Publications associées à Dosimetry modeling and experimental validation for the PETALE program in the CROCUS reactor

Tool Developments in the OpenMC Code: Correlated Sampling and Transient Fission Matrix Approach Coupled to OpenFOAM

Thomas Jean-François Ligonnet, Axel Guy Marie Laureau, Elsa Merle

This article outlines the advancements made in broadening the application scope of the OpenMC neutron transport code to include thermohydraulic coupling and nuclear data uncertainty propagation. These developments primarily involve the incorporation of the ...

Taylor & Francis Inc2024

Neutron-Gamma Noise Measurements in a Zero-Power Reactor Using Organic Scintillators

Andreas Pautz, Oskari Ville Pakari, Vincent Pierre Lamirand

Noise measurements in light water reactor systems aid in generating validation data for integral point kinetic parameter predictions and generating monitoring parameters for reactor safety and safeguards. The CROCUS zero-power reactor has been used to supp ...

Ieee-Inst Electrical Electronics Engineers Inc2024

Gamma noise to non-invasively monitor nuclear research reactors

Pavel Frajtag, Andreas Pautz, Oskari Ville Pakari, Vincent Pierre Lamirand, Tom Mager

Autonomous nuclear reactor monitoring is a key aspect of the International Atomic Energy Agency’s strategy to ensure nonproliferation treaty compliance. From the rise of small modular reactor technology, decentralized nuclear reactor fleets may strain the ...

Nature Research2024

Intra-pin Reaction Rate Measurements in the CROCUS Experimental Reactor

Andreas Pautz, Oskari Ville Pakari, Vincent Pierre Lamirand, Mathieu Hursin, Thomas Jean-François Ligonnet, Tom Mager

In response to the need for validating high-fidelity deterministic neutronics solvers capable of providing pin-resolved neutron flux distributions, intra-pin reaction rates measurements were performed in the CROCUS experimental reactor. A specially designe ...

2024

Experimental study and interpretative modelling of the Power Exhaust in Configurations with Multiple X-Points in TCV

Sophie Danielle Angelica Gorno

Nuclear fusion presents a promising clean energy source to mitigate future energy crises, with magnetic confinement fusion well-positioned to provide a baseload scenario to power future reactors. The unmitigated power exhaust of such reactors threatens its ...

EPFL2024

Gamma-ray Spectroscopy in Low-Power Nuclear Research Reactors

Andreas Pautz, Oskari Ville Pakari, Vincent Pierre Lamirand

Gamma-ray spectroscopy is an effective technique for radioactive material characterization, routine inventory verification, nuclear safeguards, health physics, and source search scenarios. Gamma-ray spectrometers typically cannot be operated in the immedia ...

MDPI2024

Reactivity of Cyanobacteria Metabolites with Ozone: Multicompound Competition Kinetics

Urs von Gunten

Cyanobacterial blooms occur at increasing frequency and intensity, notably in freshwater. This leads to the introduction of complex mixtures of their products, i.e., cyano-metabolites, to drinking water treatment plants. To assess the fate of cyano-metabol ...

Amer Chemical Soc2024

Analysis of the preliminary campaign for the PETALE program

Andreas Pautz, Vincent Pierre Lamirand, Thomas Jean-François Ligonnet, Axel Guy Marie Laureau

The PETALE program aims to provide new experimental data to constrain the stainless steel nuclear data. In this frame, a preliminary measurement campaign has been performed to characterize the neutron flux in key positions of the CROCUS reactor and to deve ...

EDP SCIENCES S A2023

Extension, validation, and optimization of Serpent/DYN3D/ATHLET code system for SFR applications

Vincenzo Anthony Di Nora

The sequence of codes Serpent/DYN3D has been developed by the Helmholtz-Zentrum Dresden-Rossendorf and successfully applied to core static and transient analyses of sodium-cooled fast reactors (SFRs). The successful application of the sequence to SFRs was ...

EPFL2023

Gamma-Blind Fast Neutron Detection for Spent Nuclear Fuel Characterization

Alexander Wolfertz

In this thesis, the development and testing of a system for measuring the axial distribution of fast neutron emission of spent nuclear fuel rods is presented. Emphasis is placed on the novel fast neutron detector used which can reliably work in extremely h ...

EPFL2023

Design of an Instrumented Fuel Rod for Intra-pin Neutron Flux Measurements in the CROCUS Experimental Reactor

Andreas Pautz, Vincent Pierre Lamirand, Mathieu Hursin, Thomas Jean-François Ligonnet, Won Dong Shin, Tom Mager

In response to the need for validating high-fidelity deterministic neutronics solvers capable of pin-resolved neutron flux distributions, an instrumented fuel rod was designed for the experimental reactor CROCUS, operated by EPFL’s Laboratory for Reactor P ...

2023

Operando identification of a side-on nickel superoxide intermediate and the mechanism of oxygen evolution on nickel oxyhydroxide

Xile Hu, Lichen Bai, Seunghwa Lee

The oxygen evolution reaction (OER) is a key electrochemical reac-tion relevant to energy storage. Ni-containing bimetallic oxyhydrox-ides are among the most active OER catalysts in alkaline medium, but the mechanism of OER on pure Ni oxyhydroxide remains ...

ELSEVIER2023

A holistic investigation of photocatalytic hydrogen generation

Sangram Ashok Savant

Photocatalytic (PC) solar hydrogen production is a promising way to provide green hydrogen using only sunlight and abundant reactants such as water. PC approaches use catalytically active semiconductor particles suspended in liquid electrolytes. The partic ...

EPFL2023

Theory-guided development of homogeneous catalysts for the reduction of CO2 to formate, formaldehyde, and methanol derivatives

Anne-Clémence Corminboeuf, Matthew Wodrich, Shubhajit Das, Hanna Hinrika Cramer

The stepwise catalytic reduction of carbon dioxide (CO2) to formic acid, formaldehyde, and methanol opens non-fossil pathways to important platform chemicals. The present article aims at identifying molecular control parameters to steer the selectivity to ...

2023

Phase Transformation-Induced Interfacial Debonding of Silica Inclusions in Iron

Andreas Mortensen, Alejandra Inés Slagter, David Hernandez Escobar, Julie Nathalie S Gheysen

We document that in unstressed, undeformed, samples of pure iron containing silica inclusions precipitated by melt deoxidation, the iron matrix and a small fraction of the silica inclusions are locally separated at room temperature by a void. Thermal cycli ...

Springer2023

HighNESS conceptual design report: Volume II. The NNBAR experiment

Xiaoxue Han, Sheng Xu, Davide Campi, Mina Akhyani

A key aim of the HighNESS project for the European Spallation Source is to enable cutting-edge particle physics experiments. This volume presents a conceptual design report for the NNBAR experiment. NNBAR would exploit a new cold lower moderator to make th ...

Ios Press2023

Reactivity of Bromine Radical with Dissolved Organic Matter Moieties and Monochloramine: Effect on Bromate Formation during Ozonation

Urs von Gunten, Sung Eun Lim

Bromine radical (Br center dot) has been hypothesized to be a key intermediate of bromate formation during ozonation. Once formed, Br center dot further reacts with ozone to eventually form bromate. However, this reaction competes with the reaction of Br c ...

AMER CHEMICAL SOC2023

Design and operational guidelines of solar-driven catalytic conversion of CO2 and H2 to fuels

Sophia Haussener, Sha Li

Sunlight-powered catalytic conversion of CO2 and (green) H2 into fuels and chemicals via Sabatier and reverse water gas shift (RWGS) processes offers a promising solution to reduce greenhouse gas emissions and increase renewable energy utilization. The suc ...

ELSEVIER SCI LTD2023

Monte Carlo analysis of BWR geometries using a cycle check-up methodology

Abdelhamid Dokhane, Hakim Ferroukhi, Alexander Vasiliev, Mathieu Hursin, Dimitri Rochman

Recent fuel anomalies at a Swiss power plant have motivated the development at PSI of the "Cycle Check-Up" (CHUP) methodology which consists in performing Monte Carlo transport calculations using nuclide compositions and thermal-hydraulic boundary conditio ...

Pergamon-Elsevier Science Ltd2023

Regressive Tomography and Direct Regressive Reconstruction: A Research Note

Henri Weisen

Two related methods for inverting line-integrated measurements are presented in this research paper in the context of the recent deuterium-tritium experiments in the JET tokamak. Unlike traditional methods of tomography, these methods rely on making use of ...

2023