Publications associées à Data and code associated with the paper 'Measurement-induced collective vibrational quantum coherence under spontaneous Raman scattering in a liquid'

Publications associées (23)

Measurement-induced collective vibrational quantum coherence under spontaneous Raman scattering in a liquid

Christophe Marcel Georges Galland, Santiago Tarrago Velez, Valeria Vento, Anna Pogrebna

Spontaneous Raman scattering is classically understood as an incoherent process. Here, the authors demonstrate that macroscopic quantum coherence among billions of vibrating molecules in a liquid is generated when single photon detection and single spatio- ...

Nature Research2023

Mode-Specific Coupling of Nanoparticle-on-Mirror Cavities with Cylindrical Vector Beams

Christophe Marcel Georges Galland, Sachin Suresh Verlekar, Valeria Vento, Philippe Andreas Rölli

Nanocavities formed by ultrathin metallic gaps permitthe reproducibleengineering and enhancement of light-matter interaction, withmode volumes reaching the smallest values allowed by quantum mechanics.While the enhanced vacuum field in metallic nanogaps ha ...

2023

Charge transfer across C-H center dot center dot center dot O hydrogen bonds stabilizes oil droplets in water

Sylvie Roke, Saranya Pullanchery Sankara Narayanan, Sergey Kulik, Benjamin Rehl

The hydrophobic-water interface plays a key role in biological interactions. However, both the hydrophobic-water interfacial molecular structure and the origin of the negative zeta potential of hydrophobic droplets in water are heavily contested. We report ...

American Association for the Advancement of Science2021

Long decay length of magnon-polarons in BiFeO3/La0.67Sr0.33MnO3 heterostructures

Jean-Philippe Ansermet, Dirk Grundler, Peng Gao, Haiming Yu, Mohammad Hamdi

Magnons can transfer information in metals and insulators without Joule heating, and therefore are promising for low-power computation. The on-chip magnonics however suffers from high losses due to limited magnon decay length. In metallic thin films, it is ...

Nature Research2021

A cryogenic electro-optic interconnect for superconducting devices

Tobias Kippenberg, Anton Lukashchuk, Nathan Rafaël Bernier, Liu Qiu, Itay Shomroni, Amir Youssefi, Philipp Johann Uhrich

A major challenge to the scalability of cryogenic computing platforms is the heat load associated with the growing number of electrical cable connections between the superconducting circuitry and the room-temperature environment. Compared with electrical c ...

2021

Magnons, worms and nanogratings in artificial magnetic quasicrystals

Sho Watanabe

Magnons (spin waves, SWs) are elementary spin excitations in magnetically ordered materials. They are the promising quanta for the transmission and processing of information. Magnons can be coupled to the electromagnetic waves utilized for the wireless com ...

EPFL2021

Nanophotonic supercontinuum-based mid-infrared dual-comb spectroscopy

Luc Thévenaz, Tobias Kippenberg, Camille Sophie Brès, Junqiu Liu, Hairun Guo, Wenle Weng, Wolfgang Hänsel

High resolution and fast detection of molecular vibrational absorption is important for organic synthesis, pharmaceutical processes, and environmental monitoring, and is enabled by mid-infrared (mid-IR) laser frequency combs via dual-comb spectroscopy. Her ...

2020

Effects of Ball Milling and TiF3 Addition on the Dehydrogenation Temperature of Ca(BH4)2 Polymorphs

Andreas Züttel

The changes introduced by both ball milling and the addition of small amounts of TiF3 in the kinetics of the hydrogen desorption of three different Ca(BH4)2 polymorphs (α, β and γ) have been systematically investigated. The samples with different polymorph ...

2020

Fabrication of Sub-10-nm Plasmonic Gaps for Ultra-Sensitive Raman Spectroscopy

Hatice Altug

The past two decades have witnessed the explosion of activities in the field of surface enhanced Raman spectroscopy (SERS). SERS platforms employ nano-structures that excite plasmonic modes with large local electromagnetic fields localized within small gap ...

SPRINGER2020

Exchange Interactions Mediated by Nonmagnetic Cations in Double Perovskites

Henrik Moodysson Rønnow, Oleg Yazyev, Peter Babkevich, Sami Juhani Vasala, Vamshi Mohan Katukuri

Establishing the physical mechanism governing exchange interactions is fundamental for exploring exotic phases such as quantum spin liquids in real materials. In this Letter, we address exchange interactions in Sr2CuTexW1-xO6, a series of double perovskite ...

AMER PHYSICAL SOC2020

Scale-invariant magnetic anisotropy in RuCl(3)at high magnetic fields

Philip Johannes Walter Moll

Scale-invariant magnetic anisotropy in RuCl(3)has been revealed through measurements of its magnetotropic coefficient, providing evidence for a high degree of exchange frustration that favours the formation of a spin liquid state. In RuCl3, inelastic neutr ...

2020

Fast remote correlation experiments for 1H homonuclear decoupling in solids

David Lyndon Emsley, Pinelopi Moutzouri, Bruno Simões de Almeida

In 1H MAS spectra, the residual homogeneous broadening under MAS is due to a combination of higher-order shifts and splittings. We have recently shown how the two-dimensional anti-z-COSY experiment can be used for the removal of the splittings. However, th ...

Academic Press Inc - Elsevier Science2020

Reducing uncertainties in energy dissipation measurements in atomic force spectroscopy of molecular networks and cell-adhesion studies

Georg Fantner, Blake William Erickson, Samuel Mendes Leitão, Soma Biswas

Atomic force microscope (AFM) based single molecule force spectroscopy (SMFS) is a valuable tool in biophysics to investigate the ligand-receptor interactions, cell adhesion and cell mechanics. However, the force spectroscopy data analysis needs to be done ...

Nature Research2018

Multilaser Conformer-Selective Spectroscopy of Cold Biomolecular Ions in the Gas Phase

Aleksandr Pereverzev

Proteins and even small peptides play crucial role in almost any biological. Biological activity and functionality of these building blocks of life are determined not only by their primary structure, but also by their 3D orientation â secondary, tertiary ...

EPFL2017

Quantum-state-resolved reactivity of overtone excited CH4 on Ni(111): Comparing experiment and theory

Rainer Beck, Phil Morten Hundt, Maarten Eduard van Reijzen

Quantum state resolved reactivity measurements probe the role of vibrational symmetry on the vibrational activation of the dissociative chemisorption of CH4 on Ni(111). IR-IR double resonance excitation in a molecular beam was used to prepare CH4 in three ...

American Institute of Physics2017

Raman Self-Frequency Shift of Dissipative Kerr Solitons in an Optical Microresonator

Tobias Kippenberg, Maxim Karpov, Martin Hubert Peter Pfeiffer, Hairun Guo, Arne Kordts, Victor Brasch, Michail Zervas, Michael Wolfgang Geiselmann

The formation of temporal dissipative Kerr solitons in microresonators driven by a continuous-wave laser enables the generation of coherent, broadband, and spectrally smooth optical frequency combs as well as femtosecond pulse sources with compact form fac ...

American Physical Society2016

Unraveling the weak hydrogen bonds of ethynylpyridines and ethynylbenzene with trimethylphosphate - A combined FT-Raman spectroscopic and quantum-chemical study

Tomislav Horvat

The interplay of secondary hydrogen bonds of 2- and 3-ethynylpyridine or ethynylbenzene with trimethylphosphate in tetrachloroethene was elucidated using FT-Raman spectroscopy and MP2/6-311 + G(d,p) calculations. The direct participation of C C moiety in t ...

Elsevier Science Bv2016

Experimental characterization of a prototype secondary spectrometer for vertically scattering multiple energy analysis at cold-neutron triple axis spectrometers

Felix Groitl

A thorough experimental characterization of a multiplexing backend with multiple energy analysis on a cold-neutron triple axis spectrometer (cTAS) is presented. The prototype employs two angular segments (2 theta-segments) each containing five vertically s ...

Elsevier2016

Second-Harmonic Scattering as a Probe of Structural Correlations in Liquids

Michele Ceriotti, Sylvie Roke, David Mark Wilkins, Gabriele Tocci, Chung-Wen Liang

econd-harmonic scattering experiments of water and other bulk molecular liquids have long been assumed to be insensitive to interactions between the molecules. The measured intensity is generally thought to arise from incoherent scattering due to individua ...

Amer Chemical Soc2016

Negative plasmon dispersion in 2H-NbS2 beyond the charge-density-wave interpretation

Helmuth Berger

We examine the experimental and theoretical electron-energy loss spectra in 2H-Cu0.2NbS2 and find that the 1 eV plasmon in this material does not exhibit the regular positive quadratic plasmon dispersion that would be expected for a normal broad-parabolic- ...

Iop Publishing Ltd2016