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Felix Thomas Eickemeyer

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Publications associées (57)

Cyclopentadiene-Based Hole-Transport Material for Cost-Reduced Stabilized Perovskite Solar Cells with Power Conversion Efficiencies Over 23%

Michael Graetzel, Shaik Mohammed Zakeeruddin, Thomas Paul Baumeler, Michael Bauer, Yuhang Liu, Felix Thomas Eickemeyer, Hongwei Zhu

Hole transport materials (HTM) are an important component in perovskite solar cells (PSC). Despite a multitude of HTMs developed in recent years, only few of them lead to solar cells with efficiencies over 20%. Therefore, it is still a challenge to develop ...

2021

Benzylammonium‐Mediated Formamidinium Lead Iodide Perovskite Phase Stabilization for Photovoltaics

Michael Graetzel, Shaik Mohammed Zakeeruddin, Ulf Anders Hagfeldt, Dominik Józef Kubicki, David Lyndon Emsley, Zaiwei Wang, Anwar Qasem M Alanazi, Jovana Milic, Dan Ren, Masaud Hassan S Almalki, Aditya Mishra, Felix Thomas Eickemeyer, Hong Zhang

There is an ongoing surge of interest in the use of formamidinium (FA) lead iodide perovskites in photovoltaics due to their exceptional optoelectronic properties. However, thermodynamic instability of the desired cubic perovskite (α-FAPbI3) phase at ambie ...

2021

Flexible perovskite solar cells with simultaneously improved efficiency, operational stability, and mechanical reliability

Michael Graetzel, Shaik Mohammed Zakeeruddin, Yuhang Liu, Felix Thomas Eickemeyer, Chen Jiang, Min Chen

Although great progress is being made toward improving the power conversion efficiency (PCE) and the operational stability of perovskite solar cells (PSCs), little attention is being paid to their mechanical reliability, which is particularly important for ...

CELL PRESS2021

Multimodal host–guest complexation for efficient and stable perovskite photovoltaics

Michael Graetzel, Shaik Mohammed Zakeeruddin, Ursula Röthlisberger, Ulf Anders Hagfeldt, Marko Mladenovic, David Lyndon Emsley, Farzaneh Jahanbakhshi, Paramvir Ahlawat, Zaiwei Wang, Jovana Milic, Dan Ren, Aditya Mishra, Felix Thomas Eickemeyer, Hong Zhang, Zhaowen Dong, Jinming Guo, Michael Allan Hope, Anurag Krishna, Olivier Ouellette, Tzu-Sen Su, Zhiwen Zhou

Formamidinium lead iodide perovskites are promising light-harvesting materials, yet stabilizing them under operating conditions without compromising optimal optoelectronic properties remains challenging. We report a multimodal host–guest complexation strat ...

Nature Research2021

Formation of High-Performance Multi-Cation Halide Perovskites Photovoltaics by delta-CsPbI3/delta-RbPbI3 Seed-Assisted Heterogeneous Nucleation

Michael Graetzel, Shaik Mohammed Zakeeruddin, Mounir Driss Mensi, Ulf Anders Hagfeldt, Thomas Paul Baumeler, Linfeng Pan, Essa Awadh R Alharbi, Zaiwei Wang, Masaud Hassan S Almalki, Bowen Yang, Felix Thomas Eickemeyer, Anurag Krishna, Olivier Ouellette

The performance of perovskite solar cells is highly dependent on the fabrication method; thus, controlling the growth mechanism of perovskite crystals is a promising way towards increasing their efficiency and stability. Herein, a multi-cation halide compo ...

2021

Synergistic Effect of Fluorinated Passivator and Hole Transport Dopant Enables Stable Perovskite Solar Cells with an Efficiency Near 24%

Michael Graetzel, Shaik Mohammed Zakeeruddin, Ulf Anders Hagfeldt, Linfeng Pan, Yuhang Liu, Felix Thomas Eickemeyer, Yameng Ren, Hongwei Zhu, Olivier Ouellette

Long-term durability is critically important for the commercialization of perovskite solar cells (PSCs). The ionic character of the perovskite and the hydrophilicity of commonly used additives for the hole-transporting layer (HTL), such as lithium bis(trif ...

2021

Ti-1-graphene single-atom material for improved energy level alignment in perovskite solar cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Zaiwei Wang, Felix Thomas Eickemeyer, Hongwei Zhu

Carbon-based perovskite solar cells (C-PSCs) are widely accepted as stable, cost-effective photovoltaics. However, C-PSCs have been suffering from relatively low power conversion efficiencies (PCEs) due to severe electrode-related energy loss. Herein, we r ...

2021

A molecular photosensitizer achieves a Voc of 1.24 V enabling highly efficient and stable dye-sensitized solar cells with copper(II/I)-based electrolyte

Michael Graetzel, Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Nikolaos Vlachopoulos, Ulf Anders Hagfeldt, Yiming Cao, Marko Stojanovic, Etienne Christophe Socie, Felix Thomas Eickemeyer, Yameng Ren, Dan Zhang

To develop photosensitizers with high open-circuit photovoltage (Voc) is a crucial strategy to enhance the power conversion efficiency (PCE) of co-sensitized solar cells. Here, we show a judiciously tailored organic photosensitizer, coded MS5, featuring th ...

Nature Research2021

Carbazol-phenyl-phenothiazine-based sensitizers for dye-sensitized solar cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Yi Ding, Wei Huang, Dan Ren, Felix Thomas Eickemeyer, Zhongjin Shen, Yunfei Jiao, Lukas Pfeifer

Heteroaromatic units are commonly used as pi-spacers for sensitizers in dye-sensitized solar cells (DSSCs). Here, we investigated the influence of the pi-spacer on the photophysical properties, electrochemical properties and photovoltaic performance of car ...

Royal Society of Chemistry2021

Low-Cost Dopant Additive-Free Hole-Transporting Material for a Robust Perovskite Solar Cell with Efficiency Exceeding 21%

Michael Graetzel, Shaik Mohammed Zakeeruddin, Ulf Anders Hagfeldt, Linfeng Pan, Yuhang Liu, Felix Thomas Eickemeyer, Yameng Ren, Hongwei Zhu, Zhongjin Shen

Developing hole-transporting materials (HTMs) with appropriate molecular configuration and charge mobility is important to improve perovskite solar cell (PSC) photovoltaic performance and their feasibility for commercialization. In this work, a novel pyram ...

2021

Vapor-assisted deposition of highly efficient, stable black-phase FAPbI(3) perovskite solar cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Ursula Röthlisberger, Ulf Anders Hagfeldt, Xiong Li, Wolfgang Richard Tress, David Lyndon Emsley, Paramvir Ahlawat, Claudia Esther Avalos, Zaiwei Wang, Yuhang Liu, Anand Agarwalla, Brian Irving Carlsen, Fan Fu, Aditya Mishra, Haizhou Lu, Felix Thomas Eickemeyer, Xianfu Zhang, Likai Zheng, Ying Yang

Mixtures of cations or halides with FAPbI(3) (where FA is formamidinium) lead to high efficiency in perovskite solar cells (PSCs) but also to blue-shifted absorption and long-term stability issues caused by loss of volatile methylammonium (MA) and phase se ...

American Association for the Advancement of Science2020

Zinc Phthalocyanine Conjugated Dimers as Efficient Dopant-Free Hole Transporting Materials in Perovskite Solar Cells

Ulf Anders Hagfeldt, Kazuteru Nonomura, Natalie Flores Diaz, Brian Irving Carlsen, Marco Alejandro Ruiz Preciado, Desiré Molina Alcaide, Bowen Yang, Felix Thomas Eickemeyer

Four ZnPc-dimers with 2,5-thienyl (ZnPc-th-ZnPc 1), 2,7-fluorenyl (ZnPc-flu-ZnPc 2), 3,6-bisthienylldiketopyrrolopyrrole (ZnPc-DPP-ZnPc 3) and 1,4-phenyl (ZnPc-p-ZnPc 4) bridges have been studied as dopant-free hole transporting materials (HTMs) in perovsk ...

WILEY-V C H VERLAG GMBH2020

Crown Ether Modulation Enables over 23% Efficient Formamidinium-Based Perovskite Solar Cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Mounir Driss Mensi, Ursula Röthlisberger, Ulf Anders Hagfeldt, Jun Ho Yum, Kevin Sivula, Marko Mladenovic, David Lyndon Emsley, Farzaneh Jahanbakhshi, Jovana Milic, Dan Ren, Aditya Mishra, Felix Thomas Eickemeyer, Hong Zhang, Michael Allan Hope, Jun Li, Anurag Krishna, Olivier Ouellette, Zhiwen Zhou

The use of molecular modulators to reduce the defect density at the surface and grain boundaries of perovskite materials has been demonstrated to be an effective approach to enhance the photovoltaic performance and device stability of perovskite solar cell ...

2020

High-Performance Lead-Free Solar Cells Based on Tin-Halide Perovskite Thin Films Functionalized by a Divalent Organic

Michael Graetzel, Shaik Mohammed Zakeeruddin, Yuhang Liu, Felix Thomas Eickemeyer, Min Chen

Tin-based halide perovskite solar cells (PSCs) hold the most promise among lead-free PSCs, but they are plagued with inadequate environmental stability and power-conversion efficiency (PCE). Here we demonstrate that the optimum incorporation of a bulky div ...

2020

Stabilization of Highly Efficient and Stable Phase-Pure FAPbI(3)Perovskite Solar Cells by Molecularly Tailored 2D-Overlayers

Michael Graetzel, Shaik Mohammed Zakeeruddin, Ulf Anders Hagfeldt, Mohammad Ibrahim Dar, Jiyoun Seo, Yuhang Liu, Seckin Akin, Jiahuan Zhang, Felix Thomas Eickemeyer, Hong Zhang, Hongwei Zhu

As a result of their attractive optoelectronic properties, metal halide APbI(3)perovskites employing formamidinium (FA(+)) as the A cation are the focus of research. The superior chemical and thermal stability of FA(+)cations makes alpha-FAPbI(3)more suita ...

Wiley-VCH Verlag GmbH2020

Tailored Amphiphilic Molecular Mitigators for Stable Perovskite Solar Cells with 23.5% Efficiency

Shaik Mohammed Zakeeruddin, Ulf Anders Hagfeldt, Mohammad Ibrahim Dar, Xiong Li, Xiaofei Dong, Linfeng Pan, Zaiwei Wang, Yuhang Liu, Brian Irving Carlsen, Dan Ren, Marco Alejandro Ruiz Preciado, Bowen Yang, Felix Thomas Eickemeyer, Hongwei Zhu, Shilong Wang

Passivation of interfacial defects serves as an effective means to realize highly efficient and stable perovskite solar cells (PSCs). However, most molecular modulators currently used to mitigate such defects form poorly conductive aggregates at the perovs ...

Wiley2020

An Improved Perylene Sensitizer for Solar Cell Applications

Michael Graetzel, Mohammad Khaja Nazeeruddin, Jun Ho Yum, Soo-Jin Moon, Felix Thomas Eickemeyer

1,6-Dithiophenol-substituted perylene organic sensitizer 1 was synthesized, and its photovoltaic properties in dye-sensitized solar cells were assessed. When anchored onto TiO2 film, the dye exhibits an unprecedented incident monochromatic photon-to-curren ...

2008

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