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Publications associées (29)

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Atomic-Step Enriched Ruthenium-Iridium Nanocrystals Anchored Homogeneously on MOF-Derived Support for Efficient and Stable Oxygen Evolution in Acidic and Neutral Media

Vasiliki Tileli, Bo Li, Junjie Li

Achieving an efficient and stable oxygen evolution reaction (OER) in an acidic or neutral medium is of paramount importance for hydrogen production via proton exchange membrane water electrolysis (PEM-WE). Supported iridium-based nanoparticles (NPs) are th ...

AMER CHEMICAL SOC2021

Systematic design of millisecond gasification reactor for the incorporation of gas-sieving nanopores in single-layer graphene

Kumar Varoon Agrawal, Luis Francisco Villalobos Vazquez de la Parra, Shiqi Huang, Shaoxian Li, Kuang-Jung Hsu

Etching an ensemble of vacancy defects (nanopores) in single-layer graphene (SLG) to obtain a high density of nanopores with an effective size that enables high-performance gas sieving is challenging. This is because nanopore nucleation and expansion are u ...

2021

Centimeter-scale gas-sieving nanoporous single-layer graphene membrane

Kumar Varoon Agrawal, Shiqi Huang, Mostapha Dakhchoune, Guangwei He, Luc Sébastien Bondaz, Wan-Chi Lee

High-permeance, molecular-sieving, nanoporous single-layer graphene (NSLG) membranes are highly promising for gas separation. However, the formation of cracks during the transfer of NSLG to a low-cost porous support is difficult to avoid. These cracks are ...

2020

Electrochemical performance of polymer-derived SiOC and SiTiOC ceramic electrodes for artificial cardiac pacemaker applications

Jürgen Brugger, Fatemeh Navaee, Jongmoon Jang, Lorenz Hagelüken

In an implantable electrode, such as a pacemaker electrode, fibrotic tissue formation due to a foreign body reaction is an important challenge affecting the efficiency to transmit the electrical signal of the device. The chemical inertness, biocompatibilit ...

2020

Synthesis of metal oxide photoanodes for water splitting using nanocrystals as precursors

Chethana Janardhana Gadiyar

Photoelectrochemical (PEC) water splitting devices are envisioned to play a key role in the societal transition towards sustainable energy sources. In this context, multinary metal oxide semiconductors are the most promising candidates for the role of phot ...

EPFL2020

Polybenzimidazole copolymer derived lacey carbon film for graphene transfer and contamination removal strategies for imaging graphene nanopores

Kumar Varoon Agrawal, Luis Francisco Villalobos Vazquez de la Parra, Shiqi Huang, Mostapha Dakhchoune, Guangwei He, Wan-Chi Lee

The study of the nanometer-scale vacancy defects (nanopores) in graphene by transmission electron microscopy (TEM) is severely hindered by the presence of polymeric residues originating from the graphene-transfer-step to the TEM grid. The state-of-the-art ...

2020

Crystallization of gas-selective nanoporous graphene by competitive etching and growth: a modeling study

Kumar Varoon Agrawal, Mojtaba Chevalier

A robust synthesis methodology for crystallizing nanoporous single-layer graphene hosting a high density of size-selective nanopores is urgently needed to realize the true potential of two-dimensional membranes for gas separation. Currently, there are no c ...

Nature Research2019

A Continuous-flow Photocatalytic Reactor for the Precisely Controlled Deposition of Metallic Nanoparticles

Sina Abdolhosseinzadeh

In this work, a novel photocatalytic reactor for the pulsed and controlled excitation of the photocatalyst and the precise deposition of metallic nanoparticles is developed. Guidelines for the replication of the reactor and its operation are provided in de ...

2019

Post-synthesis deposition of mesoporous niobic acid with improved thermal stability by kinetically controlled sol–gel overcoating

Jeremy Luterbacher, Florent Emmanuel Héroguel, Yuan-Peng Du

Niobia is a well-known solid acid catalyst owing to its intrinsic Brønsted and Lewis acidity. However, catalyst development with this oxide has been limited by our ability to control its pore structure and thermal stability. Here we report a novel post-syn ...

Royal Society of Chemistry2019