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Cristina Roldán Carmona

Cette personne a quitté l’EPFL

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Publications associées (42)

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Universal approach toward high-efficiency two-dimensional perovskite solar cells via a vertical-rotation process

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen, Cristina Roldán Carmona, Pascal Alexander Schouwink, Yong Ding, Mo Li

The emerging 2D perovskites exhibit superior stability and similar optoelectronic attributes compared to the 3D analogues, but their strong exciton-binding energy and inferior interlayer charge-transport reduce dramatically the device performance. Herein, ...

2020

One-Year stable perovskite solar cells by 2D/3D interface engineering

Michael Graetzel, Mohammad Khaja Nazeeruddin, Iwan Zimmermann, Giulia Grancini, Cristina Roldán Carmona

Despite the impressive photovoltaic performances with power conversion efficiency beyond 22%, perovskite solar cells are poorly stable under operation, failing by far the market requirements. Various technological approaches have been proposed to overcome ...

Nature Publishing Group2017

Air-Stable n-i-p Planar Perovskite Solar Cells Using Nickel Oxide Nanocrystals as Sole Hole-Transporting Material

Mohammad Khaja Nazeeruddin, Cristina Roldán Carmona

Development of low-cost solution processable inorganic hole-transporting materials (HTM) in n-i-p perovskite solar cells (PSCs) is still a challenge toward stable and cost-effective devices. Here, we report the synthesis, surface functionalization, and app ...

2019

Molecularly Engineered Phthalocyanines as Hole-Transporting Materials in Perovskite Solar Cells Reaching Power Conversion Efficiency of 17.5%

Mohammad Khaja Nazeeruddin, Peng Gao, Giulia Grancini, Kyung Taek Cho, Cristina Roldán Carmona, Paul Gratia, Olga Trukhina

Easily accessible tetra-5-hexylthiophene-, tetra-5-hexyl-2,2'-bisthiophene-substituted zinc phthalocyanines (ZnPcs) and tetra-tert-Bu ZnPc are employed as hole-transporting materials in mixed-ion perovskite [HC(NH2)2]0.85(CH3NH3)0.15Pb(I0.8 ...

2017

D-pi-A-Type Triazatruxene-Based Dopant-Free Hole Transporting Materials for Efficient and Stable Perovskite Solar Cells

Mohammad Khaja Nazeeruddin, Hiroyuki Kanda, Sanghyun Paek, Kasparas Rakstys, Cristina Roldán Carmona, Hobeom Kim, Cansu Igci

Three donor-pi-bridge-acceptor (D-pi-A)-type organic small molecules coded CI-B1, CI-B2, and CI-B3 are designed, synthesized, and used as dopant-free hole transporting materials (HTMs) for perovskite solar cells (PSCs). The strong electron-donating triazat ...

WILEY-V C H VERLAG GMBH2020

Azatruxene-Based, Dumbbell-Shaped, Donor-pi-Bridge-Donor Hole-Transporting Materials for Perovskite Solar Cells

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen, Cristina Roldán Carmona, Inés Garcia Benito, Cansu Igci

Three novel donor-pi-bridge-donor (D-pi-D) hole-transporting materials (HTMs) featuring triazatruxene electron-donating units bridged by different 3,4-ethylenedioxythiophene (EDOT) pi-conjugated linkers have been synthesized, characterized, and implemented ...

2020

Optoelectronic device comprising guanidinium in the organic-inorganic perovskite

Mohammad Khaja Nazeeruddin, Cristina Roldán Carmona

Organic-inorganic lead halide perovskites have shown impressive power conversion efficiency (PCE) in a range of solar cell architectures. Despite the multiple ionic compositions that have been reported so far, the presence of organic constituents is an ess ...

2019

Low-Cost TiS2 as Hole-Transport Material for Perovskite Solar Cells

Mohammad Khaja Nazeeruddin, Giulia Grancini, Yonghui Lee, Cristina Roldán Carmona, Aron Joel Huckaba, Saba Gharibzadeh

2018

Cation optimization for burn-in loss-free perovskite solar devices

Mohammad Khaja Nazeeruddin, Tom Theodorus Antonius Lummen, Sanghyun Paek, Cristina Roldán Carmona, Marius Franckevicius, Olga Syzgantseva

Hybrid lead halide perovskites will potentially lead the future energy scenario if highly efficient cells have long-term stability. Here we combine state-of-the art mixed-cation formulations containing formamidinium (FA) and methylammonium (MA), with optim ...

Royal Society of Chemistry2021

Low-voltage, high-brightness and deep-red light-emitting electrochemical cells (LECs) based on new ruthenium(II) phenanthroimidazole complexes

Mohammad Khaja Nazeeruddin, Cristina Roldán Carmona

Light-Emitting Electrochemical Cells (LECs) with a simple device structure ITO/Ru complex/Ga: In were prepared by using heteroleptic ruthenium(II) complexes containing 2-(2-hydroxyphenyl)-1(4-bromophenyl)-1h-imidazo[4,5-f][1,10] phenanthroline (hpbpip) as ...

Royal Society of Chemistry2016

Pulsed-current versus constant-voltage light-emitting electrochemical cells with trifluoromethyl-substituted cationic iridium(III) complexes

Michael Graetzel, Mohammad Khaja Nazeeruddin, Rosario Scopelliti, Cristina Roldán Carmona

We report on five cationic iridium(III) complexes with cyclometalating 2-(3'-trifluoromethylphenyl)pyridine and a diimine, (C boolean AND N)(2)Ir(N boolean AND N), N boolean AND N = 4,4'-R-2-2,2'-dipyridyl or 4,7-R-2-1,10-phenanthroline (R = H, Me, ...

Royal Society of Chemistry2013

Influence of Charge Transport Layers on Open-Circuit Voltage and Hysteresis in Perovskite Solar Cells

Mohammad Khaja Nazeeruddin, Giulia Grancini, Yonghui Lee, Cristina Roldán Carmona, Saba Gharibzadeh

2018

Molecular Design and Operational Stability: Toward Stable 3D/2D Perovskite Interlayers

Mohammad Khaja Nazeeruddin, Anne-Clémence Corminboeuf, Hiroyuki Kanda, Sanghyun Paek, Pascal Alexander Schouwink, Kyung Taek Cho, Cristina Roldán Carmona, Hobeom Kim, Kun-Han Lin, Marius Franckevicius, Nikita Drigo

Despite organic/inorganic lead halide perovskite solar cells becoming one of the most promising next-generation photovoltaic materials, instability under heat and light soaking remains unsolved. In this work, a highly hydrophobic cation, perfluorobenzylamm ...

2020

Doped but Stable: Spirobisacridine Hole Transporting Materials for Hysteresis-Free and Stable Perovskite Solar Cells

Mohammad Khaja Nazeeruddin, Anne-Clémence Corminboeuf, Sanghyun Paek, Pascal Alexander Schouwink, Cristina Roldán Carmona, Albertus Adrian Sutanto, Hobeom Kim, Kun-Han Lin, Marius Franckevicius, Nikita Drigo

Four spirobisacridine (SBA) hole-transporting materials were synthesized and employed in perovskite solar cells (PSCs). The molecules bear electronically inert alkyl chains of different length and bulkiness, attached to in-plane N atoms of nearly orthogona ...

AMER CHEMICAL SOC2020

Crystal Orientation Drives the Interface Physics at Two/Three-Dimensional Hybrid Perovskites

Mohammad Khaja Nazeeruddin, Jacques-Edouard Moser, Giulia Grancini, Sanghyun Paek, Kyung Taek Cho, Cristina Roldán Carmona, Valentin Ianis Emmanuel Queloz, Marine Eva Fedora Bouduban

Combining halide perovskites with tailored dimensionality into two/three-dimensional (2D/3D) systems has revealed a powerful strategy to boost the performances of perovskite photovoltaics (PVs). Despite recent advances, a clear understanding of the intimat ...

2019

Flexible high efficiency perovskite solar cells

Mohammad Khaja Nazeeruddin, Mohammad Ibrahim Dar, Cristina Roldán Carmona

Flexible perovskite based solar cells with power conversion efficiencies of 7% have been prepared on PET based conductive substrates. Extended bending of the devices does not deteriorate their performance demonstrating their suitability for roll to roll pr ...

Royal Society of Chemistry2014

Co-evaporation as an optimal technique towards compact methylammonium bismuth iodide layers

Mohammad Khaja Nazeeruddin, Hiroyuki Kanda, Mounir Driss Mensi, Cristina Roldán Carmona, Albertus Adrian Sutanto, Maria Cristina Momblona Rincón

the most studied perovskite‑based solar cells reported up to date contain the toxic lead in its composition. photovoltaic research and development towards non‑toxic, lead‑free perovskite solar cells are critical to finding alternatives to reduce human heal ...

Nature Research2020

Benzotrithiophene-Based Hole-Transporting Materials for 18.2% Perovskite Solar Cells

Michael Graetzel, Mohammad Khaja Nazeeruddin, Iwan Zimmermann, Cristina Roldán Carmona, Paul Gratia, Sadig Aghazada, Inés Garcia Benito

New star-shaped benzotrithiophene (BTT)-based hole-transporting materials (HTM) BTT-1, BTT-2 and BTT-3 have been obtained through a facile synthetic route by crosslinking triarylamine-based donor groups with a benzotrithiophene (BTT) core. The BTT HTMs wer ...

Wiley-VCH Verlag GmbH2016

Picosecond Capture of Photoexcited Electrons Improves Photovoltaic Conversion in MAPbI3 :C70 -Doped Planar and Mesoporous Solar Cells

Mohammad Khaja Nazeeruddin, Giulia Grancini, Cristina Roldán Carmona, Grégoire Clément Gschwend, Saba Gharibzadeh

Wiley2018

High efficiency methylammonium lead triiodide perovskite solar cells: the relevance of non-stoichiometric precursors

Michael Graetzel, Mohammad Khaja Nazeeruddin, Peng Gao, Iwan Zimmermann, Giulia Grancini, Cristina Roldán Carmona, Peng Gao, Paul Gratia

Methylammonium lead iodide perovskite solar cells with improved performance and stability have been successfully prepared by using a non-stoichiometric PbI2 : CH3NH3I ratio in the precursor solution, and yield a power conversion efficiency (PCE) of above 1 ...

Royal Soc Chemistry2015