Publications associées à On-the-Fly ab initio Semiclassical Evaluation of Electronic Coherences in Polyatomic Molecules Reveals a Simple Mechanism of Decoherence

Publications associées (31)

Room-Temperature Quantum Optomechanics and Free-Electron Quantum Optics

Quantum optics studies how photons interact with other forms of matter, the understanding of which was crucial for the development of quantum mechanics as a whole. Starting from the photoelectric effect, the quantum property of light has led to the develop ...

EPFL2024

A generalization of the Hawking black hole area theorem

Veronica Sacchi

Hawking's black hole area theorem was proven using the null energy condition (NEC), a pointwise condition violated by quantum fields. The violation of the NEC is usually cited as the reason that black hole evaporation is allowed in the context of semiclass ...

Springer/Plenum Publishers2024

Thermal conductivity of Li 3 PS 4 solid electrolytes with ab initio accuracy

Michele Ceriotti, Federico Grasselli, Davide Tisi, Lorenzo Gigli

The vast amount of computational studies on electrical conduction in solid-state electrolytes is not mirrored by comparable efforts addressing thermal conduction, which has been scarcely investigated despite its relevance to thermal management and (over)he ...

Amer Physical Soc2024

Universality of loop corrected soft theorems in 4d

Biswajit Sahoo

In [1], logarithmic correction to subleading soft photon and soft graviton theorems have been derived in four spacetime dimensions from the ratio of IR-finite S-matrices. This has been achieved after factoring out IR-divergent components from the tradition ...

Springer Nature2023

Advancing Computational Chemistry with Stochastic and Artificial Intelligence Approaches

Justin Villard

Computational chemistry aims to simulate reactions and molecular properties at the atomic scale, advancing the design of novel compounds and materials with economic, environmental, and societal implications. However, the field relies on approximate quantum ...

EPFL2023

A recipe for cracking the quantum scaling limit with machine learned electron densities

Mario Geiger

A long-standing goal of science is to accurately simulate large molecular systems using quantum mechanics. The poor scaling of current quantum chemistry algorithms on classical computers, however, imposes an effective limit of about a few dozen atoms on tr ...

IOP Publishing Ltd2023

Towards a nonperturbative construction of the S-matrix

Francesco Riva, Brian Quinn Henning, Matthew Thomas Walters

We present a nonperturbative recipe for directly computing the S-matrix in strongly-coupled QFTs. The method makes use of spectral data obtained in a Hamiltonian framework and can be applied to a wide range of theories, including potentially QCD. We demons ...

Springer Nature2023

Dynamical nuclear polarization for dissipation-induced entanglement in NV centers

Mayeul Sylvain Chipaux

We propose a practical implementation of a two-qubit entanglement engine which denotes a scheme to generate quantum correlations through purely dissipative processes. On a diamond platform, the electron spin transitions of two nitrogen-vacancy (NV) centers ...

Amer Physical Soc2023

Gravitational causality and the self-stress of photons

Brando Bellazzini

We study causality in gravitational systems beyond the classical limit. Using on-shell methods, we consider the 1-loop corrections from charged particles to the photon energy-momentum tensor - the self-stress - that controls the quantum interaction between ...

Springer Nature2022

Engineering and characterizing nonclassical states of light in quantum optical networks

Kilian Robert Seibold

The exploration of open quantum many-body systems -systems of microscopic size exhibiting quantum coherence and interacting with their surrounding- has emerged as a key research area over the last years. The recent advances in controlling and preserving qu ...

EPFL2022

Semiclassical methods in conformal field theories scrutinized by the epsilon-expansion

Gil Badel

Conformal Field Theories (CFTs) are crucial for our understanding of Quantum Field Theory (QFT). Because of their powerful symmetry properties, they play the role of signposts in the space of QFTs. Any method that gives us information about their structure ...

EPFL2022

Variational Monte Carlo Calculations of A

Giuseppe Carleo

The complexity of many-body quantum wave functions is a central aspect of several fields of physics and chemistry where nonperturbative interactions are prominent. Artificial neural networks (ANNs) have proven to be a flexible tool to approximate quantum m ...

AMER PHYSICAL SOC2021

Hamiltonian truncation in Anti-de Sitter spacetime

João Miguel Augusto Penedones Fernandes, Marco Meineri, Kamran Salehi Vaziri, Matthijs Jan Hogervorst

Quantum Field Theories (QFTs) in Anti-de Sitter (AdS) spacetime are often strongly coupled when the radius of AdS is large, and few methods are available to study them. In this work, we develop a Hamiltonian truncation method to compute the energy spectrum ...

Springer Nature2021

A note on the large charge expansion in 4d CFT

Gabriel Francisco Cuomo

In this letter, we discuss certain universal predictions of the large charge expansion in conformal field theories with U (1) symmetry, mainly focusing on four-dimensional theories. We show that, while in three dimensions quantum fluctuations are responsib ...

2021

Liouvillian spectral collapse in the Scully-Lamb laser model

Fabrizio Minganti

Phase transitions of thermal systems and the laser threshold were first connected more than forty years ago. Despite the nonequilibrium nature of the laser, the Landau theory of thermal phase transitions, applied directly to the Scully-Lamb laser model (SL ...

AMER PHYSICAL SOC2021

Efficient ab initio semiclassical dynamics for linear and nonlinear electronic spectroscopy

Tomislav Begusic

Molecular spectroscopy is an essential experimental technique in both fundamental physical sciences and applied research. For example, electronic spectroscopy, in which light induces a change in the electronic state of a molecule, is a powerful tool for st ...

EPFL2021

Nuclear Quantum Effects: Fast and Accurate

Venkat Kapil

Atomistic simulations are a bottom up approach that predict properties of materials by modelling the quantum mechanical behaviour of all electrons and nuclei present in a system. These simulations, however, routinely assume nuclei to be classical particles ...

EPFL2020

First-principles calculations of charge carrier mobility and conductivity in bulk semiconductors and two-dimensional materials

Samuel Poncé, Feliciano Giustino

One of the fundamental properties of semiconductors is their ability to support highly tunable electric currents in the presence of electric fields or carrier concentration gradients. These properties are described by transport coefficients such as electro ...

IOP PUBLISHING LTD2020

Quantum Measurement of Mechanical Motion close to the Standard Quantum Limit

Liu Qiu

In quantum mechanics, the Heisenberg uncertainty principle places a fundamental limit in the measurement precision for certain pairs of physical quantities, such as position and momentum, time and energy or amplitude and phase. Due to the Heisenberg uncert ...

EPFL2020

Spontaneous conformal symmetry breaking in fishnet CFT

Mikhail Chapochnikov, Georgios Karananas

Quantum field theories with exact but spontaneously broken conformal invariance have an intriguing feature: their vacuum energy (cosmological constant) is equal to zero. Up to now, the only known ultraviolet complete theories where conformal symmetry can b ...

2020