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Dominik Józef Kubicki

Cette personne n’est plus à l’EPFL

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Publications associées (48)

Cd-113 Solid-State NMR at 21.1 T Reveals the Local Structure and Passivation Mechanism of Cadmium in Hybrid and All-Inorganic Halide Perovskites

Dominik Józef Kubicki, David Lyndon Emsley, Albert Hofstetter, Brennan James Walder, Daniel Prochowicz

Cadmium doping has recently emerged as an efficacious strategy for defect suppression and band gap tuning in hybrid as well as all-inorganic halide perovskites. However, the cadmium speciation in these materials is unknown. Here, we use high-field cadmium- ...

2020

Atomistic origins of the limited phase stability of Cs+-rich FAxCs(1-x)PbI3 mixtures

Michael Graetzel, Ursula Röthlisberger, Simone Meloni, Dominik Józef Kubicki, David Lyndon Emsley, Ariadni Boziki, Aditya Mishra

Mixed cation perovskites, [HC(NH2)2]xCs(1-x)PbI3, (FAxCs(1-x)PbI3) with x=0.8 achieve high solar cell power conversion efficiencies (PCEs) while exhibiting long-term stability under ambient conditions. In this work, we perform density functional theory (DF ...

2020

Phase transitions, screening and dielectric response of CsPbBr3

Dominik Józef Kubicki

Cesium-lead-bromide (CsPbBr3) is the simplest all inorganic halide perovskite. It serves as a reference material for understanding the exceptional solar cell properties of the organic-inorganic hybrid halide perovskites and is itself discussed as an altern ...

Royal Society of Chemistry2020

Intermediate Phase Enhances Inorganic Perovskite and Metal Oxide Interface for Efficient Photovoltaics

Michael Graetzel, Ulf Anders Hagfeldt, Dominik Józef Kubicki, Wolfgang Richard Tress, David Lyndon Emsley, Claudia Esther Avalos, Zaiwei Wang, Yuhang Liu, Anand Agarwalla, Brian Irving Carlsen, Wanchun Xiang, Mona Shasti, Jiahuan Zhang, Aditya Mishra, Haizhou Lu, Ziyun Wang

Interfacial modification is crucial to fully develop the potential of semiconductor devices, including the revolutionary halide perovskite-based optoelectronics, such as photovoltaics, light-emitting diodes, and photodetectors. The all-inorganic halide per ...

CELL PRESS2020

Atomic-Level Microstructure of Efficient Formamidinium-Based Perovskite Solar Cells Stabilized by 5-Ammonium Valeric Acid Iodide Revealed by Multinuclear and Two-Dimensional Solid-State NMR

Michael Graetzel, Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Ursula Röthlisberger, Marine Eva Fedora Bouduban, Marko Mladenovic, Fabrizio Giordano, Dominik Józef Kubicki, David Lyndon Emsley, Farzaneh Jahanbakhshi, Essa Awadh R Alharbi, Daniel Prochowicz, Anwar Qasem M Alanazi, Jovana Milic, Dan Ren

Chemical doping of inorganic–organic hybrid perovskites is an effective way of improving the performance and operational stability of perovskite solar cells (PSCs). Here we use 5-ammonium valeric acid iodide (AVAI) to chemically stabilize the structure of ...

2019

Solid-state NMR approaches to lead halide perovskites

Michael Graetzel, Dominik Józef Kubicki, David Lyndon Emsley, Albert Hofstetter, Daniel Prochowicz

AMER CHEMICAL SOC2019

Atomic-level passivation mechanism of ammonium salts enabling highly efficient perovskite solar cells

Michael Graetzel, Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Fabrizio Giordano, Dominik Józef Kubicki, Jingshan Luo, Andrés Burgos Caminal, David Lyndon Emsley, Brennan James Walder, Essa Awadh R Alharbi, Anwar Qasem M Alanazi, Alexander Roland Uhl

The high conversion efficiency has made metal halide perovskite solar cells a real break-through in thin film photovoltaic technology in recent years. Here, we introduce a straight-forward strategy to reduce the level of electronic defects present at the i ...

Nature Research2019

Chromium bioavailability in aquatic systems impacted by tannery wastewaters. Part 1: Understanding chromium accumulation by indigenous chironomids

Dominik Józef Kubicki

The tanning industry uses large quantities of Cr whose contribution to the contaminant burden of aquatic organismsis not yet fully understood. The present study investigated Cr bioaccumulation by indigenous chironomids in a freshwater ecosystem impacted by ...

2019

A Factor Two Improvement in High-Field Dynamic Nuclear Polarization from Gd(III) Complexes by Design

Anne-Sophie Chauvin, Marinella Mazzanti, Dominik Józef Kubicki, David Lyndon Emsley, Gabriele Stevanato, Georges Guévork Jean-Jacques Menzildjian

Gadolinium(III) complexes have recently been demonstrated to have potential as polarizing agents for high-field dynamic nuclear polarization (DNP) NMR spectroscopy. By tailoring the ligand design to reduce the zero-field splitting (ZFS), we demonstrate a q ...

2019

Nucleobase pairing and photodimerization in a biologically derived metal-organic framework nanoreactor

Berend Smit, Dominik Józef Kubicki, David Lyndon Emsley, Samantha Lynn Anderson, Kyriakos Stylianou, Peter George Boyd, Andrzej Gladysiak, Ngoc Tú Nguyên

Biologically derived metal-organic frameworks (bio-MOFs) are of great importance as they can be used as models for bio-mimicking and in catalysis, allowing us to gain insights into how large biological molecules function. Through rational design, here we r ...

Nature Research2019

Doping and phase segregation in Mn2+- and Co2+-doped lead halide perovskites from Cs-133 and H-1 NMR relaxation enhancement

Michael Graetzel, Shaik Mohammed Zakeeruddin, Dominik Józef Kubicki, Arthur César Pinon, David Lyndon Emsley, Albert Hofstetter, Gabriele Stevanato, Daniel Prochowicz

Lead halide perovskites belong to a broad class of compounds with appealing optoelectronic and photovoltaic properties. Doping with transition metal ions such as Mn2+ and Co2+ has recently been reported to substantially enhance luminescence and stability o ...

Royal Society of Chemistry2019

Multifunctional Molecular Modulation for Efficient and Stable Hybrid Perovskite Solar Cells

Michael Graetzel, Dominik Józef Kubicki, David Lyndon Emsley, Jovana Milic

Hybrid organic-inorganic perovskites have become one of the leading thin-film semiconductors for optoelectronics. Their broad application will greatly depend on overcoming the key obstacles associated with poor stability and limited scalability. There has ...

2019

Ba-induced phase segregation and band gap reduction in mixed-halide inorganic perovskite solar cells

Michael Graetzel, Ulf Anders Hagfeldt, Dominik Józef Kubicki, Wolfgang Richard Tress, Jingshan Luo, David Lyndon Emsley, Albert Hofstetter, Xiaoyan Wang, Zaiwei Wang, Wanchun Xiang, Jiahuan Zhang, Xiaoyu Wang

All-inorganic metal halide perovskites are showing promising development towards efficient long-term stable materials and solar cells. Element doping, especially on the lead site, has been proved to be a useful strategy to obtain the desired film quality a ...

Nature Research2019

Engineering of Perovskite Materials Based on Formamidinium and Cesium Hybridization for High-Efficiency Solar Cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Dominik Józef Kubicki, Pankaj Kumar Yadav, Daniel Prochowicz, Anwar Qasem M Alanazi, Mohammad Mahdi Tavakoli, Rashmi Runjhun

Engineering the chemical composition of inorganic-organic hybrid perovskite materials is an effective strategy to boost the performance and operational stability of perovskite solar cells (PSCs). Among the diverse family of ABX(3) perovskites, methylammoni ...

AMER CHEMICAL SOC2019

Supramolecular Engineering for Formamidinium-Based Layered 2D Perovskite Solar Cells: Structural Complexity and Dynamics Revealed by Solid-State NMR Spectroscopy

Michael Graetzel, Shaik Mohammed Zakeeruddin, Amita Ummadisingu, Mohammad Ibrahim Dar, Dominik Józef Kubicki, Jeong-Hyeok Im, David Lyndon Emsley, Jiyoun Seo, Yang Li, Jovana Milic, Yang Li, Marco Alejandro Ruiz Preciado

Perovskite solar cells are one of the most promising photovoltaic technologies, although their molecular level design and stability toward environmental factors remain a challenge. Layered 2D Ruddlesden-Popper perovskite phases feature an organic spacer bi ...

WILEY-V C H VERLAG GMBH2019

F-19 Magic Angle Spinning Dynamic Nuclear Polarization Enhanced NMR Spectroscopy

David Benjamin Roger Antoine Gajan, Dominik Józef Kubicki, David Lyndon Emsley, Jasmine Viger-Gravel, Claudia Esther Avalos, Moreno Lelli

The introduction of high-frequency, high-power microwave sources, tailored biradicals, and low-temperature magic angle spinning (MAS) probes has led to a rapid development of hyperpolarization strategies for solids and frozen solutions, leading to large ga ...

Wiley-VCH Verlag GmbH2019

Europium-Doped CsPbI2Br for Stable and Highly Efficient Inorganic Perovskite Solar Cells

Michael Graetzel, Giovanni Dietler, Ulf Anders Hagfeldt, Dominik Józef Kubicki, Wolfgang Richard Tress, Jingshan Luo, David Lyndon Emsley, Jiangtao Zhou, Daniel Prochowicz, Zaiwei Wang, Wanchun Xiang, Seckin Akin

All-inorganic perovskite films hold promise for improving the stability of perovskite solar cells (PSCs). However, the 3D alpha phase of narrow-bandgap inorganic perovskites is thermodynamically unstable at room temperature, limiting the development of hig ...

CELL PRESS2019

Formation of Stable Mixed Guanidinium–Methylammonium Phases with Exceptionally Long Carrier Lifetimes for High-Efficiency Lead Iodide-Based Perovskite Photovoltaics

Shaik Mohammed Zakeeruddin, Norman Pellet, Dominik Józef Kubicki, David Lyndon Emsley, Dongqin Bi, Albert Hofstetter, Pankaj Kumar Yadav, Daniel Prochowicz

Methylammonium (MA)- and formamidinium (FA)-based organic-inorganic lead halide perovskites provide outstanding performance as photovoltaic materials, due to their versatility of fabrication and their power conversion efficiencies reaching over 22%. The pr ...

2018

Multifunctional molecular modulators for perovskite solar cells with over 20% efficiency and high operational stability

Shaik Mohammed Zakeeruddin, Pierre Mettraux, Norman Pellet, Dominik Józef Kubicki, Xiong Li, Jingshan Luo, David Lyndon Emsley, Dongqin Bi, Jovana Milic

Perovskite solar cells present one of the most prominent photovoltaic technologies, yet their stability, scalability, and engineering at the molecular level remain challenging. We demonstrate a concept of multifunctional molecular modulation of scalable an ...

Nature Research2018

One-step mechanochemical incorporation of an insoluble cesium additive for high performance planar heterojunction solar cells

Shaik Mohammed Zakeeruddin, Dominik Józef Kubicki, David Lyndon Emsley, Michael Saliba, Pankaj Kumar Yadav, Daniel Prochowicz, Mohammad Mahdi Tavakoli

Elsevier2018

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