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Michael Graetzel

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Publications associées (1 223)

A crystal capping layer for formation of black-phase FAPbI3 perovskite in humid air

Michael Graetzel, Shaik Mohammed Zakeeruddin, Mingyang Wei

Black-phase formamidinium lead iodide (α-FAPbI3) perovskites are the desired phase for photovoltaic applications, but water can trigger formation of photoinactive impurity phases such as δ-FAPbI3. We show that the classic solvent system for perovskite fabr ...

2024

Helical interfacial modulation for perovskite photovoltaics

Michael Graetzel, Shaik Mohammed Zakeeruddin, Jovana Milic, Marco Alejandro Ruiz Preciado, Felix Thomas Eickemeyer, Hong Zhang

Hybrid metal halide perovskites have demonstrated remarkable performances in modern photovoltaics, although their stabilities remain limited. We assess the capacity to advance their properties by relying on interfacial modulators featuring helical chiralit ...

Royal Soc Chemistry2024

Phase-stable indium sulfide achieves an energy conversion efficiency of 14.3% for solar-assisted carbon dioxide reduction to formate

Michael Graetzel, Jingshan Luo, Xiaoyu Zhang, Jing Gao, Qixing Zhang, Jun Li

Tremendous efforts have been made in developing highly selective catalysts for electrochemical CO 2 conversion to formate. However, the rapid deactivation resulting from structural reconstruction and phase transition poses considerable challenges to the sy ...

Cell Press2024

High-efficiency and thermally stable FACsPbI3 perovskite photovoltaics

Michael Graetzel, Mingyang Wei

α-FA1−xCsxPbI3 is a promising absorbent material for efficient and stable perovskite solar cells (PSCs)1,2. However, the most efficient α-FA1−xCsxPbI3 PSCs require the inclusion of the additive methylammonium chloride3,4, which generates volatile organic r ...

2024

Improving the operational stability of perovskite solar cells with cesium-doped graphene oxide interlayer

Michael Graetzel, Shaik Mohammed Zakeeruddin, Rita Therisod, Mostafa Rabie Shlaly Bahr Othman, Masaud Hassan S Almalki, Felix Thomas Eickemeyer, Hong Zhang, Lukas Pfeifer, Christian Michael Wolff

Perovskite solar cells (PSCs) have made great advances in terms of power conversion efficiency (PCE), yet their subpar stability continues to hinder their commercialization. The interface between the perovskite layer and the charge-carrier transporting lay ...

Elsevier2024

Buried Interface Engineering Enables Efficient and 1,960‐hour Isos‐L‐2i Stable Inverted Perovskite Solar Cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Ursula Röthlisberger, Xiong Li, Mathias Dankl, Felix Thomas Eickemeyer, Nikolaos Lempesis, Mingyang Wei, Virginia Carnevali, Lorenzo Agosta, Lin Li

High-performance perovskite solar cells (PSCs) typically require interfacial passivation, yet this is challenging for the buried interface, owing to the dissolution of passivation agents during the deposition of perovskites. Here, this limitation is overco ...

Wiley2024

Spatial Conformation Engineering of Aromatic Ketones for Highly Efficient and Stable Perovskite Solar Cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Likai Zheng, Xiaoqing Jiang

Carbonyl-containing materials employed in state-of-the-art hybrid lead halide perovskite solar cells (PSCs) exhibit a strong structure-dependent electron donor effect that predominates in defect passivation. However, the impact of the molecular spatial con ...

AMER CHEMICAL SOC2024

Research data supporting "High carrier mobility along the [111] orientation in Cu2O photoelectrodes"

Michael Graetzel, Paul Joseph Dyson, Ulf Anders Hagfeldt, Jingshan Luo, Linfeng Pan, Lu Chen, Dan Ren, Meng Xia

Included in the dataset are detailed information into the crystallography, morphology, electronic properties, (photo)electrochemical and carrier dynamics of both single-crystal Cu2O thin films and polycrystalline Cu2O with favored crystal orientations. Mul ...

Apollo - University of Cambridge Repository2024

Graphene-Templated Achiral Hybrid Perovskite for Circularly Polarized Light Sensing

Michael Graetzel, Anurag Krishna, Georgios Kakavelakis

This study points out the importance of the templating effect in hybrid organic-inorganic perovskite semiconductors grown on graphene. By combining two achiral materials, we report the formation of a chiral composite heterostructure with electronic band sp ...

2024

High carrier mobility along the [111] orientation in Cu2O photoelectrodes

Michael Graetzel, Paul Joseph Dyson, Ulf Anders Hagfeldt, Linfeng Pan, Lu Chen, Dan Ren, Meng Xia

Solar fuels offer a promising approach to provide sustainable fuels by harnessing sunlight(1,2). Following a decade of advancement, Cu2O photocathodes are capable of delivering a performance comparable to that of photoelectrodes with established photovolta ...

Nature Portfolio2024

[Correction] High carrier mobility along the [111] orientation in Cu2O photoelectrodes (vol 628, pg 765, 2024)

Michael Graetzel, Paul Joseph Dyson, Ulf Anders Hagfeldt, Linfeng Pan, Lu Chen, Dan Ren, Meng Xia

NATURE PORTFOLIO2024

Upgrading Spiro-OMeTAD with β-Chloroethylcarbazole to Improve the Stability of Perovskite Solar Cells

Michael Graetzel, Yuhang Liu, Haizhou Lu, Jialin Wang

Spiro-OMeTAD has served as a crucial hole transporting material (HTM) in the advancement of efficient perovskite solar cells (PSCs). However, the diminished thermal stability of lithium-doped Spiro-OMeTAD (Li-Spiro) has been a limiting factor, leading to a ...

AMER CHEMICAL SOC2024

Boosting Interfacial Electron Transfer and CO2 Enrichment on ZIF-8/ZnTe for Selective Photoelectrochemical Reduction of CO2 to CO

Michael Graetzel, Shaik Mohammed Zakeeruddin, Dan Ren

Artificial photosynthesis is an effective way of converting CO2 into fuel and high value-added chemicals. However, the sluggish interfacial electron transfer and adsorption of CO2 at the catalyst surface strongly hamper the activity and selectivity of CO2 ...

2024

High-Performance Perovskite Solar Cells with Zwitterion-Capped-ZnO Quantum Dots as Electron Transport Layer and NH4X (X = F, Cl, Br) Assisted Interfacial Engineering

Michael Graetzel, Shaik Mohammed Zakeeruddin, Mounir Driss Mensi, Thomas Paul Baumeler, Essa Awadh R Alharbi, Rashmi Runjhun, Felix Thomas Eickemeyer, Viktor Skorjanc, Anurag Krishna, Georgios Kakavelakis

The systematic advances in the power conversion efficiency (PCE) and stability of perovskite solar cells (PSCs) have been driven by the developments of perovskite materials, electron transport layer (ETL) materials, and interfacial passivation between the ...

Wiley2024

Formamidinium Incorporates into Rb-based Non-Perovskite Phases in Solar Cell Formulations

Michael Graetzel, David Lyndon Emsley, Michael Allan Hope, Lukas Pfeifer, Ümmügülsüm Günes, Yuxuan Zhang, Likai Zheng

Organic-inorganic hybrid perovskite materials, such as formamidinium lead iodide (FAPbI3), are among the most promising emerging photovoltaic materials. However, the spontaneous phase transition from the photoactive perovskite phase to an inactive non-pero ...

Wiley-VCH Verlag GmbH2024

Advanced High-Throughput Rational Design of Porphyrin-Sensitized Solar Cells Using Interpretable Machine Learning

Michael Graetzel, Shaik Mohammed Zakeeruddin, Aswani Yella

Accurately predicting the power conversion efficiency (PCE) in dye-sensitized solar cells (DSSCs) represents a crucial challenge, one that is pivotal for the high throughput rational design and screening of promising dye sensitizers. This study presents pr ...

2024

Combined Vacuum Evaporation and Solution Process for High-Efficiency Large-Area Perovskite Solar Cells with Exceptional Reproducibility

Michael Graetzel

Organic-inorganic hybrid perovskites exhibit outstanding performances in perovskite solar cells (PSCs). However, the complex solution chemistry of perovskites precursors renders it difficult to prepare large-area devices in a reproducible way, which is a p ...

Wiley-V C H Verlag Gmbh2023

Double Layer Composite Electrode Strategy for Efficient Perovskite Solar Cells with Excellent Reverse-Bias Stability (vol 15, 12, 2022)

Michael Graetzel, Chenyi Yi, Wolfgang Richard Tress

2023

Ion-Dipole Interaction Enabling Highly Efficient CsPbI3 Perovskite Indoor Photovoltaics

Michael Graetzel, Shaik Mohammed Zakeeruddin, Di Zhang, Meng Li, Xiaoyan Wang, Haizhou Lu, Xingyu Gao, Ziyun Wang, Jie Chen

Metal halide perovskites are ideal candidates for indoor photovoltaics (IPVs) because of their easy-to-adjust bandgaps, which can be designed to cover the spectrum of any artificial light source. However, the serious non-radiative carrier recombination und ...

Wiley-V C H Verlag Gmbh2023

Surface Passivation of FAPbI3-Rich Perovskite with Cesium Iodide Outperforms Bulk Incorporation

Michael Graetzel, Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Mounir Driss Mensi, Jun Ho Yum, Kevin Sivula, Thomas Paul Baumeler, Essa Awadh R Alharbi, Brian Irving Carlsen, Jing Gao, George Cameron Fish, Felix Thomas Eickemeyer, Lukas Pfeifer, Georgios Kakavelakis

Metal halide perovskites (MHPs) have shown an incredible increase in efficiency, reaching as high as 25.7%, which now competes with traditional photovoltaic technologies. Herein, we excluded CsX and RbX (X = I–, Br–, Cl–), the most commonly used cations to ...

2023

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