Comparison of particle number size distribution trends in ground measurements and climate models

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Highly Hygroscopic Aerosols Facilitate Summer and Early‐Autumn Cloud Formation at Extremely Low Concentrations Over the Central Arctic Ocean

Julia Schmale, Andrea Baccarini

Arctic clouds are sensitive to atmospheric particles since these are sometimes in such low concentrations that clouds cannot always form under supersaturated water vapor conditions. This is especially true in the late summer, when aerosol concentrations ar ...

2024

Influence of Ventilation on Formation and Growth of 1-20 nm Particles via Ozone-Human Chemistry

Dusan Licina, Shen Yang, Marouane Merizak, Meixia Zhang

Ozone reaction with human surfaces is an important source of ultrafine particles indoors. However, 1-20 nm particles generated from ozone-human chemistry, which mark the first step of particle formation and growth, remain understudied. Ventilation and indo ...

Amer Chemical Soc2024

Separation of CO2 and TFE by using diethanolamine and diisopropylamine

Elia Mercedes Ruiz Pachon

The near-azeotrope mixture of TFE and CO2 is an important concern urging the scientific community to develop new ways for TFE/CO2 separations. In this work, for the first time, Diisopropylamine (DIPA) and Diethanolamine (DEA) are used as solvents for separ ...

Taylor & Francis Inc2024

Reducing Aerosol Forcing Uncertainty by Combining Models With Satellite and Within-The-Atmosphere Observations: A Three-Way Street

Athanasios Nenes

Aerosol forcing uncertainty represents the largest climate forcing uncertainty overall. Its magnitude has remained virtually undiminished over the past 20 years despite considerable advances in understanding most of the key contributing elements. Recent wo ...

AMER GEOPHYSICAL UNION2023

A full year of aerosol size distribution data from the central Arctic under an extreme positive Arctic Oscillation: insights from the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition

Julia Schmale, Ivo Fabio Beck, Hélène Paule Angot, Lubna Dada, Jakob Boyd Pernov, Benjamin Jérémy Laurent Heutte

The Arctic environment is rapidly changing due to accelerated warming in the region. The warming trend is driving a decline in sea ice extent, which thereby enhances feedback loops in the surface energy budget in the Arctic. Arctic aerosols play an importa ...

Copernicus Publications2023

Physicochemical characterization and source apportionment of Arctic ice-nucleating particles observed in Ny-Alesund in autumn 2019

Athanasios Nenes, Ghislain Gilles Jean-Michel Motos

Ice-nucleating particles (INPs) initiate primary ice formation in Arctic mixed-phase clouds (MPCs), altering cloud radiative properties and modulating precipitation. For atmospheric INPs, the complexity of their spatiotemporal variations, heterogeneous sou ...

Copernicus GmbH2023

Snow-Atmosphere Humidity Exchange at the Ice Sheet Surface Alters Annual Mean Climate Signals in Ice Core Records

Sonja Wahl

Surface processes alter the water stable isotope signal of the surface snow after deposition. However, it remains an open question to which extent surface post-depositional processes should be considered when inferring past climate information from ice cor ...

Amer Geophysical Union2023

Role of K-feldspar and quartz in global ice nucleation by mineral dust in mixed-phase clouds

Athanasios Nenes

Ice-nucleating particles (INPs) enable ice formation, profoundly affecting the microphysical and radiative properties, lifetimes, and precipitation rates of clouds. Mineral dust emitted from arid regions, particularly potassium-containing feldspar (K-felds ...

Copernicus GmbH2023

Nitrogen oxides in the free troposphere: implications for tropospheric oxidants and the interpretation of satellite NO2 measurements

Ilann Ernest Valentin Bourgeois

Satellite-based retrievals of tropospheric NO(2)columns are widely used to infer NOx (equivalent to NO + NO2) emissions. These retrievals rely on model information for the vertical distribution of NO2. The free tropospheric background above 2 km is particu ...

Copernicus GmbH2023

RaFSIP: Parameterizing ice multiplication in models using a machine learning approach

Athanasios Nenes, Paraskevi Georgakaki

Accurately representing mixed-phase clouds (MPCs) in global climate models (GCMs) is critical for capturing climate sensitivity and Arctic amplification. Secondary ice production (SIP), can significantly increase ice crystal number concentration (ICNC) in ...

2024

The role of secondary ice production in mixed-phase clouds

Paraskevi Georgakaki

Clouds are omnipresent in the Earth's atmosphere. Their phase composition significantly modulates their interaction with solar and terrestrial radiation, as well as precipitation formation. Particularly for clouds containing both phases, known as mixed-pha ...

EPFL2023

Untangling the influence of Antarctic and Southern Ocean life on clouds

Julia Schmale, Hélène Paule Angot, Markus Frey

Polar environments are among the fastest changing regions on the planet. It is a crucial time to make significant improvements in our understanding of how ocean and ice biogeochemical processes are linked with the atmosphere. This is especially true over A ...

2023