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Proton-transfer-induced 3D/2D hybrid perovskites suppress ion migration and reduce luminance overshoot

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Publications associées (51)

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Multifunctional sulfonium-based treatment for perovskite solar cells with less than 1% efficiency loss over 4,500-h operational stability tests

Ulf Anders Hagfeldt, Bowen Yang, Jiajia Suo, Yeonju Kim

The stabilization of grain boundaries and surfaces of the perovskite layer is critical to extend the durability of perovskite solar cells. Here we introduced a sulfonium-based molecule, dimethylphenethylsulfonium iodide (DMPESI), for the post-deposition tr ...

Nature Portfolio2024

Strain relaxation and multidentate anchoring in n-type perovskite transistors and logic circuits

Mohammad Khaja Nazeeruddin, Olga Syzgantseva

The engineering of tin halide perovskites has led to the development of p-type transistors with field-effect mobilities of over 70 cm2 V-1 s-1. However, due to their background hole doping, these perovskites are not suitable for n-type transistors. Ambipol ...

Nature Portfolio2024

All-SnO2-Based Conformal Electron Transport Layer for Efficient Perovskite Solar Cells

Likai Zheng

The fabrication of high-performance perovskite solar cells on high-haze fluorine-doped tin oxide (FTO) substrates with superior light-trapping capabilities necessitates a highly conformal electron transport layer at the bottom interface. Herein, a conforma ...

2024

Investigating Non-equilibrium Physics in Wide Bandgap Semiconductors and Quantum Materials via Ultrafast Spectroscopy

Hui-Yuan Chen

This thesis uses femtosecond laser spectroscopy in studying strong correlation in condensed matters that are pertinent to future technology: a wide bandgap perovskite and a quantum material, with the employment of ultrafast time-resolved spectroscopy in th ...

EPFL2024

Best practices in measuring absorption at the macro- and microscale

Giulia Tagliabue, Alan Richard Bowman, Fateme Kiani Shahvandi, Jiaming Ma, German Garcia Martinez

The fraction of light absorbed in a material is a key parameter for a wide range of optoelectronic and energy devices, including solar cells, light emitting diodes, and photo(electro)chemical devices. It can reveal detailed performance information and esta ...

2024

Alleviating nanostructural phase impurities enhances the optoelectronic properties, device performance and stability of cesium-formamidinium metal-halide perovskites

Anaël Morgane Jaffrès, Christophe Ballif, Quentin Thomas Jeangros, Aïcha Hessler-Wyser, Christian Michael Wolff, Mostafa Rabie Shlaly Bahr Othman, Daniel Anthony Jacobs, Austin George Kuba

The technique of alloying FA+ with Cs+ is often used to promote structural stabilization of the desirable alpha-FAPbI3 phase in halide perovskite devices. However, the precise mechanisms by which these alloying approaches improve the optoelectronic quality ...

Royal Soc Chemistry2024

The predictive power of NLP models on Perovskite solar cells: BERTforPSC

Mohammad Khaja Nazeeruddin, François Maréchal, Naveen Bhati

With the advent of ChatGPT, natural language processing (NLP) models have gained tremendous interest from the research community and have been applied to a plethora of scientific domains like batteries, pharmaceuticals, recycling plastics, etc., to obtain ...

Elsevier2024

Machine Learning for Screening Small Molecules as Passivation Materials for Enhanced Perovskite Solar Cells

Mohammad Khaja Nazeeruddin, Bin Ding, Xianfu Zhang

Utilization of small molecules as passivation materials for perovskite solar cells (PSCs) has gained significant attention recently, with hundreds of small molecules demonstrating passivation effects. In this study, a high-accuracy machine learning model i ...

Wiley-VCH Verlag Gmbh2024

Perovskite Solar Cells: Challenges Facing Polymeric Hole Selective Materials in p-i-n Configuration

Mohammad Khaja Nazeeruddin

Polymeric hole-selective materials (P-HSMs) offer advantages like solution processability, tunable energy levels, and improved mechanical stability, making them suitable for large-scale and flexible substrates. Poly[bis(4-phenyl) (2,4,6-trimethylphenyl) am ...

WILEY-V C H VERLAG GMBH2024

Stable cones in the thin one-phase problem

Xavier Fernandez-Real Girona

The aim of this work is to study homogeneous stable solutions to the thin (or fractional) one -phase free boundary problem. The problem of classifying stable (or minimal) homogeneous solutions in dimensions n >= 3 is completely open. In this context, axial ...

Johns Hopkins Univ Press2024

Anomalous Electroluminescence Characteristics of Perovskite Modules

Mohammad Khaja Nazeeruddin, Paul Joseph Dyson

Spatially resolved photoluminescence (PL) and electroluminescence (EL) imaging technologies play a crucial role in evaluating the performance and stability of photovoltaic devices. However, their application in perovskite devices presents unique challenges ...

2024

Font Side Solutions for c-Si Solar Cells with High-Temperature Passivating Contacts

Ezgi Genç

In this work, we studied the potential of using thin films deposited by plasma-enhanced chemical vapor deposition (PECVD) for two main purposes: introducing an n-type passivating contact at the front of a TOPCon solar cell, or simplifying the fabrication o ...

EPFL2024

Quasi-Planar Core Based Spiro-Type Hole-Transporting Material for Dopant-Free Perovskite Solar Cells

Mohammad Khaja Nazeeruddin, Jianxing Xia

Hole-transporting material (HTMs) are crucial for obtaining the stability and high efficiency of perovskite solar cells (PSCs). However, the current state-of-the-art n-i-p PSCs relied on the use of 2,2′,7,7′-tetrakis(N,N-di-p-methoxyphenylamine)-9,9′-spiro ...

Wiley-VCH Verlag GmbH2024

3D diffractive optics for linear interconnects and nonlinear processing

Niyazi Ulas Dinç

The optical domain presents potential avenues for enhancing both computing and communication due to its inherent properties of bandwidth, parallelism, and energy efficiency. This research focuses on harnessing 3-Dimensional (3D) diffractive optics for nove ...

EPFL2024

Smart Photovoltaic Windows for Next-Generation Energy-Saving Buildings

Mohammad Khaja Nazeeruddin

The global energy system transforming from fossil fuels to renewable green energy through the adaption of innovative and dynamic green technologies. Energy-saving buildings (ESBs) are attracting extensive attention as intelligent architectures capable of s ...

WILEY2024

Shortwave Infrared-Sensitive, Narrowband Organic Upconversion Devices with a Gain

Wei-Hsu Hu

Sensing and imaging of light in the shortwave infrared (SWIR) range is increasingly used in various fields, including bio-imaging, remote sensing, and semiconductor process control. SWIR-sensitive organic photodetectors (OPDs) are promising because organic ...

EPFL2024

Methylammonium Nitrate-Mediated Crystal Growth and Defect Passivation in Lead Halide Perovskite Solar Cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Kevin Sivula, Jun Ho Yum, Yeonju Kim

Additive engineering has been a crucial strategy to improve photovoltaic properties by reducing carrier trap centers or increasing carrier diffusion lengths in the lead halide perovskite active layer. We introduced a small amount of CH3NH3 +NO3 - (methylam ...

Amer Chemical Soc2024

Fiber-Coupled Absorption-based Quantum Sensing with Nitrogen Vacancy Ensembles in a Suspended Diamond Photonic Cavity

Darin Ali Naushad Merchant, Christophe Marcel Georges Galland, Amirali Arabmoheghi, Claudio Alejandro Jaramillo Concha, Yuchun Zhu

Low photon extraction efficiency limits the optical spin readout fidelity in emerging quantum sensing technologies in diamond. Here, we propose and fabricate integrated diamond nanoprobes based on cavity-enhanced IR absorption of embedded Nitrogen Vacancy ...

IEEE Computer Society2024

Study of growth-induced point defects and their impact on InGaN-based optoelectronic devices

Yao Chen

GaN exhibits a decomposition tendency for temperatures far below its melting point and common growth temperatures used in metal-organic vapour phase epitaxy (MOVPE).This characteristic is known to be a major obstacle for realising GaN bulk substrate. There ...

EPFL2024

Stress tolerance of lightweight glass-free PV modules for vehicle integration

Kléber Nicolet-dit-Félix, Christophe Ballif, Matthieu Despeisse, Aïcha Hessler-Wyser, Jacques Levrat, Antonin Faes, Gianluca Cattaneo, Umang Bhupatrai Desai, Fahradin Mujovi

Electric vehicles (EVs) currently dominate the sales in the automotive market. A big leap in this market can be made by developing a photovoltaic product that can be integrated to an EV, as it can boost the driving range of the EV while reducing the chargi ...

Edp Sciences S A2024