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Cu(In1-xGax)S-2 nanocrystals and films: low-temperature synthesis with size and composition control

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Crystallization and Organic Field-Effect Transistor Performance of a Hydrogen-Bonded Quaterthiophene

Rosario Scopelliti, Anne-Clémence Corminboeuf, Holger Frauenrath, Philippe Bugnon, Stéphane Suarez, Riccardo Petraglia, Jan Gebers, Bilal Özen, Piotr De Silva

Crystalline thin films of pi-conjugated molecules are relevant as the active layers in organic electronic devices. Therefore, materials with enhanced control over the supramolecular arrangement, crystallinity, and thin-film morphology are desirable. Herein ...

2020

Structural and photophysical investigation of single-source evaporation of CsFAPbI(3) and FAPbI(3) perovskite thin films

Mohammad Khaja Nazeeruddin, Hiroyuki Kanda, Albertus Adrian Sutanto, Maria Cristina Momblona Rincón, Nadja Isabelle Desiree Klipfel

Thermal vacuum deposition is a stimulating technique for upscaling perovskite solar cells. However, the operational complexity of multisource vapor deposition (MSVD) and achieving stoichiometric perovskite layers may impede its implementation. The single-s ...

Royal Society of Chemistry2022

High-Performance Lead-Free Solar Cells Based on Tin-Halide Perovskite Thin Films Functionalized by a Divalent Organic

Michael Graetzel, Shaik Mohammed Zakeeruddin, Felix Thomas Eickemeyer, Yuhang Liu

Tin-based halide perovskite solar cells (PSCs) hold the most promise among lead-free PSCs, but they are plagued with inadequate environmental stability and power-conversion efficiency (PCE). Here we demonstrate that the optimum incorporation of a bulky div ...

2020

Semiconducting two dimensional transition metal dichalcogenides via solution-processable routes

Rebekah Anne Wells

Two-dimensional (2D) transition metal dichalcogenides (TMDs) possess remarkable optoelectronic properties which are unique and tunable based on composition and thickness. These materials are posed to revolutionize ultrathin devices across many fields inclu ...

EPFL2022

Applications of vacuum vapor deposition for perovskite solar cells: A progress review

Michael Graetzel

Metal halide perovskite solar cells (PSCs) have made substantial progress in power conversion efficiency (PCE) and stability in the past decade thanks to the advancements in perovskite deposition methodology, charge transport layer (CTL) optimization, and ...

TSINGHUA UNIV PRESS2022

Solution Processing and Self-Organization of PbS Quantum Dots Passivated with Formamidinium Lead Iodide (FAPbI(3))

Frank Nüesch

Solution-processed lead sulfide quantum dots (PbS QDs) are very attractive as NIR-active semiconductors for the fabrication of cost-efficient optoelectronic devices. To control the thin film carrier transport, as well as stability, surface passivation is o ...

2020

Towards Quantitative Interpretation of Fourier-Transform Photocurrent Spectroscopy on Thin-Film Solar Cells

Franz-Josef Haug, Michael Elias Stückelberger, Jakub Holovsky

The method of detecting deep defects in photovoltaic materials by Fourier-Transform Photocurrent Spectroscopy has gone through continuous development during the last two decades. Still, giving quantitative predictions of photovoltaic device performance is ...

2020

Molybdenum disulphide nanoporous membranes as nanofluidic platforms - large-area engineering and study

Michal Daniel Macha

The work demonstrated in this thesis represent the path towards developing the large-scale fabrication of two-dimensional nanoporous membrane devices and use thereof as platforms to study nanoscale physics of water and ion flow through confined channels. M ...

EPFL2022

Increasing Functionality of III-V Nanowires on Silicon Substrates

Wonjong Kim

Progress in nanotechnology, including fabrication and characterization tools, opened up the unprecedented low dimensional materials era, where we can manipulate and structure matter on a size scale that we could not reach before. Due to many interesting pr ...

EPFL2020

On the Response Speed of Narrowband Organic Optical Upconversion Devices

Frank Nüesch, Surendra Babu Anantharaman, Matthias Diethelm, Wei-Hsu Hu

Organic upconversion devices (OUCs) consist of an organic infrared photodetector and an organic visible light-emitting diode (OLED), connected in series. OUCs convert photons from the infrared to the visible and are of use in applications such as process c ...

WILEY-V C H VERLAG GMBH2022

Composition and Interface Engineering of High Performing Perovskite Solar Cells

Mousa Abdulla M E Abuhelaiqa

Perovskite solar cells have been established as a disruptive technology in the domain of photo-voltaics. Their facile, low-temperature processing and high-power conversion efficiency make them stand-out among other mature solar technologies. The performanc ...

EPFL2022

High-Efficiency Silicon Heterojunction Solar Cells: Materials, Devices and Applications

Mathieu Gérard Boccard

Photovoltaic (PV) technology offers an economic and sustainable solution to the challenge of increasing energy demand in times of global warming. The world PV market is currently dominated by the homo-junction crystalline silicon (c-Si) PV technology based ...

2020

In Situ Reflectometry and Diffraction Investigation of the Multiscale Structure of p-Type Polysilicon Passivating Contacts for c-Si Solar Cells

Christophe Ballif, Franz-Josef Haug, Andrea Ingenito, Audrey Marie Isabelle Morisset

The integration of passivating contacts based on a highly doped polycrystalline silicon (poly-Si) layer on top of a thin silicon oxide (SiOx) layer has been identified as the next step to further increase the conversion efficiency of current mainstream cry ...

AMER CHEMICAL SOC2022

Physical vapour deposition of cyanine salts and their first application in organic electronic devices

Frank Nüesch, Jakob Heier, Antonia Neels, Donatas Gesevicius

A symmetrical trimethine indocyanine dye chromophore was modified with the bistriflylimide anion to study the changes in Coulomb interactions, thermal stability and the volatility of the organic salt. The bulky bistriflylimide anion minimizes electrostatic ...

Royal Society of Chemistry2019

Self-Exciting Point Processes: Identification and Control

Michael Mark

This thesis addresses theoretical and practical aspects of identification and subsequent control of self-exciting point processes. The main contributions correspond to four separate scientific papers. In the first paper, we address the challenge of robust ...

EPFL2022

Gallium‐Based Thin Films for Wearable Human Motion Sensors

Stéphanie Lacour, Ivan Furfaro, Laurent Mirko Dejace

Wearable electronic circuits based on the films of gallium and its alloys offer promising implementations in health monitoring and gaming sensing applications. However, the complex rheology of liquid metals makes it challenging to manufacture thin gallium‐ ...

2019

Synthesis, structural and magnetic characterization of thin films of the chiral magnets CoZnMn and FeGe

Anna Kúkol'ová

Skyrmions are topologically protected nanometer-sized magnetic vortices that have sparked interest for future spintronics applications aiming at high-density, high-speed and low-power consuming magnetic memory devices. One type of skyrmions appears in non- ...

EPFL2021

Stress mitigation for adhesively bonded photovoltaics with fibre reinforced polymer composites in load carrying applications

Thomas Keller, Yu Bai

Structural loads, especially in-plane compression, may cause local buckling and debonding of the photovoltaic (PV) cells that are mechanically integrated with structural members and this may lead to degradation in their electrical performance. This paper p ...

ELSEVIER SCI LTD2019

High-temperature annealing effects on molybdenum-silicon contact substrate for vertically structured silicon quantum-dot solar cells

Chien-Jen Yang

This paper studies the applicability of sputtered Molybdenum (Mo) thin films on silicon wafers (Mo-Si) to act as contact substrates for vertically structured Si quantum-dot (QD) solar cells. The compatibility of Mo-Si contact substrate with Si QD material ...

2019

Ligand Locking on Quantum Dot Surfaces via a Mild Reactive Surface Treatment

Raffaella Buonsanti, Aurélien Bornet, Anna Loiudice, Ona Segura Lecina

At the outermost surface of colloidal QDs are organic surface ligands which dynamically bind and release in solution to control the growth kinetics, control the size/shape of the crystals, passivate surface states, and provide colloidal stability through f ...

2021