Publications associées à Evidence that Pacific tuna mercury levels are driven by marine methylmercury production and anthropogenic inputs

Near-bed stratification controls bottom hypoxia in ice-covered alpine lakes

Damien Bouffard, Pascal Perolo, Tomy Doda, Nicolas Thomas Georges Escoffier, Janine Rüegg, Hannah Elisa Chmiel, Hugo Nicolás Ulloa Sánchez, Camille Roland Marie Minaudo

In ice-covered lakes, near-bottom oxygen concentration decreases for most of the wintertime, sometimes down to the point that bottom waters become hypoxic. Studies insofar have reached divergent conclusions on whether climate change limits or reinforces th ...

American Society of Limnology and Oceanography2023

Modelling the coupled mercury-halogen-ozone cycle in the central Arctic during spring

Jenny Thomas, Julia Schmale, Ivo Fabio Beck, Hélène Paule Angot

Near-surface mercury and ozone depletion events occur in the lowest part of the atmosphere during Arctic spring. Mercury depletion is the first step in a process that transforms long-lived elemental mercury to more reactive forms within the Arctic that are ...

2023

Consider the Anoxic Microsite: Acknowledging and Appreciating Spatiotemporal Redox Heterogeneity in Soils and Sediments

Vincent Noel, Meret Aeppli

Reduction-oxidation (redox) reactions underlie essentially all biogeochemical cycles. Like most soil properties and processes, redox is spatiotemporally heterogeneous. However, unlike other soil features, redox heterogeneity has yet to be incorporated into ...

AMER CHEMICAL SOC2023

What are the likely changes in mercury concentration in the Arctic atmosphere and ocean under future emissions scenarios?

Hélène Paule Angot

Arctic mercury (Hg) concentrations respond to changes in anthropogenic Hg emissions and environmental change. This manuscript, prepared for the 2021 Arctic Monitoring and Assessment Programme Mercury Assessment, explores the response of Arctic Ocean Hg con ...

2022

Arctic mercury cycling

Hélène Paule Angot

Anthropogenic mercury (Hg) emissions have driven marked increases in Arctic Hg levels, which are now being impacted by regional warming, with uncertain ecological consequences. This Review presents a comprehensive assessment of the present-day total Hg mas ...

2022

Arctic atmospheric mercury: Sources and changes

Hélène Paule Angot

Global anthropogenic and legacy mercury (Hg) emissions are the main sources of Arctic Hg contamination, primarily transported there via the atmosphere. This review summarizes the state of knowledge of the global anthropogenic sources of Hg emissions, and e ...

2022

Mercury isotope evidence for Arctic summertime re-emission of mercury from the cryosphere

Jenny Thomas, Jakob Boyd Pernov

During Arctic springtime, halogen radicals oxidize atmospheric elemental mercury (Hg0), which deposits to the cryosphere. This is followed by a summertime atmospheric Hg0 peak that is thought to resultmostly fromterrestrial Hg inputs to the ArcticOcean, fo ...

Nature Research2022

Atmospheric mercury sources in a coastal-urban environment: a case study in Boston, Massachusetts, USA

Hélène Paule Angot

Mercury (Hg) is an environmental toxicant dangerous to human health and the environment. Its anthropogenic emissions are regulated by global, regional, and local policies. Here, we investigate Hg sources in the coastal city of Boston, the third largest met ...

2021

Towards an improved understanding of biogeochemical processes across surface-groundwater interactions in intermittent rivers and ephemeral streams

Oleksandra Shumilova, Luis Gómez Gener

Surface-groundwater interactions in intermittent rivers and ephemeral streams (IRES), waterways which do not flow year-round, are spatially and temporally dynamic because of alternations between flowing, non-flowing and dry hydrological states. Interaction ...

2021

Model-based data analysis of the effect of winter mixing on primary production in a lake under reoligotrophication

Alfred Johny Wüest, Hugo Nicolás Ulloa Sánchez, Shubham Krishna, Camille Roland Marie Minaudo

Nutrient loading, in combination with climate change are important drivers of primary productivity in lakes. Understanding and forecasting future changes in primary production (PP) in response to local and global forcing are major challenges for developing ...

ELSEVIER2020

The role of Organophosphate Esters Flame Retardants and plasticizers (OPEs) in Phosphorus Cycle in the atmosphere of the Mediterranean Sea

Athanasios Nenes, Kalliopi Violaki, Christos Panagiotopoulos

The atmosphere is considered as an important external nutrient source for the marine environment, especially in remote ocean waters or the oligotrophic Mediterranean Sea. Phosphorus (P) is a critical nutrient affecting primary productivity in large areas o ...

2020

Mechanistic Investigations of Nickamine-catalyzed Hydrosilylation of Alkenes: Nickel Nanoparticles Are the Active Species

Xile Hu, Marten Leendert Ploeger

Hydrosilylation is an important chemical process for the synthesis of organosilanes and for the production of silicone polymers. The wide variety of catalysts developed for this reaction generally follow a Chalk-Harrod, or a sigma-bond metathesis mechanism ...

SWISS CHEMICAL SOC2020

Using small-scale measurements to estimate hypolimnetic oxygen depletion in a deep lake

Alfred Johny Wüest, Damien Bouffard, Robert Vincent Schwefel

Low oxygen concentrations in lakes and reservoirs are an ongoing environmental concern, particularly in light of increasing anthropogenic activity and climate change. Oxygen depletion processes in lakes are still not completely understood and a variety of ...

American Society of Limnology and Oceanography2018

Fast Potentiometric CO2 Sensor for High-Resolution in Situ Measurements in Fresh Water Systems

Bernhard Wehrli, Nadezda Pankratova

We present a new potentiometric sensor principle and a calibration protocol for in situ profiling of dissolved CO2 with high temporal and spatial resolution in fresh water lakes. The sensor system is based on the measurement of EMF between two solid-contac ...

AMER CHEMICAL SOC2018

Oxygen depletion in Lake Geneva

Robert Vincent Schwefel

Low oxygen concentrations remain a global concern for the ecological health of lakes. High nutrient inputs and climate-induced changes in stratification and mixing are anthropogenic threats which largely impact aquatic oxygen budgets and overall ecosystem ...

EPFL2017

Oxygen depletion in stratified lakes - why shallow and deep lakes react differently

Alfred Johny Wüest, Robert Vincent Schwefel

Oxygen is the most important element in natural waters for any higher aquatic life, such as fish. As with humans, almost all members of aquatic ecosystems need oxygen to breathe. Building on this, treatment of drinking water is easier for oxic than for ano ...

2016

Effects of climate change on deep-water oxygen and winter mixing in a deep lake (Lake Geneva)

Alfred Johny Wüest, Damien Bouffard, Robert Vincent Schwefel

Oxygen is the most important dissolved gas for lake ecosystems. Because low oxygen concentrations are an ongoing problem in many parts of the oceans and numerous lakes, oxygen depletion processes have been intensively studied over the last decades and were ...

2016

Equation of state of liquid mercury to 520 K and 7 GPa from acoustic velocity measurements

Livia Eleonora Bove Kado

Ultrafast acoustics measurements on liquid mercury have been performed at high pressure and temperature in a diamond anvil cell using picosecond acoustic interferometry. We extract the density of mercury from adiabatic sound velocities using a numerical it ...

American Institute of Physics2014

Factors affecting the development and dynamics of hypoxia in a large shallow stratified lake: Hourly to seasonal patterns

Damien Bouffard

[1] The examination of hypoxia in the hypolimnion of large lakes traditionally focuses on the assessment of its spatial and temporal extent and its effect on water quality. In Lake Erie, hypoxia typically occurs between July and October in the central basi ...

American Geophysical Union2013

Hypolimnetic Oxygen Depletion in Eutrophic Lakes

Alfred Johny Wüest, Beat Mueller

The oxygen-consuming processes in the hypolimnia of freshwater lakes leading to deep-water anoxia are still not well understood, thereby constraining suitable management concepts. This study presents data obtained from 11 eutrophic lakes and suggests a mod ...

Amer Chemical Soc2012