Picosecond solvation dynamics of alkali cations in superfluid 4He nanodroplets

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The alkali halides are ionic compounds. Each alkali atom donates an electron to a halogen atom, leading to ions with full shells. The valence band is mainly located on halogen atoms, while, in a traditional picture, the conduction band is mainly located on ...

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The angular momentum of rotating superfluid droplets originates from quantized vortices and capillary waves, the interplay between which remains to be uncovered. Here, the rotation of isolated submicrometer superfluid He-4 droplets is studied by ultrafast ...

The relaxation of photoexcited nanosystems is a fundamental process of light–matter interaction. Depending on the couplings of the internal degrees of freedom, relaxation can be ultrafast, converting electronic energy in a few fs, or slow, if the energy is ...

Metal-Organic Frameworks (MOFs) are an emerging class of materials that consist of metal ions which are linked with organic ligands via coordination bonds to form extended networks. MOF structures consists predominantly of open voids which makes them among ...

This thesis explores the application of semiclassical methods in the study of states with large quantum numbers for theories invariant under internal symmetries. In the first part of the thesis, we study zero-temperature superfluids. These provide a gener ...

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A highly stable nanocomposite of antioxidant activity was developed by immobilization of a superoxide dismutase-mimicking metal complex on copolymer-functionalized nanoclay. The layered double hydroxide (LDH) nanoclays were synthesized and surface modifica ...

The possibility for helium-induced electronic transitions in a photo-excited atom is investigated using Ba+ excited to the 6p 2P state as a prototypical example. A diabatization scheme has been designed to obtain the necessary potential energy surfaces and ...

Microcavity polaritons are hybrid quasiparticles emerging from the strong coupling between quantum well excitons and light in the resonator. Their unique half-light half-matter nature brings in specific properties like low effective mass, nonlinearity due ...

The displacement of water molecule(s) from the inner coordination sphere of [Gd(DTTA–Me)(H2O)2]− (DTTA = ethylenetriamine-N,N,N″,N″-tetraacetate) by fluoride has been studied by multinuclear NMR relaxation (1H, 17O, 19F) and DFT calculations. Fluoride anio ...

The reduction of the nitride-bridged diuranium(IV) complex Cs[{U(OSi((OBu)-Bu-t)(3))(3)}(2)(mu-N)] affords the first example of a uranium nitride complex containing uranium in the +III oxidation state. Two nitride-bridged complexes containing the heteromet ...

The redox chemistry of f-elements is drawing the attention of inorganic chemists due to their unusual reaction pathways. Notably low-valent f-element complexes have been shown to be able to activate small molecules such as CO2 and N2 in mild conditions. Co ...

Multimetallic cooperative binding of heteroallenes provides an attractive route to their activation, but the reduction of CS2 at heterobimetallic sites, associating an electron-rich metal with a main group Lewis acid has not been explored. Here we show tha ...

Whereas most of the phenomena associated with superfluidity have been observed in finite-size helium systems, the nucleation of quantized vortices has proven elusive. Here we show that the solvation of a Ba+ ion created by photoionization of neutral Ba at ...

We report a study of the basal-plane anisotropy of the superfluid density in underdoped YBa2Cu4O8 (Y124), showing the effects of both the CuO2 planes and the fully occupied CuO chains. From small-angle neutron scattering measurements of the vortex lattice, ...

Single crystals of MgCNi3, with areas sized up to 1 mm(2), were grown by the self-flux method using a cubic anvil high-pressure technique. In low applied fields, the dc magnetization exhibited a very narrow transition into the superconducting state, demons ...

The quest for identification and understanding of fractional vorticity is a major subject of research in the quantum fluids domain, ranging from superconductors, superfluid Helium-3 to cold atoms. In a two-dimensional Bose degenerate gas with a spin degree ...

Picosecond solvation dynamics of alkali cations in superfluid 4He nanodroplets

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