Publications related to Modelling the coupled mercury-halogen-ozone cycle in the central Arctic during spring

Nanocluster Aerosols from Ozone-Human Chemistry Are Dominated by Squalene-Ozone Reactions

Dusan Licina, Shen Yang

Nanocluster aerosols (NCAs,

Amer Chemical Soc2024

Nanocluster aerosol formation via ozone chemistry on worn clothing: Influence of environmental parameters

Dusan Licina, Shen Yang

Nanocluster aerosols (NCA, particles

Pergamon-Elsevier Science Ltd2024

Influence of Ventilation on Formation and Growth of 1-20 nm Particles via Ozone-Human Chemistry

Dusan Licina, Shen Yang, Marouane Merizak, Meixia Zhang

Ozone reaction with human surfaces is an important source of ultrafine particles indoors. However, 1-20 nm particles generated from ozone-human chemistry, which mark the first step of particle formation and growth, remain understudied. Ventilation and indo ...

Amer Chemical Soc2024

Squalene Depletion in Skin Following Human Exposure to Ozone under Controlled Chamber Conditions

Shen Yang

A major component of human skin oil is squalene, a highly unsaturated hydrocarbon that protects the skin from atmospheric oxidants. Skin oil, and thus squalene, is continuously replenished on the skin surface. Squalene is also quickly consumed through reac ...

Amer Chemical Soc2024

Urban boundary-layer flows in complex terrain: Dynamic interactions during a hot and dry summer season in Phoenix, Arizona

Aldo Brandi

Anthropogenic modification of natural landscapes to urban environments impacts land-atmosphere interactions in the boundary layer. Ample research has demonstrated the effect of such landscape transitions on development of the urban heat island (UHI), but c ...

Wiley2024

Data and scripts for "Unraveling secondary ice production in winter orographic clouds through a synergy of in-situ observations, remote sensing and modeling"

Alexis Berne, Satoshi Takahama, Athanasios Nenes, Georgia Sotiropoulou, Anne-Claire Marie Billault--Roux, Paraskevi Georgakaki, Romanos Foskinis, Kunfeng Gao

This repository contains field observations and processed data from the Weather Research and Forecasting (WRF) model simulations and the Cloud Resolving Model Radar Simulator (CR-SIM), alongside scripts designed to reproduce the figures presented in the pa ...

Zenodo2024

Characteristics and sources of fluorescent aerosols in the central Arctic Ocean

Benjamin Jérémy Laurent Heutte, Julia Schmale, Ivo Fabio Beck, Margarida Teles Nogueira Rolo, Hélène Paule Angot, Oliver Müller, Jakob Boyd Pernov, Nora Bergner, Alireza Moallemi, Markus Frey

The Arctic is sensitive to cloud radiative forcing. Due to the limited number of aerosols present throughout much of the year, cloud formation is susceptible to the presence of cloud condensation nuclei and ice nucleating particles (INPs). Primary biologic ...

2024

Atmospheric isoprene measurements reveal larger-than-expected Southern Ocean emissions

Julia Schmale, Andrea Baccarini

Isoprene is a key trace component of the atmosphere emitted by vegetation and other organisms. It is highly reactive and can impact atmospheric composition and climate by affecting the greenhouse gases ozone and methane and secondary organic aerosol format ...

Nature Research2024

Turbulence and Heat exchange in the Near-Surface Boundary Layer over Patchy Snow

Michael Haugeneder

The atmospheric layer adjacent to the earth's surface is of crucial importance for weather models due to the exchange of energy between the surface and the atmosphere. This exchange is dependent on the various surface properties and influences the state of ...

EPFL2024

Good enough: Intermediate complexity atmospheric models improve the representation of processes affecting seasonal snow

Dylan Stewart Reynolds

Snow plays a crucial role in processes regulating ecosystems, the climate, and human development. Mountain snowpack in particular has great relevance for downstream communities. Knowledge about the distribution and properties of the snowpack thus help in p ...

EPFL2024

Reactions of hypobromous acid with dimethyl selenide, dimethyl diselenide and other organic selenium compounds: kinetics and product formation

Urs von Gunten

Selenium (Se) is an essential micronutrient for many living organisms particularly due to its unique redox properties. We recently found that the sulfur (S) analog for dimethyl selenide (DMSe), i.e. dimethyl sulfide (DMS), reacts fast with the marine oxida ...

Royal Soc Chemistry2024

Simulations of primary and secondary ice production during an Arctic mixed-phase cloud case from the Ny-Ålesund Aerosol Cloud Experiment (NASCENT) campaign

Georgia Sotiropoulou, Paraskevi Georgakaki

The representation of Arctic clouds and their phase distributions, i.e., the amount of ice and supercooled water, influences predictions of future Arctic warming. Therefore, it is essential that cloud phase is correctly captured by models in order to accur ...

Copernicus GmbH2024

Snowfall deposition in mountainous terrain: a statistical downscaling scheme from high-resolution model data on simulated topographies

Michael Lehning

One of the primary causes of non-uniform snowfall deposition on the ground in mountainous regions is the preferential deposition of snow, which results from the interaction of near-surface winds with topography and snow particles. However, producing high-r ...

Frontiers Media Sa2024

Widespread detection of chlorine oxyacids in the Arctic atmosphere

Julia Schmale, Ivo Fabio Beck, Hélène Paule Angot

Observations are reported of HClO3 and HClO4 in the atmosphere and their widespread occurrence over the pan-Arctic during spring, providing further insights into atmospheric chlorine cycling in the polar environment. ...

Nature Portfolio2023

Low ozone dry deposition rates to sea ice during the MOSAiC field campaign: Implications for the Arctic boundary layer ozone budget

Julia Schmale, Ivo Fabio Beck, Hélène Paule Angot

Dry deposition to the surface is one of the main removal pathways of tropospheric ozone (O3). We quantified for the first time the impact of O3 deposition to the Arctic sea ice on the planetary boundary layer (PBL) O3 concentration and budget using year-ro ...

2023

Critical Review on Bromate Formation during Ozonation and Control Options for Its Minimization

Urs von Gunten

Ozone is a commonly applied disinfectant and oxidantin drinkingwater and has more recently been implemented for enhanced municipalwastewater treatment for potable reuse and ecosystem protection. Onedrawback is the potential formation of bromate, a possible ...

AMER CHEMICAL SOC2023

RaFSIP: Parameterizing ice multiplication in models using a machine learning approach

Athanasios Nenes, Paraskevi Georgakaki

Accurately representing mixed-phase clouds (MPCs) in global climate models (GCMs) is critical for capturing climate sensitivity and Arctic amplification. Secondary ice production (SIP), can significantly increase ice crystal number concentration (ICNC) in ...

2024

A full year of aerosol size distribution data from the central Arctic under an extreme positive Arctic Oscillation: insights from the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition

Benjamin Jérémy Laurent Heutte, Federico Bianchi, Julia Schmale, Ivo Fabio Beck, Lubna Dada, Hélène Paule Angot, Jakob Boyd Pernov

The Arctic environment is rapidly changing due to accelerated warming in the region. The warming trend is driving a decline in sea ice extent, which thereby enhances feedback loops in the surface energy budget in the Arctic. Arctic aerosols play an importa ...

Copernicus Publications2023

Arctic tropospheric ozone: assessment of current knowledge and model performance

Luca Pozzoli, Jakob Boyd Pernov, Ilann Ernest Valentin Bourgeois

As the third most important greenhouse gas (GHG) after carbon dioxide (CO2) and methane (CH4), tropospheric ozone (O3) is also an air pollutant causing damage to human health and ecosystems. This study brings together recent research on observations and mo ...

Copernicus Publications2023

Evaluation of the role of superoxide radical as chain carrier for the formation of hydroxyl radical during ozonation

Gang Yu, Urs von Gunten, Yan Wang

Superoxide radicals (O-2(center dot-)) have been suggested as an important chain carrier in the radical chain reaction that promotes ozone (O-3) decomposition to hydroxyl radicals ((OH)-O-center dot) during ozonation. However, due to the difficulty in meas ...

PERGAMON-ELSEVIER SCIENCE LTD2023