Publications de Frank van Mourik

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In 2-color optical Kerr effect measurements of water, addnl. signals can occur in the pulse overlap region if the energy difference between pump and probe pulses approaches the Raman resonance of the OH-stretch vibration. These features can be understood b ...

We present a simple electron time of flight spectrometer for time resolved photoelectron spectroscopy of liquid samples using a vacuum ultraviolet (VUV) source produced by high-harmonic generation. The field free spectrometer coupled with the time-preservi ...

The authors measured the elec. field induced linear dichroism for a wide range of sizes of CdSe nanocrystals. Large ground-state dipole moments were obsd., esp. for the smallest crystals. In these, the authors found a very large anisotropy of the absorptio ...

It was recently demonstrated that in ferric myoglobins (Mb) the fluorescence quenching of the photoexcited tryptophan 14 (*Trp(14)) residue is in part due to an electron transfer to the heme porphyrin (porph), turning it to the ferrous state. However, the ...

The fs-time-resolved study of a small UV dye in different solvents with fluorescence up-conversion and photon-echo techniques in the UV range provides new insight in cooling relaxation and solvation dynamics of non-polar molecules in polar solvents. ...

Tryptophan is commonly used to study protein structure and dynamics, such as protein folding, as a donor in fluorescence resonant energy transfer (FRET) studies. By using ultra-broadband ultrafast two-dimensional (2D) spectroscopy in the ultraviolet (UV) a ...

Time-resolved Optical Kerr Effect (OKE) measurements were used to det. the orientational dynamics of water and acetonitrile in the bulk and in pores of ZrO2 nanostructured films. The expts. were performed with a home-built OKE microscope, capable of provid ...

Femtosecond photoluminescence (PL) up-conversion studies in polychromatic mode and laser-power-dependence studies of the PL were carried out on colloidal solutions of CdSe quantum dots with diameters ranging from 2.4 to 4 nm. The main features of the spect ...

A tuneable repetition rate extreme ultraviolet source (Harmonium) for time resolved photoelectron spectroscopy of liquids is presented. High harmonic generation produces 30-110 eV photons, with fluxes ranging from similar to 2 x 10(11) photons/s at 36 eV t ...

Symmetry breaking across phase transitions often causes changes in selection rules and emergence of optical modes which can be detected via spectroscopic techniques or generated coherently in pump-probe experiments. In second-order or weakly first-order tr ...

The (sub)-ps relaxation processes in PbSe quantum dots of different sizes were measured by near-IR luminescence upconversion. The early-time spectra are characterized by emission from several low-lying excited states. The direct measurement of the Huang-Rh ...

We developed a fast multichannel detection system for pump-probe spectroscopy, capable of detecting single shot super-continuum spectra at the repetition rate (10-50 kHz) of an amplified femtosecond laser system. By tandem pumping the amplifier with three ...

Mol. dynamics simulations at 298 K are used to study an aq. dissolved dye (eosin Y) adsorbed at the TiO2(1 1 0) surface to ext. static and dynamic information of solvation. Differences in the phys. behavior of the dye at the surface and in bulk H2O are com ...

We review our recent studies of excited state structures and dynamics of chemical and biological systems with pico- and femtosecond X-ray absorption spectroscopy in the liquid phase. ...

We present the extension of time-resolved optical pump/x-ray absorption spectroscopy (XAS) probe experiments towards data collection atMHz repetition rates. The use of a high-power picosecond laser operating at an integer fraction of the repetition rate of ...

We present a new photon echo set-up operating in the UV range and our 1st results of photon echo peak shift (PEPS) expts. of a small non-polar dye mol., p-terphenyl (pTP), in 3 different solvents: EtOH, MeOH, and 2-propanol. The expts. show the feasibility ...

The authors present photon echo peak shift and femtosecond fluorescence up-conversion studies of nonpolar solvation dynamics of a simple nonpolar dye p-terphenyl in EtOH and cyclohexane, using excitation in the UV range at 290 nm. The UV fluorescence up-co ...

The authors studied ultrafast relaxation of localized excited states at Ge-related O deficient centers in SiO2 using femtosecond transient-absorption spectroscopy. The relaxation dynamics exhibits a biexponential decay, which the authors ascribe to the dep ...

The temp. dependence of the absorption and fluorescence spectra of colloidal CdSe nanocrystals was compared for three different shapes (dots, rods, and tetrapods) at 4-300 K. While the shift of the fluorescence max. indicates little dependence on the shape ...

In cuprates, a precursor state of superconductivity is speculated to exist above the critical temperature T-c. Here we show via a combination of far-infrared ellipsometry and ultrafast broadband optical spectroscopy that signatures of such a state can be o ...

Frank van Mourik

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Raman-induced signals in optical Kerr effect measurements of water with elliptically polarized pulses

A simple electron time-of-flight spectrometer for ultrafast vacuum ultraviolet photoelectron spectroscopy of liquid solutions

Linear dichroism of CdSe nanodots: Large anisotropy of the band-gap absorption induced by ground-state dipole moments

Tryptophan-to-heme electron transfer in ferrous myoglobins

Broadband femtosecond fluorescence up-conversion and photon echo experiments in the UV

Ultrafast Tryptophan-to-Heme Electron Transfer in Myoglobins Revealed by UV 2D Spectroscopy

Liquid dynamics in ZrO2 nanoporous films

Spectral and dynamical characterization of multiexcitons in colloidal CdSe semiconductor quantum dots

Harmonium: A pulse preserving source of monochromatic extreme ultraviolet (30–110 eV) radiation for ultrafast photoelectron spectroscopy of liquids

Coherent generation of symmetry-forbidden phonons by light-induced electron-phonon interactions in magnetite

Subpicosecond near-infrared fluorescence upconversion study of relaxation processes in PbSe quantum dots

Femtosecond pump/supercontinuum-probe setup with 20 kHz repetition rate

Modelling of aqueous solvation of eosin Y at the rutile TiO2(110)/water interface

Ultrafast X-ray Absorption Studies of the Structural Dynamics of Molecular and Biological Systems in Solution

A high-repetition rate scheme for synchrotron-based picosecond laser pump/x-ray probe experiments on chemical and biological systems in solution

Photon echo peak shift experiments in the UV: p-terphenyl in different solvents

Ultrafast UV photon echo peak shift and fluorescence up conversion studies of non-polar solvation dynamics

Relaxation processes of point defects in vitreous silica from femtosecond to nanoseconds

Temperature effects on the spectral properties of colloidal CdSe nanodots, nanorods, and tetrapods

Clocking the onset of bilayer coherence in a high-Tc cuprate