Publication

Photoelectron Spectroscopy of Doped Helium Droplets

Publications associées (30)

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Photoelectrons produced from the excitation of spin-degenerate states in solids can have a sizable spin polarization, which is related to the phase of interfering channels in the photoemission matrix elements. Such spin polarization can be measured by spin ...

Amer Physical Soc2017

Spin-resolved band structure of a densely packed Pb monolayer on Si(111)

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Monolayer structures of Pb on Si(111) attracted recently considerable interest as superconductivity was found in these truly two-dimensional (2D) structures. In this study, we analyzed the electronic surface band structure of the so-called striped incommen ...

Amer Physical Soc2017

Hallmarks of Hunds coupling in the Mott insulator Ca2RuO4

Marco Grioni, Henrik Moodysson Rønnow, Simon Karl Moser, Johan Juul Chang, Claudia Giuseppina Fatuzzo, Gianmarco Gatti

A paradigmatic case of multi-band Mott physics including spin-orbit and Hund's coupling is realized in Ca2RuO4. Progress in understanding the nature of this Mott insulating phase has been impeded by the lack of knowledge about the low-energy electronic str ...

Nature Research2017

Chemical Distribution of Multiple Cation (Rb+, Cs+, MA(+), and FA(+)) Perovskite Materials by Photoelectron Spectroscopy

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Lead-based mixed perovskite materials have emerged in the last couple of years as promising photovoltaic materials. Recently, it was shown that improved material stability can be achieved by incorporating small amounts of inorganic cations (Cs+ and Rb+), p ...

American Chemical Society2017

Valence Level Character in a Mixed Perovskite Material and Determination of the Valence Band Maximum from Photoelectron Spectroscopy: Variation with Photon Energy

Ulf Anders Hagfeldt, Juan-Pablo Correa-Baena, Tor Jesper Jacobsson

A better understanding of the electronic structure of perovskite materials used in photovoltaic devices is essential for their development and optimization. In this investigation, synchrotron-based photoelectron spectroscopy (PES) was used to experimentall ...

American Chemical Society2017

Instability in CH3NH3PbI3 perovskite solar cells due to elemental migration and chemical composition changes

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Organic-inorganic halide perovskites have rapidly grown as favorable materials for photovoltaic applications, but accomplishing long-term stability is still a major research problem. This work demonstrates a new insight on instability and degradation facto ...

Springer Nature2017

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In materials where electrons interact strongly, a number of exotic and exciting phenomena arise. The mechanisms at the base of many of these phenomena remain debated, as strongly correlated electron physics represents one of the biggest challenges for mode ...

EPFL2017

Ultrafast Photoelectron Spectroscopy of Liquid Samples

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This thesis focuses on the commissioning and characterization of HARMONIUM, an ultrafast tunable EUV source based on high-harmonic generation for performing photoelectron spectroscopy of liquids. In ultrafast photoelectron spectroscopy a short pump pulse i ...

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The need to interpret ultraviolet photoemission data strongly motivates the refinement of first-principles techniques that are able to accurately predict spectral properties. In this work, we employ Koopmans-compliant functionals, constructed to enforce pi ...

Amer Chemical Soc2016

A Gibeon meteorite yields a high-performance water oxidation electrocatalyst

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Examining the electrocatalytic performance of naturally-occurring metallic minerals is of interest for energy conversion applications given their unique atomic composition and formation history. Herein, we report the electrocatalytic function of an iron-ba ...

2016