Publications associées à Valence photoemission

Publications associées (29)

Visualizing hot carrier dynamics by nonlinear optical spectroscopy at the atomic length scale

Probing and manipulating the spatiotemporal dynamics of hot carriers in nanoscale metals is crucial to a plethora of applications ranging from nonlinear nanophotonics to single-molecule photochemistry. The direct investigation of these highly non-equilibri ...

Springer Science and Business Media LLC2025

All Hard X-ray Transient Grating Spectroscopy

Majed Chergui

Optical-domain transient grating (TG) spectroscopy is the ideal tool to investigate transport phenomena in gases, liquids and solids, but it is limited to typically micron-size grating periods. Extreme-Ultraviolet TG has represented a major leap forward to ...

NATURE PORTFOLIO2025

Giant Purcell Broadening and Lamb Shift for DNA-Assembled Near-Infrared Quantum Emitters

Christophe Marcel Georges Galland, Sachin Suresh Verlekar

Controlling the light emitted by individual molecules is instrumental to a number of advanced nanotechnologies ranging from super-resolution bioimaging and molecular sensing to quantum nanophotonics. Molecular emission can be tailored by modifying the loca ...

2025

Achieving Ultra-Broadband Sunlight-Like Emission in Single-Phase Phosphors: The Interplay of Structure and Luminescence

Jean-Claude Bünzli

The quest for artificial light sources mimicking sunlight has been a long-standing endeavor, particularly for applications in anticounterfeiting, agriculture, and color hue detection. Conventional sunlight simulators are often cost-prohibitive and bulky. T ...

Wiley2024

Investigation of Interface Interactions Between Monolayer MoS2 and Metals: Implications on Strain and Surface Roughness

Klaus Kern

Achieving a low contact resistance has been an important issue in the design of two-dimensional (2D) semiconductor-metal interfaces. The metal contact resistance is dominated by interfacial interactions. Here, we systematically investigate 2D semiconductor ...

2024

Thulium-doped fiber cavities for frequency comb generation at 2 micron

Moritz Bartnick

The invention of the laser in the 1960s heralded a new era in photonics. Owing to both, academic and industrial research, photonics technologies have long become part of our everyday life. This PhD thesis explores two subfields of laser technologies: Frequ ...

EPFL2024

Rapid, Sensitive and Selective Optical Glucose Sensing with Stimulated Raman Scattering (SRS)

Christian Enz, Sandro Carrara, Assim Boukhayma, Ata Jedari Golparvar

Optical blood glucose sensing offers pain-free, non-invasive, continuous monitoring with minimum risk of infection since it does not require breaking the skin barrier. Among various optical detection and spectroscopic techniques, only Raman scattering offe ...

IEEE2022

Ultrafast Single-particle Imaging with Intense X-ray Pulses

Christoph Bostedt

Ultrafast single-particle imaging with intense x-ray pulses from free-electron laser sources provides a new approach for visualizing structure and dynamics on the nanoscale. After a short introduction to the novel free-electron laser sources and methods, w ...

SWISS CHEMICAL SOC2022

Anti-Jahn-Teller effect induced ultrafast insulator to metal transition in perovskite BaBiO3

Changpeng Lin

The Jahn-Teller (JT) effect involves the ions M with a degenerate electronic state distorting the corner-sharing MO6 octahedra to lift the degeneracy, inducing strong coupling of electrons to lattice, and mediating the exotic properties in perovskite oxide ...

NATURE PORTFOLIO2022

Continuous-wave frequency upconversion with a molecular optomechanical nanocavity

Christophe Marcel Georges Galland, Tobias Kippenberg, Philippe Andreas Rölli, Sakthi Priya Amirtharaj, Wen Chen, Sachin Suresh Verlekar

Coherent upconversion of terahertz and mid-infrared signals into visible light opens new horizons for spectroscopy, imaging, and sensing but represents a challenge for conventional nonlinear optics. Here, we used a plasmonic nanocavity hosting a few hundre ...

American Association for the Advancement of Science2021

Photoinduced long-lived state in FeSe0.4Te0.6

Alberto Crepaldi

Fe(Sex)Te(1-)x compounds display a rich phase diagram, ranging from the nematicity of FeSe to the (pi, pi) magnetism of FeTe. We focus on FeSe0.4Te0.6, and exploit tr-ARPES to study its ultrafast electron dynamics following photoexcitation by near-infrared ...

ELSEVIER2021

Femtosecond X-ray emission study of the spin cross-over dynamics in haem proteins

Majed Chergui, Giulia Fulvia Mancini, Dominik Kinschel, James Michael Budarz, Boris Sorokin, Oliviero Cannelli, Camila Bacellar Cases Da Silveira, Jérémy Raymond Jean Maurice Rouxel

In haemoglobin the change from the low-spin (LS) hexacoordinated haem to the high spin (HS, S = 2) pentacoordinated domed deoxy-myoglobin (deoxyMb) form upon ligand detachment from the haem and the reverse process upon ligand binding are what ultimately dr ...

Nature Research2020

Structural and Photophysical Templating of Conjugated Polyelectrolytes with Single-Stranded DNA

Ursula Röthlisberger, Polydefkis Diamantis, Natalie Renuka Banerji

A promising approach to influence and control the photophysical properties of conjugated polymers is directing their molecular conformation by templating. We explore here the templating effect of single-stranded DNA oligomers (ssDNAs) on cationic polythiop ...

AMER CHEMICAL SOC2020

Fundamentals and perspectives of ultrafast photoferroic recording

Anna Pogrebna

The ability to switch ferroics (ferro-, ferri-, antiferromagnets, ferroelectrics, multiferroics) between two stable bit states is one of the keystones of modern data storage technology. Due to many new ideas, originating from fundamental research during th ...

2020

Variational approach to time-dependent fluorescence of a driven qubit

Yang Zhao, Lipeng Chen

We employ the Dirac-Frenkel variational principle and the multiple Davydov ansatz to study time-dependent fluorescence spectra of a driven qubit in the weak to strong qubit-reservoir coupling regimes, where both the Rabi frequency and the spontaneous decay ...

AMER PHYSICAL SOC2020

Experimental station Bernina at SwissFEL: condensed matter physics on femtosecond time scales investigated by X-ray diffraction and spectroscopic methods

Christopher Alexander Arrell, Christoph Peter Hauri, Giulia Fulvia Mancini, Jochen Rittmann

The Bernina instrument at the SwissFEL Aramis hard X-ray free-electron laser is designed for studying ultrafast phenomena in condensed matter and material science. Ultrashort pulses from an optical laser system covering a large wavelength range can be used ...

International Union of Crystallography (IUCr)2019

Scattering HCl Molecules from Au(111) and Ag(111) Surfaces

Jan Daniel Geweke

In this thesis, I present an experimental molecular beam surface scattering study of dynamical processes involved when HCl molecules are scattered from Au(111) and Ag(111) surfaces. I investigated vibrational excitation, translational inelasticity and diss ...

EPFL2019

Observation of an Excited B-c(+) State

Christoph Frei, Aurelio Bay, Minh Tâm Tran, François Fleuret, Tatsuya Nakada, Guido Haefeli, Olivier Schneider, Mingkui Wang, Chitsanu Khurewathanakul, Frédéric Blanc, Axel Kuonen, Olivier Göran Girard, Liang Sun, Maxime Schubiger, Brice Emile Maurin, Hang Yin, Greig Alan Cowan, Thi Dung Nguyen, Guillaume Max Pietrzyk, Matthieu Philippe Luther Marinangeli, Vladislav Balagura, Lino Ferreira Lopes, Zhirui Xu, Mark Tobin, Violaine Bellée, Mirco Dorigo, Vincenzo Battista, Maurizio Martinelli, Tommaso Colombo, Guido Andreassi, Plamen Hristov Hopchev, Jian Wang, Liupan An, Preema Rennee Pais, Pavol Stefko, Ho Ling Li, Yi Zhang, Maria Elena Stramaglia, Lei Zhang, Luca Pescatore, Vladimir Macko, Pietro Marino, Simon Van Mulders, Tara Nanut, Ana Bárbara Rodrigues Cavalcante, Federico Leo Redi, Michel De Cian, Sebastian Schulte, Veronica Sølund Kirsebom, Elena Graverini, Maria Vieites Diaz, Yi Wang, Donal Patrick Hill, Renato Quagliani, Aravindhan Venkateswaran, Yiming Li, Vitalii Lisovskyi, Luis Miguel Garcia Martin, Katharina Müller

Using pp collision data corresponding to an integrated luminosity of 8.5 fb(-1) recorded by the LHCb experiment at center-of-mass energies of root s = 7, 8, and 13 TeV, the observation of an excited B-c(+) state in the B-c(+)pi(+)pi(-) invariant-mass spect ...

2019

Stacking transition in rhombohedral graphite

Fabrizio Carbone, Ivan Madan, Gabriele Berruto, Tatiana Latychevskaia

Few-layer graphene (FLG) has recently been intensively investigated for its variable electronic properties, which are defined by a local atomic arrangement. While the most natural arrangement of layers in FLG is ABA (Bernal) stacking, a metastable ABC (rho ...

HIGHER EDUCATION PRESS2019

Dynamics of the MnAs alpha/beta-Striped Microstructure and of the Fe Magnetization Reversal in Fe/MnAs/GaAs(001): An Optical-Laser Pump-Free-Electron-Laser Probe Scattering Experiment

Eugenio Ferrari

It was shown recently that the Fe magnetization reversal in the Fe/MnAs/GaAs(001) epitaxial system, attained by temperature control of the regular stripe pattern of the MnAs alpha- and beta-phases, can also be driven by an ultrashort optical laser pulse. I ...

Mdpi Ag2017