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The attosecond quantum beat of an electronic state superposition was captured in SiH4 using soft-X-Ray attosecond transient-absorption spectroscopy. Its decoher-ence and revival, induced by non-adiabatic vibrational dynamics, were reproduced using MCTDH calculations. (C) 2021 The Author(s)
Nikolaos Stergiopoulos, Vasiliki Bikia, Georgios Rovas