Publications associées à Frequent new particle formation over the high Arctic pack ice by enhanced iodine emissions

Highly Hygroscopic Aerosols Facilitate Summer and Early‐Autumn Cloud Formation at Extremely Low Concentrations Over the Central Arctic Ocean

Arctic clouds are sensitive to atmospheric particles since these are sometimes in such low concentrations that clouds cannot always form under supersaturated water vapor conditions. This is especially true in the late summer, when aerosol concentrations ar ...

2024

Characteristics and sources of fluorescent aerosols in the central Arctic Ocean

Benjamin Jérémy Laurent Heutte, Julia Schmale, Ivo Fabio Beck, Margarida Teles Nogueira Rolo, Hélène Paule Angot, Oliver Müller, Jakob Boyd Pernov, Nora Bergner, Alireza Moallemi, Markus Frey

The Arctic is sensitive to cloud radiative forcing. Due to the limited number of aerosols present throughout much of the year, cloud formation is susceptible to the presence of cloud condensation nuclei and ice nucleating particles (INPs). Primary biologic ...

2024

New Particle Formation Events Can Reduce Cloud Droplets in Boundary Layer Clouds at the Continental Scale

Athanasios Nenes, Spyros Pandis

New particle formation (NPF) substantially contributes to global cloud condensation nuclei (CCN), and their climate impacts. Individual NPF events are also thought to increase local CCN, cloud droplet number (CDN), and cloud albedo. High resolution simulat ...

Amer Geophysical Union2024

Glucose Enhances Salinity-Driven Sea Spray Aerosol Production in Eastern Arctic Waters

Guangyu Li, Julia Schmale, Athanasios Nenes, André Welti

Sea spray aerosols (SSA) greatly affect the climate system by scattering solar radiation and acting as seeds for cloud droplet formation. The ecosystems in the Arctic Ocean are rapidly changing due to global warming, and the effects these changes have on t ...

2024

Simulations of primary and secondary ice production during an Arctic mixed-phase cloud case from the Ny-Ålesund Aerosol Cloud Experiment (NASCENT) campaign

Georgia Sotiropoulou, Paraskevi Georgakaki

The representation of Arctic clouds and their phase distributions, i.e., the amount of ice and supercooled water, influences predictions of future Arctic warming. Therefore, it is essential that cloud phase is correctly captured by models in order to accur ...

Copernicus GmbH2024

Temperature, humidity, and ionisation effect of iodine oxoacid nucleation

Andrea Baccarini, Lubna Dada, Houssni Lamkaddam, Imad El Haddad

Iodine oxoacids are recognised for their significant contribution to the formation of new particles in marine and polar atmospheres. Nevertheless, to incorporate the iodine oxoacid nucleation mechanism into global simulations, it is essential to comprehend ...

Royal Soc Chemistry2024

The Influence of the Planetary Boundary Layer on the Atmospheric State at an Orographic Site at the Eastern Mediterranean

Athanasios Nenes, Romanos Foskinis, Kunfeng Gao

We studied the influence of the Planetary Boundary Layer (PBL) on the air masses sampled at the mountaintop Hellenic Atmospheric Aerosol and Climate Change station ((HAC) 2 ) at Mount Helmos (Greece) during the Cloud-AerosoL InteractionS in the Helmos back ...

Stockholm Univ Press2024

Influence of Ventilation on Formation and Growth of 1-20 nm Particles via Ozone-Human Chemistry

Dusan Licina, Shen Yang, Marouane Merizak, Meixia Zhang

Ozone reaction with human surfaces is an important source of ultrafine particles indoors. However, 1-20 nm particles generated from ozone-human chemistry, which mark the first step of particle formation and growth, remain understudied. Ventilation and indo ...

Amer Chemical Soc2024

The molecular scale mechanism of deposition ice nucleation on silver iodide

Mária Lbadaoui-Darvas, Athanasios Nenes, André Welti

Heterogeneous ice nucleation is a ubiquitous process in the natural and built environment. Deposition ice nucleation, i.e. heterogeneous ice nucleation that - according to the traditional view - occurs in a subsaturated water vapor environment and in the a ...

Royal Soc Chemistry2024

A Method of Moments Estimator for Interacting Particle Systems and their Mean Field Limit

Andrea Zanoni, Grigorios A. Pavliotis

We study the problem of learning unknown parameters in stochastic interacting particle systems with polynomial drift, interaction, and diffusion functions from the path of one single particle in the system. Our estimator is obtained by solving a linear sys ...

Siam Publications2024

Effects of Hyporheic Exchange and Settlement on the Particle Size Distribution of Colloids

David Andrew Barry, Qihao Jiang

Colloid particle size plays an important role in contaminant adsorption and clogging in the hyporheic zone, but it remains unclear how the particle size changes during the transport of colloids. This study investigated the variation of the particle size of ...

Springer2024

Iodine oxoacids enhance nucleation of sulfuric acid particles in the atmosphere

Andrea Baccarini, Lubna Dada, André Welti, Houssni Lamkaddam, Imad El Haddad, Mihnea Surdu

The main nucleating vapor in the atmosphere is thought to be sulfuric acid (H2SO4), stabilized by ammonia (NH3). However, in marine and polar regions, NH3 is generally low, and H2SO4 is frequently found together with iodine oxoacids [HIOx, i.e., iodic acid ...

American Association for the Advancement of Science2023

Aerosol and dynamical contributions to cloud droplet formation in Arctic low-level clouds

Guangyu Li, Athanasios Nenes, Jörg Wieder, Paraskevi Georgakaki, Ghislain Gilles Jean-Michel Motos

The Arctic is one of the most rapidly warming regions of the globe. Low-level clouds and fog modify the energy transfer from and to space and play a key role in the observed strong Arctic surface warming, a phenomenon commonly termed "Arctic amplification" ...

Copernicus GmbH2023

Arctic warming by abundant fine sea salt aerosols from blowing snow

Xin Yang, Jian Wang, Julia Schmale, Nora Bergner, Markus Frey

The Arctic warms nearly four times faster than the global average, and aerosols play an increasingly important role in Arctic climate change. In the Arctic, sea salt is a major aerosol component in terms of mass concentration during winter and spring. Howe ...

2023

Measurements of aerosol microphysical and chemical properties in the central Arctic atmosphere during MOSAiC

Benjamin Jérémy Laurent Heutte, Julia Schmale, Ivo Fabio Beck, Lubna Dada, Hélène Paule Angot, Nora Bergner

The Arctic environment is transforming rapidly due to climate change. Aerosols’ abundance and physicochemical characteristics play a crucial, yet uncertain, role in these changes due to their influence on the surface energy budget through direct interactio ...

2023

Multi-campaign ship and aircraft observations of marine cloud condensation nuclei and droplet concentrations

Jian Wang, Athanasios Nenes

In-situ marine cloud droplet number concentrations (CDNCs), cloud condensation nuclei (CCN), and CCN proxies, based on particle sizes and optical properties, are accumulated from seven field campaigns: ACTIVATE; NAAMES; CAMP(2)EX; ORACLES; SOCRATES; MARCUS ...

NATURE PORTFOLIO2023

Measurement report: High Arctic aerosol hygroscopicity at sub- and supersaturated conditions during spring and summer

Jakob Boyd Pernov

Aerosol hygroscopic growth and cloud droplet formation influence the radiation transfer budget of the atmosphere and thereby the climate. In the Arctic, these aerosol properties may have a more pronounced effect on the climate compared to the midlatitudes. ...

Copernicus Publications2023

The role of secondary ice production in mixed-phase clouds

Paraskevi Georgakaki

Clouds are omnipresent in the Earth's atmosphere. Their phase composition significantly modulates their interaction with solar and terrestrial radiation, as well as precipitation formation. Particularly for clouds containing both phases, known as mixed-pha ...

EPFL2023

Physicochemical characterization and source apportionment of Arctic ice-nucleating particles observed in Ny-Alesund in autumn 2019

Guangyu Li, Athanasios Nenes, Jörg Wieder, Ghislain Gilles Jean-Michel Motos

Ice-nucleating particles (INPs) initiate primary ice formation in Arctic mixed-phase clouds (MPCs), altering cloud radiative properties and modulating precipitation. For atmospheric INPs, the complexity of their spatiotemporal variations, heterogeneous sou ...

Copernicus GmbH2023

Role of sesquiterpenes in biogenic new particle formation

Federico Bianchi, Andrea Baccarini, Lubna Dada, Imad El Haddad

Biogenic vapors form new particles in the atmosphere, affecting global climate. The contributions of monoterpenes and isoprene to new particle formation (NPF) have been extensively studied. However, sesquiterpenes have received little attention despite a p ...

2023