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Stefano Rusponi

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Publications associées (60)

Uniaxial 2D Superlattice of Fe-4 Molecular Magnets on Graphene

Harald Brune, Stefano Rusponi, Luca Gragnaniello, Fabian Paschke

We demonstrate that electrospray deposition enables the fabrication of highly periodic self-assembled arrays of Fe4H single molecule magnets on graphene/Ir(111). The energetic positions of molecular states are probed by means of scanning tunneling spectros ...

American Chemical Society2017

Two-Orbital Kondo Screening in a Self-Assembled Metal Organic Complex

Harald Brune, Stefano Rusponi, Oleg Yazyev, Marina Pivetta, Fabio Donati, Luca Gragnaniello, Gabriel Albert Autes, Giulia Elisabetta Pacchioni

Iron atoms adsorbed on a Cu(111) surface and buried under polyphenyl dicarbonitrile molecules exhibit strongly spatial anisotropic Kondo features with directionally dependent Kondo temperatures and line shapes, as evidenced by scanning tunneling spectrosco ...

American Chemical Society2017

4 f occupancy and magnetism of rare-earth atoms adsorbed on metal substrates

Harald Brune, Pietro Gambardella, Stefano Rusponi, Sebastian Stepanow, Fabio Donati, Aparajita Singha, Jan Gui-Hyon Dreiser, Christian Wäckerlin, Romana Baltic

We report x-ray absorption spectroscopy and x-ray magnetic circular dichroism measurements as well as multiplet calculations for Dy, Ho, Er, and Tm atoms adsorbed on Pt(111), Cu(111), Ag(100), and Ag(111). In the gas phase, all four elements are divalent a ...

Amer Physical Soc2017

Complex Magnetic Exchange Coupling between Co Nanostructures and Ni(111) across Epitaxial Graphene

Harald Brune, Pietro Gambardella, François Patthey, Stefano Rusponi, Marina Pivetta, Fabio Donati

We report on the magnetic coupling between isolated Co atoms as well as small Co islands and Ni(111) mediated by an epitaxial graphene layer. X-ray magnetic circular dichroism and scanning tunneling microscopy combined with density functional theory calcul ...

American Chemical Society2016

Giant apparent lattice distortions in STM images of corrugated sp2-hybridised monolayers

Laurent Claude, Harald Brune, Alfredo Pasquarello, François Patthey, Stefano Rusponi, Anne Lehnert, Quentin Dubout, Markus Etzkorn, Donat Fabian Natterer

We report on the strengths and limitations of scanning tunnelling microscopy (STM) when used for characterising atomic-scale features of quasi two-dimensional materials, such as graphene and single layers of hexagonal boron nitride, which may present stron ...

Institute of Physics (IoP) and Deutsche Physikalische Gesellschaft2016

Magnetic Hysteresis in Er Trimers on Cu(111)

Harald Brune, Stefano Rusponi, Marina Pivetta, Fabio Donati, Aparajita Singha, Jan Gui-Hyon Dreiser, Christian Wäckerlin, Romana Baltic

We report magnetic hysteresis in Er clusters on. Cu(111) starting from the size-of three atoms. combining Xray magnetic circular dichroism, scanning tunneling microscopy, and mean-field nucleation theory, we determine the size dependent magnetic properties ...

American Chemical Society2016

Tunable spin polarization and superconductivity in engineered oxide interfaces

Stefano Rusponi

Advances in growth technology of oxide materials allow single atomic layer control of heterostructures. In particular delta doping, a key materials' engineering tool in today's semiconductor technology, is now also available for oxides. Here we show that a ...

Nature Publishing Group2016

Out-of-Plane Alignment of Er(trensal) Easy Magnetization Axes Using Graphene

Harald Brune, Stefano Rusponi, Marina Pivetta, Alberto Cavallin, Fabio Donati, Luca Gragnaniello, Giulia Elisabetta Pacchioni, Jan Gui-Hyon Dreiser

We have studied Er(trensal) single -ion magnets adsorbed on graphene/Ru(0001), on graphene/Ir(111), and on bare Ru(0001) by scanning tunneling microscopy and X-ray absorption spectroscopy. On graphene, the molecules self -assemble into dense and well -orde ...

American Chemical Society2016

Magnetic remanence in single atoms

Harald Brune, Pietro Gambardella, François Patthey, Stefano Rusponi, Zeljko Sljivancanin, Edgar Fernandes, Fabio Donati, Aparajita Singha, Jan Gui-Hyon Dreiser, Christian Wäckerlin, Romana Baltic, Katharina Johanna Diller

A permanent magnet retains a substantial fraction of its saturation magnetization in the absence of an external magnetic field. Realizing magnetic remanence in a single atom allows for storing and processing information in the smallest unit of matter. We s ...

American Association for the Advancement of Science2016

Strong antiferromagnetic exchange between manganese phthalocyanine and ferromagnetic europium oxide

Stefano Rusponi, Fabio Donati, Aparajita Singha, Jan Gui-Hyon Dreiser, Christian Wäckerlin, Romana Baltic

We report on the antiferromagnetic exchange coupling between a submonolayer of Mn(II)-phthalocyanine molecules and a ferromagnetic Eu(II)-oxide thin film. The exchange energy is larger by nearly two orders of magnitude compared to previous studies involvin ...

Royal Society of Chemistry2015

Interfacial properties of LaMnO3/LaNiO3 superlattices grown along (001) and (111) orientations

Harald Brune, Stefano Rusponi, Jan Gui-Hyon Dreiser

We have employed x-ray absorption spectroscopy and x-ray magnetic circular dichroism (XMCD) at the Ni andMn L-3,L-2 edges in LaMnO3/LaNiO3 superlattices grown along (001) and (111) orientations. Our results show a significant XMCD signal and thus the prese ...

American Physical Society2015

Origin of Perpendicular Magnetic Anisotropy and Large Orbital Moment in Fe Atoms on MgO

Harald Brune, Pietro Gambardella, Stefano Rusponi, Marina Pivetta, Fabio Donati, Luca Gragnaniello, Giulia Elisabetta Pacchioni, Jan Gui-Hyon Dreiser

We report on the magnetic properties of individual Fe atoms deposited on MgO(100) thin films probed by x-ray magnetic circular dichroism and scanning tunneling spectroscopy. We show that the Fe atoms have strong perpendicular magnetic anisotropy with a zer ...

American Physical Society2015

Transport properties of a quasi-two-dimensional electron system formed in LaAlO3/EuTiO3/SrTiO3 heterostructures

Stefano Rusponi, Zoran Ristic

We study the structural, magnetic, and transport properties of LaAlO3/EuTiO3/SrTiO3 heterostructures grown by pulsed laser deposition. The samples are characterized in situ by electron diffraction and scanning probe microscopy and ex situ by transport meas ...

Amer Physical Soc2014

Magnetism and morphology of Co nanocluster superlattices on GdAu2/Au(111)-(13 x 13)

Harald Brune, Stefano Rusponi, Alberto Cavallin

We present a comprehensive study of the magnetism and morphology of an ultrahigh density array of Co nanoclusters self-assembled on the single atomic layer GdAu2 on Au(111) template surface. Combining scanning tunneling microscopy, x-ray magnetic circular ...

American Physical Society2014

Low Temperature Ferromagnetism in Chemically Ordered FeRh Nanocrystals

Harald Brune, Stefano Rusponi, Sergio Vlaic, Alberto Cavallin, Jan Gui-Hyon Dreiser

In sharp contrast to previous studies on FeRh bulk, thin films, and nanoparticles, we report the persistence of ferromagnetic order down to 3 K for size-selected 3.3 nm diameter nanocrystals embedded into an amorphous carbon matrix. The annealed nanopartic ...

Amer Physical Soc2013

Two Distinct Phases of Bilayer Graphene Films on Ru(0001)

Harald Brune, Marco Grioni, Stefano Rusponi, Anne Lehnert, Daniela Pacilè, Quentin Dubout, Emmanouil Frantzeskakis, Donat Fabian Natterer

By combining angle-resolved photoemission spectroscopy and scanning tunneling microscopy we reveal the structural and electronic properties of multilayer graphene on Ru(0001). We prove that large ethylene exposure allows the synthesis of two distinct phase ...

Amer Chemical Soc2012

An Endohedral Single-Molecule Magnet with Long Relaxation Times: DySc_{2}N@C_{80}

Harald Brune, Stefano Rusponi, Jan Gui-Hyon Dreiser

The magnetism of DySc2N@C80 endofullerene was studied with X-ray magnetic circular dichroism (XMCD) and a magnetometer with a superconducting quantum interference device (SQUID) down to temperatures of 2 K and in fields up to 7 T. XMCD shows hysteresis of ...

2012

Atomic-scale engineering of magnetic anisotropy of nanostructures through interfaces and interlines

Philipp Buluschek, Harald Brune, Stefano Rusponi, Géraud Moulas, Sergio Vlaic

The central goals of nanoscale magnetic materials science are the self-assembly of the smallest structure exhibiting ferromagnetic hysteresis at room temperature, and the assembly of these structures into the highest density patterns. The focus has been on ...

Nature Publishing Group2012

X-ray Magnetic Circular Dichroism (XMCD) Study of a Methoxide-Bridged Dy^III-Cr^III Cluster Obtained by Fluoride Abstraction from cis-[Cr^III F_2 (phen)_2]^+

Harald Brune, Stefano Rusponi, Jan Gui-Hyon Dreiser

An isostructural series of dinuclear chromium(III)-lanthanide(III) clusters is formed by fluoride abstraction of cis-CrF2(phen)(2) by Ln(3+) resulting in LnF(3) and methoxide-bridged Cr-Ln clusters (Ln = Nd (1), Tb (2), Dy (3)) of formula [Cr-III(phen ...

Amer Chemical Soc2012

Optimizing long-range order, band gap, and group velocities for graphene on close-packed metal surfaces

Harald Brune, Stefano Rusponi, Donat Fabian Natterer

We compare different growth methods with the aim of optimizing the long-range order of a graphene layer grown on Ru(0001). Combining chemical vapor deposition with carbon loading and segregation of the surface layer leads to autocorrelation lengths of 240 ...

2012

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