Publications de Vasiliki Tileli

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Micro- and nanoscale metallic glasses offer exciting opportunities for both fundamental research and applications in healthcare, micro-engineering, optics and electronics. The scientific and technological challenges associated with the fabrication and util ...

Liquid-phase transmission electron microscopy (LPTEM) is an essential tool for studying the dynamics of materials interactions at the nanoscale, in and/or with their operational environment. Microfabricated SiNx membrane cells further allow the integration ...

Ni-rich layered oxides are promising positive electrodes for fulfillment of government and industry targets for lithium-ion-battery-operated electric mobility purposes. Apart from ongoing research focusing on their design and material production, advanced ...

A three-dimensional finite element method (FEM) model simulating the electrochemical behaviour of Pt coplanar thin-film electrodes used for liquid cell transmission electron microscopy measurements was developed. The model included reaction kinetics and it ...

Tailoring the surface properties of 2D materials, such as transition metal dichalcogenides (TMDCs), at the nanoscale is becoming essential in the fabrication of various 2D material-based nanoelectronic devices. Due to the chemical inertness of their basal ...

Nanowire-based devices can potentially be of use in a variety of electronic applications, from ultrascaled digital circuits to 5G communication networks. However, the devices are typically restricted to low-power applications due to the relatively low elec ...

Understanding the interaction between water and oxides is critical for many technological applications, including energy storage, surface wetting/self-cleaning, photocatalysis and sensors. Here, we report observations of strong structural oscillations of B ...

In this Account, we describe the challenges and promising applications of transmission electron microscopy (TEM) imaging and spectroscopy at cryogenic temperatures. Our work focuses on two areas of application: the delay of electron-beam-induced degradatio ...

The ability to resolve the dynamic evolution of electrocatalytically induced processes with electrochemical liquid-phase electron microscopy (EM) is limited by the microcell configuration. Herein, a free-standing tri-layer graphene is integrated as a membr ...

Non-noble metal catalysts (NNMCs) are regarded as a promising alternative to the costly Pt-based materials required to catalyze the oxygen reduction reaction (ORR) in proton exchange membrane fuel cell (PEMFC) cathodes. However, the large diversity of NNMC ...

Non-noble metal catalysts (NNMCs) hold the potential to replace the expensive Pt-based materials currently used to speed up the oxygen reduction reaction (ORR) in proton exchange membrane fuel cell (PEMFC) cathodes, but they feature poor durability that in ...

It is of great interest to the energy community to understand how the mechano-physico-chemical phenomena that eventually lead to device degradation are related to the startup, operation, and shutdown phases. For electrocatalytic systems operating in liquid ...

High activity and durability are two key requirements for the successful development of Pt-based ORR catalyst layers for polymer electrolyte fuel cell (PEFC) cathodes. Unsupported Pt-Ni aerogels consisting of an interconnected nanoparticle network have bee ...

The surface wettability of catalysts is typically controlled via surface treatments that promote catalytic performance. Here we report on potential-regulated hydrophobicity/hydrophilicity at cobalt-based oxide interfaces with an alkaline solution. The swit ...

This study explores the intricate chemical processes at the interface between the topological insulator Bi2Se3 and deposited Au. The study mainly focused on room-temperature interactions that can cause the aging of, e.g., gold contacts on electronic device ...

Water management by gas diffusion electrodes is a fundamental aspect of the performance of electrochemical cells. Herein, we introduce the characteristic constrictions size as a descriptor for microporous layers (MPL). This parameter is calculated by volum ...

Strategies for forming liquid dispersions of nanomaterials typically focus on retarding reaggregation, for example via surface modification, as opposed to promoting the thermodynamically driven dissolution common for molecule-sized species. Here we demonst ...

Vasiliki Tileli

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Structured nanoscale metallic glass fibres with extreme aspect ratios

Considerations of Liquid-Phase Transmission Electron Microscopy Applied to Heterogeneous Electrocatalysis

Charge/discharge cycling of Li1+x(Ni0.6Co0.2Mn0.2)1−xO2 primary particles performed in a liquid microcell for transmission electron microscopy studies

Simulating Current Distribution of Oxygen Evolution Reaction in Microcells Using Finite Element Method

Electrochemical Functionalization of Selectively Addressed MoS2 Nanoribbons for Sensor Device Fabrication

Multi-channel nanowire devices for efficient power conversion

Nanoscale structural oscillations in perovskite oxides induced by oxygen evolution

Challenges and Applications to Operando and In Situ TEM Imaging and Spectroscopic Capabilities in a Cryogenic Temperature Range

Graphene Electrode for Studying CO2 Electroreduction Nanocatalysts under Realistic Conditions in Microcells

Catalyst Aggregate Size Effect on the Mass Transport Properties of Non-Noble Metal Catalyst Layers for PEMFC Cathodes

Decoupling the Contributions of Different Instability Mechanisms to the PEMFC Performance Decay of Non-noble Metal O2-Reduction Catalysts

Quasi-operando Transmission Electron Microscopy Diagnostics for Electrocatalytic Processes in Liquids

Up-Scaled Preparation of Pt-Ni Aerogel Catalyst Layers for Polymer Electrolyte Fuel Cell Cathodes

Switchable wetting of oxygen-evolving oxide catalysts

Chemical Interactions at the Interface of Au on Bi2Se3 Topological Insulator

Charge/discharge cycling of Li1+x(Ni0.6Co0.2Mn0.2)(1-x)O-2 primary particles performed in a liquid microcell for transmission electron microscopy studies (vol 2, 034007, 2020)

On the role of pore constrictions in gas diffusion electrodes

Ionic solutions of two-dimensional materials

Local hard and soft pinning of 180° domain walls in BaTiO3 probed by in situ transmission electron microscopy