC2024

Correlating long-lived photogenerated hole populations with photocurrent densities in hematite water oxidation photoanodes

Michael Graetzel, Kevin Sivula

Photogenerated charge carrier dynamics are investigated as a function of applied bias in a variety of different hematite photoanodes for solar water oxidation. Transient absorption spectroscopy is used to probe the photogenerated holes, while transient pho ...

2012

SnS Quantum Dots as Hole Transporter of Perovskite Solar Cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Ulf Anders Hagfeldt, Peng Wang, Yuhang Liu, Dan Ren, Zaiwei Wang, Yang Li

Perovskite solar cells have achieved comparable power conversion efficiencies as commercial silicon cells, making the issue of long-term operation stability as the most critical scientific factor toward industrial realization. In this work, we introduce Sn ...

AMER CHEMICAL SOC2019