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Synthesis of high quality zinc blende CdSe nanocrystals

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Revealing Exciton and Metal–Ligand Conduction Band Charge Transfer Absorption Spectra in Cu-Zn-In-S Nanocrystals

Jacques-Edouard Moser, Etienne Christophe Socie, Brener Rodrigo De Carvalho Vale

Copper indium sulfide quantum dots (QDs) have attracted substantial attention in recent years due to environmental issues and diverse applications. We report the synthesis and characterization of copper-zinc-indium-sulfide (CZIS) QDs and CZIS treated with ...

2020

Spontaneous Formation of CdSe Photoluminescent Nanotubes with Visible-Light Photocatalytic Performance

Martinus Adela Maria Gijs, Virendra Kumar Parashar, Xiaopeng Huang

Two-dimensional (2D) colloidal CdSe nanocrystals (NCs) with precise atomic-scale thickness have attracted intensive attention in recent years due to their optical properties and quantum confinement effects originating from their particular band structure. ...

2019

Direct Observation of Shallow Trap States in Thermal Equilibrium with Band‐Edge Excitons in Strongly Confined CsPbBr 3 Perovskite Nanoplatelets

Jacques-Edouard Moser, Etienne Christophe Socie, Andrés Burgos Caminal, Brener Rodrigo De Carvalho Vale

Lead halide perovskites exhibit great potential for light-emitting devices. Enhanced photoluminescence (PL) is obtained in perovskite materials of reduced dimensionalities due to the large exciton binding energy. However, as the nanocrystal size is reduced ...

2021

Exciton Dynamics and Effects of Structural Order in Morphology-Controlled J-Aggregate Assemblies

Frank Nüesch, Jakob Heier, Surendra Babu Anantharaman

Narrow-band photoluminescence (PL) together with high quantum efficiency from organic molecules is essential for high-color-purity emitters. Supramolecular assemblies like J-aggregates are promising materials due to their narrow PL signal with full-width a ...

2019

Optoelectronic and magnetic properties induced by atomic defects in two-dimensional semiconductors

Alessio Scavuzzo

Two-dimensional (2D) materials have attracted increasing attention over the last decade owing to their remarkable mechanical, electrical and optical properties. Following the groundbreaking discovery of graphene, a plethora of other atomically-thin materia ...

EPFL2020

Physics of optically driven nanojunctions

Philippe Andreas Rölli

Recent years have seen spectacular developments in the domain of nano-optics. Alongside the well-known techniques of super-resolution microscopy progress in nanofabrication has enabled important improvements in the fields of optical imaging and spectros ...

EPFL2020

Photocatalytic ammonia production enhanced by a plasmonic near-field and hot electrons originating from aluminium nanostructures

Olivier Martin, Christian Santschi, Madasamy Thangamuthu

Ammonia production at room temperature and atmospheric pressure is in high demand to assist in energy saving and the protection of the environment worldwide, as well as to help reduce CO2 emissions. Recently, plasmonic nanomaterials have been frequently us ...

2019

Colloidal copper-based nanocrystals: synthesis and mechanistic studies

Valeria Mantella

The growing interest in nanotechnology stems from its promise of developing new materials and devices by taking advantage of unique phenomena emerging at the nanoscale. In this size regime, parameters like size and shape strongly impact the physico-chemica ...

EPFL2020

Toward Bright and Pure Single Photon Emitters at 300 K Based on GaN Quantum Dots on Silicon

Nicolas Grandjean, Raphaël Butté, Gordon Jens Callsen, Sebastian Pascal Tamariz Kaufmann, Johann Nicolaï Stachurski, Kanako Shojiki

Quantum dots (QDs) based on III-nitride semi-conductors are promising for single photon emission at noncryogenic temperatures due to their large exciton binding energies. Here, we demonstrate GaN QD single photon emitters operating at 300 K with g((2)) (0) ...

AMER CHEMICAL SOC2020

Probing Alloy Formation Using Different Excitonic Species: The Particular Case of InGaN

Nicolas Grandjean, Raphaël Butté, Gordon Jens Callsen

Since the early 1960s, alloys are commonly grouped into two classes that feature either bound states in the band gap (I) or additional, nondiscrete band states (II). Consequently, one can observe either excitons bound to isoelectronic impurities or the typ ...

American Physical Society2019

Mechanisms shifting the emission energy of self-assembled quantum dots in nanowires

Luca Francaviglia

This thesis is dedicated to the engineering of the emission energy of quantum dots embedded in core-shell GaAs-AlGaAs nanowires. The goal is to redshift the quantum-dot emission energy in resonance with a gas of Rb atoms. Segregation processes on the nanow ...

EPFL2019

Quasi-Heteroface Perovskite Solar Cells

Ulf Anders Hagfeldt, Peng Wang

Perovskite solar cells (PSCs) have attracted unprecedented attention due to their rapidly rising photoelectric conversion efficiency (PCE). In order to further improve the PCE of PSCs, new possible optimization path needs to be found. Here, quasi-heterofac ...

WILEY-V C H VERLAG GMBH2020

Tailored-Potential Semiconductor Quantum Nanostructures Grown in Inverted Pyramids

Mikhail Lazarev

We have focused on the ability to tune the aluminum (Al) content of the AlGaAs alloy along the growth direction in inverted pyramids (by MOVPE), thus tailoring the potential along a QWR nanostructure. Three parabolic-potential QDs (PQDs) of different poten ...

EPFL2019

Exciton, Biexciton, and Hot Exciton Dynamics in CsPbBr3 Colloidal Nanoplatelets

Jacques-Edouard Moser, Etienne Christophe Socie, Andrés Burgos Caminal, Brener Rodrigo De Carvalho Vale

Lead halide perovskites have emerged as promising materials for light-emitting devices. Here, we report the preparation of colloidal CsPbBr3 nanoplatelets (3 × 4 × 23 nm3) experiencing a strong quasi-one-dimensional quantum confine- ment. Ultrafast transie ...

2020

Formation and stabilization of all-inorganic perovskites for photovoltaics

Zaiwei Wang

All-inorganic perovskite films hold promise for improving stability of perovskite solar cells. However, the desirable narrow-bandgap inorganic perovskites (such as CsPbI3 and CsPbI2Br) are suffering from the thermodynamic phase instability, as the photoact ...

EPFL2020

Exciton Dynamics in 2D Organic Assemblies for Realization of Next-generation Optoelectronic Devices

Surendra Babu Anantharaman

Supramolecular assemblies of cyanine dye molecules formed by weak van der Waals forces have gained immense attention for their distinct optical properties (high extinction coefficient, narrow absorption and photoluminescence line-width and small Stokes shi ...

EPFL2019

RbF post deposition treatment for narrow bandgap Cu(In, Ga)Se-2 solar cells

Fan Fu

Multi-junction solar cells are known to have a considerably increased efficiency potential over their typical single junction counterparts. In order to produce low cost and lightweight multi-junction devices, the availability of suitable narrow (< 1.1 eV) ...

ELSEVIER SCIENCE SA2019

Charge-carrier Dynamics in Metal Oxides and Hybrid Lead Perovskites investigated by Time-Resolved UV and X-ray Spectroscopy

Thomas Charles Henry Rossi

In modern ultrafast optoelectronic technologies based on wide band gap insulators, the non-equilibrium dynamics of photogenerated charges plays a major role. Unravelling the mechanisms of interaction between these charge carriers and their environment is c ...

EPFL2018

Review on Recent Progress of All-Inorganic Metal Halide Perovskites and Solar Cells

Wolfgang Richard Tress

All-inorganic perovskites are considered to be one of the most appealing research hotspots in the field of perovskite photovoltaics in the past 3 years due to their superior thermal stability compared to their organic-inorganic hybrid counterparts. The pow ...

Wiley-V C H Verlag Gmbh2019