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The present study measures the sticking probability of heavy water (D2O) on H2O- and on D2O-ice and probes the inﬂuence of selective OD-stretch excitation on D2O sticking on these ices. Molecular beam techniques are combined with infrared laser excitation ...

Newly available, powerful infrared laser sources enable the preparation of intense molecular beams of quantum-state prepared and aligned molecules for gas/surface reaction dynamics experiments. We present a stereodynamics study of the chemisorption of vibr ...

The reactivity of methane (CH4) on Pt(110)-(1×2) has been studied by quantum state-resolved surface reactivity measurements. Ground state reaction probabilities, S0(v=0) ~ S0(laser-off), as well as state-resolved reaction probabilities S0(2v3), for CH4 exc ...

Quantum state-resolved sticking coefficients on Pt(111) and Ni(111) surfaces have been measured for CH4 excited to the first overtone of the antisymmetric C-H stretch (2ν3) at well defined kinetic energies in the range of 10-90 kJ/mol. The ground state rea ...

We present a stereodynamics study of the dissociative chemisorption of vibrationally excited methane on the (100), (110), and (111) planes of a nickel single crystal surface. Using linearly polarized infrared excitation of the antisymmetric C–H stretch nor ...

The state-resolved reaction probability of CH4 on Pt(110)-(1×2) was measured as a function of CH4 translational energy for four vibrational eigenstates comprising different amounts of C-H stretch and bend excitation. State-specific reactivity is observed b ...

We report the design and characterization of a new molecular-beam/surface-science apparatus for quantum state-resolved studies of gas/surface reaction dynamics combining optical state-specific reactant preparation in a molecular beam by rapid adiabatic pas ...

Reflection absorption infrared spectroscopy (RAIRS) was used to probe for vibrational bond-selectivity in the dissociative chemisorption of three partially deuterated methane isotopologues on a Pt(111) surface. While a combination of incident translational ...

The quantum state-resolved reactivity S0 of SiH4 on Si(100)-2x1 has been measured for the first time for two vibrationally excited Si-H stretch local mode states (|2000> and |1100>) as well the ground state S0 as a function of translational energy En and s ...

In their article, Inanaga et al. have presented an angular distribution for the desorption of hydrogen molecules induced by hydrogen atoms impinging on a hydrogenated Si(100) surface and compared the measurement with classical trajectory calculations based ...

Absorption spectra of silane in the region of the first overtone of the Si-H stretch vibration have been recorded in a seeded supersonic jet expansion by cavity ring-down spectroscopy as well as in a static gas cell at room temperature by photoacoustic spe ...

Régis Bisson

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The sticking probability of D2O-water on ice: Isotope effects and the inﬂuence of vibrational excitation

Steric Effects in the Chemisorption of Vibrationally Excited Methane on Ni(100)

State-resolved reactivity of CH4 on Pt(110)-(1 x 2): The role of surface orientation and impact site

State-Resolved Reactivity of CH4(2ν3) on Pt(111) and Ni(111): Effects of Barrier Height and Transition State Location

Alignment dependent chemisorption of vibrationally excited CH4(3) on Ni(100), Ni(110), and Ni(111)

Mode-specific reactivity of CH4 on Pt(110)-(1×2): The concerted role of stretch and bend excitation

Quantum state-resolved gas/surface reaction dynamics probed by reflection absorption infrared spectroscopy

Vibrationally bond-selected chemisorption of methane isotopologues on Pt(111) studied by reflection absorption infrared spectroscopy

Vibrational Activation in Direct and Precursor-Mediated Chemisorption of SiH4 on Si(100)

Comment on « Angular distributions of H-induced HD and D2 desorptions from the Si(100) surfaces » [J. Chem. Phys. 124, 054715 (2006)]

Cavity ring-down spectroscopy of jet-cooled silane isotopologues in the Si-H stretch overtone region