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Marcel Drabbels

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Publications associées (54)

Ultrafast relaxation of photoexcited superfluid He nanodroplets

Marcel Drabbels, Alberto Hernando de Castro

The relaxation of photoexcited nanosystems is a fundamental process of light–matter interaction. Depending on the couplings of the internal degrees of freedom, relaxation can be ultrafast, converting electronic energy in a few fs, or slow, if the energy is ...

Nature Research2020

Real-time observation of jumping and spinning nanodroplets

Marcel Drabbels, Ulrich Lorenz, Pavel Olshin, Jonathan Mark Voss

The manipulation of liquids at nanoscale dimensions is a central goal of the emergent nanofluidics field. Such endeavors extend to nanodroplets, which are ubiquitous objects involved in many technological applications. Here, we employ time-resolved electro ...

2020

Tracking attosecond electronic coherences using phase-manipulated extreme ultraviolet pulses

Marcel Drabbels, Primoz Rebernik Ribic

The recent development of ultrafast extreme ultraviolet (XUV) coherent light sources bears great potential for a better understanding of the structure and dynamics of matter. Promising routes are advanced coherent control and nonlinear spectroscopy schemes ...

Nature Research2020

Time-resolved formation of excited atomic and molecular states in XUV-induced nanoplasmas in ammonia clusters

Marcel Drabbels, Andrew Daniel Bonnar Clark, Verónica Oliver Álvarez de Lara

High intensity XUV radiation from a free-electron laser (FEL) was used to create a nanoplasma inside ammonia clusters with the intent of studying the resulting electron-ion interactions and their interplay with plasma evolution. In a plasma-like state, ele ...

ROYAL SOC CHEMISTRY2020

Intense microsecond electron pulses from a Schottky emitter

Marcel Drabbels, Ulrich Lorenz, Pavel Olshin, Gabriele Bongiovanni

Thanks to their high brightness, field emitters are the electron sources of choice in most high-end electron microscopes. Under typical operating conditions, the available emission current from these emitters is largely limited by practical considerations, ...

AIP American Institute of Physics2020

In Situ Observation of Coulomb Fission of Individual Plasmonic Nanoparticles

Marcel Drabbels, Ulrich Lorenz, Pavel Olshin, Jonathan Mark Voss

Reshaping plasmonic nanoparticles with laser pulses has been extensively researched as a tool for tuning their properties. However, in the absence of direct observations of the processes involved, important mechanistic details have remained elusive. Here, ...

2019

Helium-induced electronic transitions in photo-excited Ba+–Hen exciplexes

Marcel Drabbels

The possibility for helium-induced electronic transitions in a photo-excited atom is investigated using Ba+ excited to the 6p 2P state as a prototypical example. A diabatization scheme has been designed to obtain the necessary potential energy surfaces and ...

2018

Harmonium: An Ultrafast Vacuum Ultraviolet Facility

Marco Grioni, Marcel Drabbels, Majed Chergui, Frank van Mourik, Christopher Alexander Arrell, Alberto Crepaldi, José Javier Pancracio Ojeda Andara, Andrew Daniel Bonnar Clark, Gianmarco Gatti, Luca Longetti, Silvan Dino Marcos Roth

Harmonium is a vacuum ultraviolet (VUV) photon source built within the Lausanne Centre for Ultrafast Science (LACUS). Utilising high harmonic generation, photons from 20-110 eV are available to conduct steady-state or ultrafast photoelectron and photoion s ...

Swiss Chemical Soc2017

Dynamics of photoexcited Ba+ cations in 4He nanodroplets

Marcel Drabbels, Xiaohang Zhang, Alberto Hernando de Castro

We present a joint experimental and theoretical study on the desolvation of Ba+ cations in 4He nanodroplets excited via the 6p 6s transition. The experiments reveal an efficient desolvation process yielding mainly bare Ba+ cations and Ba+Hen exciplexes wit ...

American Institute of Physics2016

Migration of surface excitations in highly-excited nanosystems probed by intense resonant XUV radiation

Marcel Drabbels

Ionization dynamics of resonantly excited helium nanodroplets have been studied by intense XUV light. By doping the nanodroplets with atoms that either attach to the surface or submerge into the center of the droplet, one can study the dynamics of excitati ...

2015

Excitation of Sodium Atoms Attached to Helium Nanodroplets: The 3p

Marcel Drabbels, Evgeniy Loginov, Alberto Hernando de Castro

The dynamics of Na atoms on the surface of helium nanodroplets following excitation via the 3p

American Chemical Society2015

Nucleation of quantized vortex rings in 4He nanodroplets

Marcel Drabbels, Xiaohang Zhang

Whereas most of the phenomena associated with superfluidity have been observed in finite-size helium systems, the nucleation of quantized vortices has proven elusive. Here we show that the solvation of a Ba+ ion created by photoionization of neutral Ba at ...

American Institute of Physics2014

Dynamics of Excited Sodium Atoms Attached to Helium Nanodroplets

Marcel Drabbels, Evgeniy Loginov

The dynamics of laser-excited sodium atoms at the surface of helium nanodroplets has been investigated as a function of quantum state. For all cases excitation of the system leads to desorption of the sodium atom from the droplet surface. The mean kinetic ...

American Chemical Society2014

Elementary Excitations of Superfluid Helium Droplets Probed by Ion Spectroscopy

Marcel Drabbels, Xiaohang Zhang

Electronic spectra of molecules in helium droplets reveal spectral features that are related to the elementary excitations of the superfluid helium environment. In order to determine to what extend the interaction strength of the molecule with the helium a ...

Amer Chemical Soc2014

Picosecond solvation dynamics of alkali cations in superfluid 4He nanodroplets

Marcel Drabbels, Alberto Hernando de Castro

The dynamics following the photoionization of neutral Rb and Cs atoms residing in a dimple at the surface of a superfluid 4He1000 nanodroplet has been investigated within time-dependent density functional theory, complementing a previous study on Ba. The c ...

American Physical Society2014

Translational dynamics of photoexcited atoms in 4He nanodroplets: the case of silver

Marcel Drabbels, Evgeniy Loginov, Alberto Hernando de Castro

The dynamics following the photoexcitation of Ag atoms in 4He nanodroplets via the 5p 2P1=2 ← 5s2S1=2 and 5p 2P3=2 ← 5s2S1=2 transitions has been investigated in a joint experimental and theoretical effort. It has been experimentally found that upon excita ...

Royal Soc Chemistry2013

Critical Landau velocity in helium nanodroplets

Marcel Drabbels, Evgeniy Loginov, Nils Benedict Brauer, Alberto Hernando de Castro

The best-known property of superfluid helium is the vanishing viscosity that objects experience while moving through the liquid with speeds below the so-called critical Landau velocity. This critical velocity is generally considered a macroscopic property ...

American Physical Society2013

Barium Ions and Helium Nanodroplets: Solvation and Desolvation

Marcel Drabbels, Xiaohang Zhang

The solvation of Ba+ ions created by the photoionization of barium atoms located on the surface of helium nanodroplets has been investigated. The excitation spectra corresponding to the 6p 2P1/2

American Institute of Physics2012

Spectroscopy and Dynamics of Barium-doped Helium Nanodroplets

Marcel Drabbels, Evgeniy Loginov

Excitation spectra up to the ionization threshold are reported for barium atoms located on the surface of helium nanodroplets. For states with low principal quantum number, the resonances are substantially broadened and shifted towards higher energy with r ...

American Institute of Physics2012

Mid-Infrared Spectroscopy of Molecular Ions in Helium Nanodroplets

Marcel Drabbels, Nils Benedict Brauer, Xiaohang Zhang

High resolution IR spectra of aniline, styrene and 1,1-diphenylethylene cations embedded in superfluid helium nanodroplets have been recorded in the 300-1700 cm-1 range using the free-electron laser FELIX as radiation source. Comparison of the spectra with ...

American Institute of Physics2012

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