Andreas Tortschanoff

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We report on photoluminescence decay measurements of CdSe nanoparticles over several decades of intensities and times, and as a function of size and temp. A model is proposed for the multi-exponential decay kinetics, and their temp. dependence, in which a ...

Broadband transient absorption (TA) spectroscopy, three-pulse photon echo peak shift (3PEPS), and anisotropy decay measurements were used to study the solvation dynamics in bulk water and interfacial water at ZrO2 surfaces, using Eosin Y as a probe. The 3P ...

In 2-color optical Kerr effect measurements of water, addnl. signals can occur in the pulse overlap region if the energy difference between pump and probe pulses approaches the Raman resonance of the OH-stretch vibration. These features can be understood b ...

The fs-time-resolved study of a small UV dye in different solvents with fluorescence up-conversion and photon-echo techniques in the UV range provides new insight in cooling relaxation and solvation dynamics of non-polar molecules in polar solvents. ...

Time-resolved Optical Kerr Effect (OKE) measurements were used to det. the orientational dynamics of water and acetonitrile in the bulk and in pores of ZrO2 nanostructured films. The expts. were performed with a home-built OKE microscope, capable of provid ...

We compare UV transient grating (TG) experiments of aqueous tryptophan with transient absorption (TA) and fluorescence up-conversion measurements. The TG and TA signals show a bi-exponential rise with sub-ps and ps time constants, which are consistent with ...

The (sub)-ps relaxation processes in PbSe quantum dots of different sizes were measured by near-IR luminescence upconversion. The early-time spectra are characterized by emission from several low-lying excited states. The direct measurement of the Huang-Rh ...

Mol. dynamics simulations at 298 K are used to study an aq. dissolved dye (eosin Y) adsorbed at the TiO2(1 1 0) surface to ext. static and dynamic information of solvation. Differences in the phys. behavior of the dye at the surface and in bulk H2O are com ...

We present a new photon echo set-up operating in the UV range and our 1st results of photon echo peak shift (PEPS) expts. of a small non-polar dye mol., p-terphenyl (pTP), in 3 different solvents: EtOH, MeOH, and 2-propanol. The expts. show the feasibility ...

The authors present photon echo peak shift and femtosecond fluorescence up-conversion studies of nonpolar solvation dynamics of a simple nonpolar dye p-terphenyl in EtOH and cyclohexane, using excitation in the UV range at 290 nm. The UV fluorescence up-co ...

The temp. dependence of the absorption and fluorescence spectra of colloidal CdSe nanocrystals was compared for three different shapes (dots, rods, and tetrapods) at 4-300 K. While the shift of the fluorescence max. indicates little dependence on the shape ...

We present ultrafast pump-probe studies on chem. prepd. CdSe nanocrystals. Upon pulsed optical excitation we find pronounced oscillations, indicating strong coupling to a LO phonon mode. From the polarization dependence of the signal addnl. information abo ...

Time resolved optical Kerr effect measurements have been used to det. the orientational dynamics of water in the pores of ZrO2 nanostructured films. We demonstrate that local heating effects can safely be ignored and present our results which are manifestl ...

We show a femtosecond fluorescence upconversion setup with broadband detection to measure time-resolved emission spectra in the 300-550 nm range, upon excitation between 250 and 300 nm, with a time resolution of 100 fs. We present time-resolved fluorescenc ...

The authors present a detailed study of the nonresonant 3rd-order ultrafast response of TiO2 nanostructured films, combining a classical heterodyned optical Kerr effect expt., with 2 polarization selective Kerr techniques, based on transient lensing and ph ...

Andreas Tortschanoff

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A model for the multi-exponential excited-state decay of CdSe nanocrystals

Aqueous Solvation Dynamics at Metal Oxide Surfaces

Raman-induced signals in optical Kerr effect measurements of water with elliptically polarized pulses

Broadband femtosecond fluorescence up-conversion and photon echo experiments in the UV

Liquid dynamics in ZrO2 nanoporous films

Ultraviolet transient absorption, transient grating and photon echo studies of aqueous tryptophan

Subpicosecond near-infrared fluorescence upconversion study of relaxation processes in PbSe quantum dots

Modelling of aqueous solvation of eosin Y at the rutile TiO2(110)/water interface

Photon echo peak shift experiments in the UV: p-terphenyl in different solvents

Ultrafast UV photon echo peak shift and fluorescence up conversion studies of non-polar solvation dynamics

Temperature effects on the spectral properties of colloidal CdSe nanodots, nanorods, and tetrapods

Femtosecond polarization relaxation in CdSe nanocrystals

Optical Kerr effect studies of the dynamics of confined water

Femtosecond fluorescence upconversion setup with broadband detection in the ultraviolet

Ultrafast nonresonant response of TiO2 nanostructured films