The 2022 solar fuels roadmap

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The 2D/3D or 2D/quasi-2D composite mixed-dimensional construction of hybrid perovskite interfaces is gaining increasing attention due to their enhanced stability toward degradation without compromising the corresponding solar cell efficiency. Much of this ...

The rapid crystallization of mixed tin‐lead (Sn‐Pb) perovskites and their dependence on antisolvent processes limit the development of large‐area Sn‐Pb perovskite solar cells (PSCs). Vacuum‐flash‐assisted solution processing (VASP) has emerged as a promisi ...

Mixed Sn-Pb perovskites are attracting significant attention due to their narrow bandgap and consequent potential for all-perovskite tandem solar cells. However, the conventional hole transport materials can lead to band misalignment or induce degradation ...

The stabilization of grain boundaries and surfaces of the perovskite layer is critical to extend the durability of perovskite solar cells. Here we introduced a sulfonium-based molecule, dimethylphenethylsulfonium iodide (DMPESI), for the post-deposition tr ...

The global energy system transforming from fossil fuels to renewable green energy through the adaption of innovative and dynamic green technologies. Energy-saving buildings (ESBs) are attracting extensive attention as intelligent architectures capable of s ...

With the advent of ChatGPT, natural language processing (NLP) models have gained tremendous interest from the research community and have been applied to a plethora of scientific domains like batteries, pharmaceuticals, recycling plastics, etc., to obtain ...

Catalysts play a major role in chemical synthesis, and catalysis is considered to be a green and economic process. Catalysis is dominated by covalent interactions between the catalyst and substrate. The design of non-covalent catalysts came into limelight ...

High-entropy alloys (HEAs), containing several metallic elements in near-equimolar proportions, have long been of interest for their unique mechanical properties. More recently, they have emerged as a promising platform for the development of novel heterog ...

Highlights Integration of decentralized models with a centralized national energy system framework. Strategic reduction in photovoltaic (PV) installation requirements and system cost through decentralized approaches. Optimization of self-consumption to min ...

Spatially resolved photoluminescence (PL) and electroluminescence (EL) imaging technologies play a crucial role in evaluating the performance and stability of photovoltaic devices. However, their application in perovskite devices presents unique challenges ...

The methanol-to-olefins (MTO) process on zeolite-based catalysts enables the production of olefins from green methanol. Selectivity control requires an understanding of the nature and evolution of hydrocarbon species that act as catalytically active center ...

Utilization of small molecules as passivation materials for perovskite solar cells (PSCs) has gained significant attention recently, with hundreds of small molecules demonstrating passivation effects. In this study, a high-accuracy machine learning model i ...

Organic/inorganic metal halide perovskites attract substantial attention as key materials for next-generation photovoltaic technologies due to their potential for low cost, high performance, and solution processability. The unique properties of perovskites ...

In this work, an inexpensive and reliable microstructured electrode for the hydrogen evolution reaction (HER) is developed. This cathode is made of Earth-abundant elements consisting of iron phosphide as an electrocatalyst and carbon felt (CF) as a flexibl ...

Supported Co-based catalysts exhibit promising catalytic activities in the oxygen evolution reaction (OER) during alkaline water electrolysis. Surface functionalization of the support modulates the dispersion of the catalysts and their interaction with the ...

Tandem solar cells are a key technology for exceeding the theoretical efficiency limit of single-junction cells. One of the most promising combinations is the silicon-perovskite tandem cells, considering their potential for high efficiency, fabrication on ...

In this study, a series of donor-acceptor-donor (D-A-D) type small molecules based on the fluorene and diphenylethenyl enamine units, which are distinguished by different acceptors, as holetransporting materials (HTMs) for perovskite solar cells is present ...

Organic-inorganic hybrid perovskites exhibit outstanding performances in perovskite solar cells (PSCs). However, the complex solution chemistry of perovskites precursors renders it difficult to prepare large-area devices in a reproducible way, which is a p ...

The 2022 solar fuels roadmap

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Tuning Electronic and Optical Properties of 2D/3D Interfaces of Hybrid Perovskites through Interfacial Charge Transfer: Prediction of Higher-Efficiency Interface Solar Cells Using Hybrid-DFT Methods

High‐Efficiency Sn‐Pb Perovskite Solar Cells via Nucleation and Crystallization Control

Buried Hole-selective Interface Engineering for High-efficiency Tin-lead Perovskite Solar Cells with Enhanced Interfacial Chemical Stability

Multifunctional sulfonium-based treatment for perovskite solar cells with less than 1% efficiency loss over 4,500-h operational stability tests

Smart Photovoltaic Windows for Next-Generation Energy-Saving Buildings

The predictive power of NLP models on Perovskite solar cells: BERTforPSC

Chalcogen bonding catalysis

Surface segregation in high-entropy alloys from alchemical machine learning

Power to the People: On the Role of Districts in Decentralized Energy Systems

Anomalous Electroluminescence Characteristics of Perovskite Modules

Correlating the Nature of Carbenium Ions in Zeolites to the Product Distribution in the Methanol-to-Olefins Process

Machine Learning for Screening Small Molecules as Passivation Materials for Enhanced Perovskite Solar Cells

Next-generation applications for integrated perovskite solar cells

Flexible and Binder-Free Iron Phosphide Electrodes Using a Three-Dimensional Support for High Hydrogen Productivity

Understanding the role of surface oxygen-containing functional groups on carbon-supported cobalt catalysts for the oxygen evolution reaction

Passivating contact-based tunnel junction Si solar cells using machine learning for tandem cell applications

Passivating Defects of Perovskite Solar Cells with Functional Donor-Acceptor-Donor Type Hole Transporting Materials

Combined Vacuum Evaporation and Solution Process for High-Efficiency Large-Area Perovskite Solar Cells with Exceptional Reproducibility