Ultrabroadband tunable difference frequency generation in a standardized thin-film lithium niobate platform

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We obtained gas-phase UV and IR spectra of 1:2 potassium ion-crown ether (CE) complexes (benzo-15-crown-5 (B15C5), benzo-18-crown-6 (B18C6), dibenzo-18-crown-6 (DB18C6), and 18-crown-6 (18C6)) at approximately 10 K and determined the structure and intermol ...

One route to the control of quantum magnetism at ultrafast timescales is magnetophononics, the modulation of magnetic interactions by coherently driven lattice excitations. Theoretical studies of a gapped quantum magnet subject to continuous, single-freque ...

Controlling the light emitted by individual molecules is instrumental to a number of advanced nanotechnologies ranging from super-resolution bioimaging and molecular sensing to quantum nanophotonics. Molecular emission can be tailored by modifying the loca ...

Probing and manipulating the spatiotemporal dynamics of hot carriers in nanoscale metals is crucial to a plethora of applications ranging from nonlinear nanophotonics to single-molecule photochemistry. The direct investigation of these highly non-equilibri ...

The invention of the laser in the 1960s heralded a new era in photonics. Owing to both, academic and industrial research, photonics technologies have long become part of our everyday life. This PhD thesis explores two subfields of laser technologies: Frequ ...

We report the first, to our knowledge, observation of the nonlinear phenomenon known as modulation instability (MI) in a coherently driven fiber resonator pumped at 1972 nm. To compensate for the very high losses in this spectral region, we have integrated ...

On-chip coherent light generation has wide-ranging applications in metrology, spectroscopy, quantum optics, etc. In this study, we demonstrate the generation of coherent light from a silicon-nitride microring resonator using cascaded nonlinear processes. T ...

Frequency up-conversion has become amongst the most prevalent techniques for detection of terahertz waves in metrology systems. State-of-the-art up-conversion techniques rely on the coherent transferring of the information encoded in all degrees of freedom ...

When a nanoparticle (NP) is introduced into a biological environment, its identity and interactions are immediately attributed to the dense layer of proteins that quickly covers the particle. The formation of this layer, dubbed the protein corona, is in ge ...

Near-infrared (NIR) fluorescence lifetime imaging (FLI) provides a unique contrast mechanism to monitor biological parameters and molecular events in vivo. Single-photon avalanche diode (SPAD) cameras have been recently demonstrated in FLI microscopy (FLIM ...

Layered materials (LMs), such as graphite, hexagonal boron nitride, and transition-metal dichalcogenides, are at the center of an ever-increasing research effort, due to their scientific and technological relevance. Raman and infrared spectroscopies are ac ...

Difference-frequency generation (DFG) is elemental for nonlinear parametric processes such as optical parametric oscillation and is instrumental for generating coherent light at long wavelengths, especially in the middle infrared. Second-order nonlinear fr ...

Low-loss nanostructured dielectric metasurfaces have emerged as a breakthrough platform for ultrathin optics and cutting-edge photonic applications, including beam shaping, focusing, and holography. However, the static nature of their constituent materials ...

The growing interest in near-infrared (NIR) imaging is explained by the increasing number of applications in this spectral range, which includes process monitoring and medical imaging. NIR-to-visible optical upconverters made by integrating a NIR photosens ...

Infrared spectroscopy resolves the structure of molecules by detecting their characteristic vibrational fingerprints. Subwavelength light confinement and nanophotonic enhancement have extended the scope of this technique for monolayer studies. However, cur ...

Earth-like planets, dark energy and variability of fundamental physical constants can be discovered by observing wavelength shifts in the optical spectra of astronomical objects(1-5). These wavelength shifts are so tiny that exquisitely accurate and precis ...

I present a molecular beam study of methane dissociation on differ-ent surface sites of several platinum single crystal surfaces (Pt(111), Pt(211), Pt(210), Pt(110)-(2x1)). The experiments were performed in a molecular beam/surface-science apparatus that c ...

Ultrabroadband tunable difference frequency generation in a standardized thin-film lithium niobate platform

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Structure and Interactions in 1:2 K+–Crown Ether Complexes via Gas-Phase Cold UV and IR Spectroscopy

Pulsed Magnetophononics in Gapped Quantum Magnets

Giant Purcell Broadening and Lamb Shift for DNA-Assembled Near-Infrared Quantum Emitters

Visualizing hot carrier dynamics by nonlinear optical spectroscopy at the atomic length scale

Thulium-doped fiber cavities for frequency comb generation at 2 micron

Observation of modulation instability in a coherently driven active fiber ring resonator at 2 µm wavelength

UV, visible and near-infrared light generation through cascaded nonlinear processes in silicon-nitride microring resonators pumped at telecom wavelength

Resolving sub-cycle signatures: A perspective on hallmarks of terahertz metrology

Lysozyme Interaction with Phospholipid Nanodroplets Probed by Sum Frequency Scattering Vibrational Spectroscopy

In vitro and in vivo NIR fluorescence lifetime imaging with a time-gated SPAD camera

Shear and Breathing Modes of Layered Materials

Difference-frequency generation in optically poled silicon nitride waveguides

All-Dielectric Programmable Huygens' Metasurfaces

Recent advances with optical upconverters made from all-organic and hybrid materials

Angle-multiplexed all-dielectric metasurfaces for broadband molecular fingerprint retrieval

A microphotonic astrocomb

Bond-selective and surface-site-specific dissociation of methane on platinum