Publications associées à Linking Morphology and Multi-Physical Transport in Structured Photoelectrodes

High-throughput parallel testing of ten photoelectrochemical cells for water splitting: case study on the effects of temperature in hematite photoanodes

Sophia Haussener, Isaac Thomas Holmes-Gentle, Roberto Valenza, Franky Esteban Bedoya Lora

High-throughput testing of photoelectrochemical cells and materials under well-defined operating conditions can accelerate the discovery of new semiconducting materials, the characterization of the phenomena occurring at the semiconductor-electrolyte inter ...

Royal Soc Chemistry2024

Multiphysics model for assessing photoelectrochemical phenomena under concentrated irradiation

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A multiphysics model was developed for a photoelectrochemical (PEC) cell at the device level to simulate water splitting operating under concentrated irradiation (between 50 to 600 kW m−2). The 2D model couples charge, heat, mass, photon, and momentum tran ...

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Zinc carboxylate optimization strategy for extending Al-air battery system's lifetime

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Although Al-air batteries are expected to be the candidates for energy conversion systems in renewable energy market due to the higher energy density, richer reserves, and lighter mass of Al metal, the anode self-discharge is seen as a notorious issue that ...

ELSEVIER SCI LTD2023

Scrutinizing thermally stimulated current transients originating from trapped charges in organic semiconductors: A drift-diffusion study

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AIP Publishing2022

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Electronic synergy to boost the performance of NiCoP-NWs@FeCoP-NSs anodes for flexible lithium-ion batteries

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Research and development of flexible lithium-ion batteries (LIBs) with high energy density and long cycle life for portable and wearable electronic devices has been a cutting-edge effort in recent years. In this paper, a novel flexible self-standing anode ...

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EPFL2022

Multi-configuration evaluation of a megajoule-scale high-temperature latent thermal test-bed

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Thermal energy storage via latent heat provides an energy dense solution and, during discharge, a hot stream at a well-defined temperature. Utilizing metal phase change materials (PCMs) and high-temperature operation might enable fast (dis)charging and app ...

PERGAMON-ELSEVIER SCIENCE LTD2022

Active sites on copper-based catalysts for electrochemical CO2 reduction selectively to C2+ products

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Electric vehicles (EVs) have gained widespread attention in recent years as the dominant strategy for curbing CO2 emissions through transport electrification. Lithium-ion batteries (LIBs) are currently the most suitable and almost exclusively employed ener ...

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SnSb binary alloy induced heterogeneous nucleation within the confined nanospace: Toward dendrite-free, flexible and energy/power dense sodium metal batteries

Dou Du, Yujie Liu

Rechargeable sodium (Na) metal batteries (SMBs) provide an alternative energy-dense, low-cost energy storage system beyond prevailing Li-ion technologies. However, their practical deployment requires the performance evaluation of Na anodes on the device le ...

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Spray Synthesis of CuFeO2 Photocathodes and In-Operando Assessment of Charge Carrier Recombination

Kevin Sivula, Florian Le Formal, Nestor Guijarro Carratala, Yongpeng Liu, Florent Alexandre Boudoire, Charles Roger Jean Lhermitte

Semiconducting delafossite-phase CuFeO2 is a promising photocathode material for solar-driven hydrogen production given its suitable energy levels and established robustness for photoelectrochemical water reduction. Nevertheless, reported methods for prepa ...

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Inorganic and Metal-Organic Heterogeneous Catalysts for Hydrogen Energy Applications

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EPFL2021

Mitigating voltage losses in photoelectrochemical cell scale-up

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In solar water splitting, efforts in scaling up the photoelectrochemical cell beyond laboratory scale have started to attract significant attention. Several large-area devices have been demonstrated, but typically the efficiencies are much lower than their ...

ROYAL SOC CHEMISTRY2020

Synthesis of metal oxide photoanodes for water splitting using nanocrystals as precursors

Chethana Janardhana Gadiyar

Photoelectrochemical (PEC) water splitting devices are envisioned to play a key role in the societal transition towards sustainable energy sources. In this context, multinary metal oxide semiconductors are the most promising candidates for the role of phot ...

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Continuously-fed density currents over impermeable and porous substrates

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Gravity currents are buoyancy-driven flows having a significant impact on the environment and human life. They can be observed in a vast range of natural and anthropogenic scenarios, such as seawater and freshwater, the atmosphere, or industrial processes. ...

EPFL2020

Understanding Surface Recombination Processes Using Intensity-Modulated Photovoltage Spectroscopy on Hematite Photoanodes for Solar Water Splitting

Kevin Sivula, Nestor Guijarro Carratala, Yongpeng Liu

Converting solar energy into hydrogen through photoelectrochemical (PEC) water splitting offers a promising route towards a fully renewable energy economy. A fundamental understanding of photogenerated charge recombination processes in semiconducting photo ...

WILEY-V C H VERLAG GMBH2020

Theoretical maximum photogeneration efficiency and performance characterization of InxGa1-xN/Si tandem water-splitting photoelectrodes

Yannick Kenneth Gaudy, Sophia Haussener

InxGa1-xN is a promising material for flexible and efficient water-splitting photoelectrodes since the bandgap is tunable by modifying the indium content. We investigate the potential of an InxGa1-xN/Si tandem used as a water-splitting photoelectrode. We p ...

2020

Thermal coarsening of individual titanate nanowires and their assemblies: Surface vs. bulk diffusion

Luca Rossi, László Forró, Xavier Berdat, Massimo Spina, Endre Horvath, Laurent Syavoch Bernard, Sergiy Katrych

The thermal coarsening of titanate nanowires was investigated from room temperature to 1000 degrees C by AFM, SEM, XRD and Raman spectroscopy. Phase transformation kinetics and the external morphology were studied in two configurations: i) as individual an ...

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Inflection Phenomenon in Cryogenic MOSFET Behavior

Christian Enz, Farzan Jazaeri, Arnout Lodewijk M Beckers

This brief reports the analytical modeling and measurements of the inflection in the MOSFET transfer characteristics at cryogenic temperatures. Inflection is the inward bending of the drain current versus gate voltage, which reduces the current in weak and ...

2020