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Giulia Tagliabue

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Publications associées (41)

Quantum-mechanical effects in photoluminescence from thin crystalline gold films

Giulia Tagliabue, Fateme Kiani Shahvandi, Theodoros Tsoulos, Alan Richard Bowman

Luminescence constitutes a unique source of insight into hot carrier processes in metals, including those in plasmonic nanostructures used for sensing and energy applications. However, being weak in nature, metal luminescence remains poorly understood, its ...

2024

Augmenting intrinsic second-order nonlinear response of monocrystalline gold with plasmon resonances

Olivier Martin, Giulia Tagliabue, Fateme Kiani Shahvandi, Sergejs Boroviks

2023

Transport and Interfacial Injection of d-Band Hot Holes Control Plasmonic Chemistry

Giulia Tagliabue, Fateme Kiani Shahvandi, Omer Can Karaman, Milad Sabzehparvar, Alan Richard Bowman

Harnessing nonequilibrium hot carriers from plasmonic metal nanostructures constitutes a vibrant research field with the potential to control photochemical reactions, particularly for solar fuel generation. However, a comprehensive understanding of the int ...

AMER CHEMICAL SOC2023

Light-Driven Thermo-Optical Effects in Nanoresonator Arrays

Giulia Tagliabue, Alfredo Angelo Luigi Naef, Ershad Mohammadi, Theodoros Tsoulos

Thermonanophotonics, that is the study of photothermal effects in optical nanoantennas, has recently attracted growing interest. In particular, going beyond thermoplasmonic designs, thermo-optical modulation of dielectric nanoantennas opens new opportuniti ...

WILEY-V C H VERLAG GMBH2023

Understanding Wavelength-Dependent Synergies between Morphology and Photonic Design in TiO2-Based Solar Powered Redox Cells

Giulia Tagliabue, Jiaming Ma, Kiseok Oh

Solar powered redox cells (SPRCs) are promising for large-scale and long-term storage of solar-energy, particularly when coupled with redox flow batteries (RFBs). While efforts have primarily focused on heterostructure engineering, the potential of synergi ...

AMER CHEMICAL SOC2023

Plasmonic Nanofluids: Enhancing Photothermal Gradients toward Liquid Robots

Giulia Tagliabue, Matteo Bevione

In situ energy generation in soft, flexible, autonomous devices is challenging due to the need for highly stretchable and fault-resistant components. Nanofluids with pyro-, tribo-, or thermoelectric properties have recently emerged as promising solutions f ...

Amer Chemical Soc2023

Photo-modulated optical and electrical properties of graphene

Giulia Tagliabue, Tarique Anwar, Hongyu Tang

Photo-modulation is a promising strategy for contactless and ultrafast control of optical and electrical properties of photoactive materials. Graphene is an attractive candidate material for photo-modulation due to its extraordinary physical properties and ...

WALTER DE GRUYTER GMBH2022

Plasmon-induced near-infrared fluorescence enhancement of single-walled carbon nanotubes

Giulia Tagliabue, Amirmostafa Amirjani, Ardemis Anoush Boghossian, Sayyed Hashem Sajjadi, Shang-Jung Wu, Alessandra Antonucci, Theodoros Tsoulos

Single-walled carbon nanotubes (SWCNTs) emit near-infrared (NIR) fluorescence that is ideal for optical sensing. However, the low quantum yields diminish the sensor’s signal-to-noise ratio and limits the penetration depths for in vivo measurements. In this ...

2022

Thermally reconfigurable metalens

Giulia Tagliabue, Nathanaël Restori, Anna Archetti, Fateme Kiani Shahvandi, Theodoros Tsoulos, Ren-Jie Lin

Reconfigurable metalenses are compact optical components composed by arrays of meta-atoms that offer unique opportunities for advanced optical systems, from microscopy to augmented reality platforms. Although poorly explored in the context of reconfigurabl ...

WALTER DE GRUYTER GMBH2022

High Aspect Ratio Au Microflakes via Gap-Assisted Synthesis

Giulia Tagliabue, Fateme Kiani Shahvandi

Ultrathin and extra-large single-crystalline Au microflakes (Au MFs) have a huge potential in applications ranging from nanophotonics to catalysis. Yet, wet chemical synthesis approaches cannot access this size range due to the proportionality between grow ...

2022

Thermally reconfigurable varifocal silicon metalens

Giulia Tagliabue, Nathanaël Restori, Anna Archetti, Ren-Jie Lin

Active optical components are essential building blocks for a wide variety of applications such as optical communications, microscopy, and illumination systems. Reconfigurable metasurfaces, which consist of arrays of sub-wavelength meta-atoms, can be engin ...

SPIE-INT SOC OPTICAL ENGINEERING2021

Intrinsic luminescence blinking from plasmonic nanojunctions

Magalí Alejandra Lingenfelder, Christophe Marcel Georges Galland, Tobias Kippenberg, Philippe Andreas Rölli, Giulia Tagliabue, Karla Banjac, Aqeel Ahmed, Wen Chen, Sachin Suresh Verlekar

Plasmonic nanojunctions, consisting of adjacent metal structures with nanometre gaps, can support localised plasmon resonances that boost light matter interactions and concentrate electromagnetic fields at the nanoscale. In this regime, the optical respons ...

Nature Research2021

Self-induced thermo-optical effects in silicon and germanium dielectric nanoresonators

Giulia Tagliabue, Theodoros Tsoulos

Dielectric nanoresona tors uniquely support both magnetic and electric resonances across a wide wavelength range. They are thus being exploited in a growing number of groundbreaking applications. In particular, they have been recently suggested as promisin ...

2020

Hot-Hole versus Hot-Electron Transport at Cu/GaN Heterojunction Interfaces

Giulia Tagliabue

Among all plasmonic metals, copper (Cu) has the greatest potential for realizing optoelectronic and photochemical hot-carrier devices, thanks to its CMOS compatibility and outstanding catalytic properties. Yet, relative to gold (Au) or silver (Ag), Cu has ...

AMER CHEMICAL SOC2020

Challenges in Plasmonic Catalysis

Giulia Tagliabue

The use of nanoplasmonics to control light and heat close to the thermodynamic limit enables exciting opportunities in the field of plasmonic catalysis. The decay of plasmonic excitations creates highly nonequilibriumdistributions of hot carriers that can ...

2020

Ultra-Broadband and Omnidirectional Perfect Absorber Based on Copper Nanowire/Carbon Nanotube Hierarchical Structure

Giulia Tagliabue, Fateme Kiani Shahvandi, Theodoros Tsoulos

Zero reflection and complete light absorption are required in a wide range of applications ranging from sensing devices to solar heaters and photoelectrodes. However, simultaneously satisfying the requirements of the broadband spectrum, omnidirectionality, ...

AMER CHEMICAL SOC2020

Transport of hot carriers in plasmonic nanostructures

Giulia Tagliabue

Plasmonic hot carrier devices extract excited carriers from metal nanostructures before equilibration and have the potential to surpass semiconductor light absorbers. However their efficiencies have so far remained well below theoretical limits, which nece ...

AMER PHYSICAL SOC2019

Quantifying the role of surface plasmon excitation and hot carrier transport in plasmonic devices

Giulia Tagliabue

Harnessing photoexcited “hot” carriers in metallic nanostructures could define a new phase of non-equilibrium optoelectronics for photodetection and photocatalysis. Surface plasmons are considered pivotal for enabling efficient operation of hot carrier dev ...

Nature Research2018

Rapid-Response Low Infrared Emission Broadband Ultrathin Plasmonic Light Absorber

Dimos Poulikakos, Giulia Tagliabue

Plasmonic nanostructures can significantly advance broadband visible-light absorption, with absorber thicknesses in the sub-wavelength regime, much thinner than conventional broadband coatings. Such absorbers have inherently very small heat capacity, hence ...

Nature Publishing Group2014

A micro particle shadow velocimetry (mu PSV) technique to measure flows in microchannels

John Richard Thome, Navid Borhani, Sepideh Khodaparast, Giulia Tagliabue

A micro particle shadow velocimetry (mu PSV) system based on back-lit illumination and forward scatter observation of light from non-fluorescent particles has been developed. Relatively high luminous efficiencies and particle image contrasts were achieved ...

Springer-Verlag2013

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