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Majed Chergui

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Publications associées (250)

Revealing hole trapping in zinc oxide nanoparticles by time-resolved X-ray spectroscopy

Majed Chergui, Wojciech Gawelda, Thomas James Penfold, Jochen Rittmann, Fabio Giacomo Santomauro

AMER CHEMICAL SOC2018

Perspective: Opportunities for ultrafast science at SwissFEL

Majed Chergui, Paul Beaud

We present the main specifications of the newly constructed Swiss Free Electron Laser, SwissFEL, and explore its potential impact on ultrafast science. In light of recent achievements at current X-ray free electron lasers, we discuss the potential territor ...

2018

Photophysical Heavy-Atom Effect in Iodinated Metallocorroles: Spin-Orbit Coupling and Density of States

Majed Chergui, Marine Eva Fedora Bouduban, Enrico Pomarico

Excited-state dynamics and electronic structures of Al and Ga corrole complexes were studied as a function of the number of beta-pyrrole iodine substituents. Using spectrally broad-band femtosecond-resolved fluorescence upconversion, we determined the kine ...

AMER CHEMICAL SOC2018

Discovery and room-temperature ultrafast manipulation of strongly bound excitons in anatase TiO2

Majed Chergui, Tania Palmieri, Edoardo Baldini

AMER CHEMICAL SOC2018

Nonadiabatic effects in electronic and nuclear dynamics

Majed Chergui, Ursula Röthlisberger, Jiri Vanicek, Aurélien Kevin Fabrice Patoz, Tomas Zimmermann, Elisa Liberatore, Nicholas John Browning, Martin Peter Bircher

Due to their very nature, ultrafast phenomena are often accompanied by the occurrence of nonadiabatic effects. From a theoretical perspective, the treatment of nonadiabatic processes makes it necessary to go beyond the (quasi) static picture provided by th ...

2017

Implications of short time scale dynamics on long time processes

Majed Chergui, Jean-Pierre Wolf, Ursula Röthlisberger, Luigi Bonacina, Cédric Schmidt, Siri Camee van Keulen, Swarnendu Bhattacharyya

2017

Anomalous anisotropic exciton temperature dependence in rutile TiO2

Majed Chergui, Edoardo Baldini

Elucidating the details of electron-phonon coupling in semiconductors and insulators is a topic of pivotal interest, as it governs the transport mechanisms and is responsible for various phenomena such as spectral-weight transfers to phonon sidebands and s ...

2017

Localized holes and delocalized electrons in photoexcited inorganic perovskites: Watching each atomic actor by picosecond X-ray absorption spectroscopy

Majed Chergui, Andre Al Haddad, Lars-Hendrik Mewes, Thomas Charles Henry Rossi, Gloria Capano, Jakob Grilj, Fabio Giacomo Santomauro, Dominik Kinschel, James Michael Budarz

We report on an element-selective study of the fate of charge carriers in photoexcited inorganic CsPbBr3 and CsPb(ClBr)(3) perovskite nanocrystals in toluene solutions using time-resolved X-ray absorption spectroscopy with 80 ps time resolution. Probing th ...

Amer Inst Physics2017

Photophysics of a copper phenanthroline elucidated by trajectory and wavepacket-based quantum dynamics: a synergetic approach

Majed Chergui, Ivano Tavernelli, Thomas James Penfold, Gloria Capano

On-the-fly excited state molecular dynamics is a valuable method for studying non-equilibrium processes in excited states and is beginning to emerge as a mature approach much like its ground state counterparts. In contrast to quantum wavepacket dynamics me ...

Royal Society of Chemistry2017

Harmonium: An Ultrafast Vacuum Ultraviolet Facility

Marco Grioni, Marcel Drabbels, Majed Chergui, Frank van Mourik, Christopher Alexander Arrell, Alberto Crepaldi, José Javier Pancracio Ojeda Andara, Andrew Daniel Bonnar Clark, Gianmarco Gatti, Luca Longetti, Silvan Dino Marcos Roth

Harmonium is a vacuum ultraviolet (VUV) photon source built within the Lausanne Centre for Ultrafast Science (LACUS). Utilising high harmonic generation, photons from 20-110 eV are available to conduct steady-state or ultrafast photoelectron and photoion s ...

Swiss Chemical Soc2017

Charge separation and carrier dynamics in donor-acceptor heterojunction photovoltaic systems

Jacques-Edouard Moser, Majed Chergui, Joël Teuscher, Jean-Pierre Wolf, Ursula Röthlisberger, Jan Cornelius Brauer, Alicia Solano, Natalie Renuka Banerji, Ariadni Boziki

Electron transfer and subsequent charge separation across donor-acceptor heterojunctions remain the most important areas of study in the field of third-generation photovoltaics. In this context, it is particularly important to unravel the dynamics of indiv ...

2017

Photoaquation Mechanism of Hexacyanoferrate(II) Ions: Ultrafast 2D UV and Transient Visible and IR Spectroscopies

Majed Chergui, Gerald Auböck, Marco Eli Reinhard, Thomas James Penfold, Raphaël Horváth

Ferrous iron(II) hexacyanide in aqueous solutions is known to undergo photoionization and photoaquation reactions depending on the excitation wavelength. To investigate this wavelength dependence, we implemented ultrafast two-dimensional UV transient absor ...

American Chemical Society2017

Preface to Special Topic: Ultrafast Structural Dynamics-A Tribute to Ahmed H. Zewail

Majed Chergui

Amer Inst Physics2017

Photoemission and photoionization time delays and rates

Majed Chergui, Ursula Röthlisberger, Christopher Alexander Arrell, Elisa Liberatore

2017

Time-resolved ARPES at LACUS: Band Structure and Ultrafast Electron Dynamics of Solids

Helmuth Berger, Philippe Bugnon, Marco Grioni, Majed Chergui, Frank van Mourik, Arnaud Magrez, Christopher Alexander Arrell, Alberto Crepaldi, José Javier Pancracio Ojeda Andara, Gianmarco Gatti, Silvan Dino Marcos Roth

The manipulation of the electronic properties of solids by light is an exciting goal, which requires knowledge of the electronic structure with energy, momentum and temporal resolution. Time- and angle-resolved photoemission spectroscopy (tr-ARPES) is the ...

2017

Charge migration and charge transfer in molecular systems

Jacques-Edouard Moser, Majed Chergui, Joël Teuscher, Ursula Röthlisberger, Christopher Alexander Arrell, Andrea Cannizzo, Pablo Lopez Tarifa, Natalie Renuka Banerji, Elisa Liberatore

The transfer of charge at the molecular level plays a fundamental role in many areas of chemistry, physics, biology and materials science. Today, more than 60 years after the seminal work of R. A. Marcus, charge transfer is still a very active field of res ...

2017

Charge-transfer and impulsive electronic-to-vibrational energy conversion in ferricyanide: ultrafast photoelectron and transient infrared studies'

Majed Chergui, Christopher Alexander Arrell, José Javier Pancracio Ojeda Andara, Luca Longetti

The photophysics of ferricyanide in H2O, D2O and ethylene glycol was studied upon excitation of ligand-to-metal charge transfer (LMCT) transitions by combining ultrafast photoelectron spectroscopy (PES) of liquids and transient vibrational spectroscopy. Up ...

Royal Society of Chemistry2017

Time-resolved Element-selective Probing of Charge Carriers in Solar Materials

Majed Chergui, Mercedes Hannelore Rittmann-Frank, Jochen Rittmann, Thomas Charles Henry Rossi, Fabio Giacomo Santomauro, Dominik Kinschel, James Michael Budarz

We review our recent results on the implementation of picosecond (ps) X-ray absorption spectroscopy to probe the electronic and geometric structure of centres formed by photoexcitation of solar materials such as TiO2 polymorphs and inorganic Cs-based perov ...

2017

The LOUVRE Laboratory: State-of-the-Art Ultrafast Ultraviolet Spectroscopies for Molecular and Materials Science

Majed Chergui, Frank van Mourik, Natalia Nagornova, Lars-Hendrik Mewes, Thomas Charles Henry Rossi, Tania Palmieri, Edoardo Baldini, Malte Oppermann, Benjamin Bauer, Aurelio Oriana

We describe the facilities for ultraviolet studies in the femtosecond to nanosecond time domain. These facilities consist of: i) a set-up for deep-ultraviolet spectroscopy in the 260–380 nm range in both pump and probe pulses for transient absorption/refle ...

2017

Photoinduced Structural Dynamics of Molecular Systems Mapped by Time-Resolved X-ray Methods

Majed Chergui

We review the tremendous advances in ultrafast X-ray science, over the past 15 years, making the best use of new ultrashort X-ray sources including table-top or large-scale facilities. Different complementary X-ray-based techniques, including spectroscopy, ...

American Chemical Society2017

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