Magnetic properties of single crystal beta-TeVO4 with a zigzag chain of magnetic centers (V4+ ions, S = 1/2) are analyzed in the framework of the J(1)-J(2) model. The best agreement with experimental data is obtained for the J(1)-J(2) model with parameters J(1)/k(B) = -38.33K and J(2)/k(B) = 29.48K (g(b) = 2.07, g(a, c) = 1.99). In contrast to the previously used model (a uniform antiferromagnetic spin chain system with J(1)/k(B) = 21.4 K (g(b) = 2.28, g(a, c) = 2.18)), this improved result allows one to consider the object under study as a zigzag chain system with a dominant ferromagnetic exchange between the nearest neighbors and an antiferromagnetic interaction between the next-nearest neighbors. (C) 2015 AIP Publishing LLC.
Olivier Schneider, Aurelio Bay, Guido Haefeli, Tatsuya Nakada, Frédéric Blanc, Lesya Shchutska, Elena Graverini, Sebastian Schulte, Donal Patrick Hill, Marie Theres Christin Bachmayer, Serhii Cholak, Ettore Zaffaroni, Aravindhan Venkateswaran, Luis Miguel Garcia Martin, Vitalii Lisovskyi, Elisabeth Maria Niel, Federico Ronchetti, Radoslav Marchevski, Anni Matilda Kauniskangas, Dimitrios Kaminaris, Raphaël van Laak, Pierre Paul Louis Mayencourt, Brianna Leililani Thielen, Arnaud Merlin Gauthey, Gianluca Zunica, Abdul-Kerim Guseinov, Esteban Curras Rivera, Yifei Song, Roberto Ribatti, Alexandre Brea Rodriguez, Rita De Sousa Ataíde Da Silva