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Concept

Graphene oxide paper

Publications associées (27)

Functionalized Å-scale Pores in Graphene for Carbon Capture

Kuang-Jung Hsu

Single-layer graphene, hosting a high density of functionalized molecular-sieving atom-thick pores, is considered to be an excellent material for gas separation membranes. These functionalized atom-thick pores enable the shortest transport pathway across t ...

EPFL2024

Resonant Transducers Consisting of Graphene Ribbons with Attached Proof Masses for NEMS Sensors

Luis Guillermo Villanueva Torrijo, Daniel Moreno Garcia

The unique mechanical and electrical properties of graphene make it an exciting material for nanoelectromechanical systems (NEMS). NEMS resonators with graphene springs facilitate studies of graphene's fundamental material characteristics and thus enable i ...

Amer Chemical Soc2023

Mass transport of water vapor and ions from Å-scale graphene nanopores

Wan-Chi Lee

Hydrodynamics at the nanoscale involves both fundamental study and application of fluid and mass transport phenomena in nanometer-sized confinements. Nanopores in single-layer graphene can be highly attractive for exploring the molecular transport of gas a ...

EPFL2022

Demonstrating and Unraveling a Controlled Nanometer-Scale Expansion of the Vacancy Defects in Graphene by CO2

Kumar Varoon Agrawal, Luis Francisco Villalobos Vazquez de la Parra, Kuang-Jung Hsu, Mojtaba Chevalier

A controlled manipulation of graphene edges and vacancies is desired for molecular separation, sensing and electronics applications. Unfortunately, available etching methods always lead to vacancy nucleation making it challenging to control etching. Herein ...

Wiley-VCH Verlag GmbH2022

Rapid Gas Transport from Block-Copolymer Templated Nanoporous Carbon Films

Kumar Varoon Agrawal, Luis Francisco Villalobos Vazquez de la Parra, Mostapha Dakhchoune, Kuang-Jung Hsu, Marina Micari, Jing Zhao, Xuekui Duan

Porous carbon films, attributed to their superior thermal and chemical robustness, are attractive for a number of applications. In the context of molecular separation, a major focus has been on films where the effective pore diameter is lower than 1 nm, e. ...

AMER CHEMICAL SOC2021

Exploring optically active defects in wide-bandgap materials using fluorescence microscopy

Evgenii Glushkov

Defects in solid-state systems can be both detrimental, deteriorating the quality of materials, or desired, thanks to the novel functionality they bring. Optically active point defects, producing fluorescent light, are a great example of the latter. Natura ...

EPFL2021

Etching nanopores in single-layer graphene with a sub-angstrom resolution in molecular sieving

Shiqi Huang

Single-layer graphene (SLG) membranes, hosting molecular-sieving nanopores have been regarded as the ultimate gas separation membranes, attributing to the fact that they are the thinnest possible molecular barrier. However, the expected attractive performa ...

EPFL2021

Manufacture and characterization of graphene membranes with suspended silicon proof masses for MEMS and NEMS applications

Luis Guillermo Villanueva Torrijo

Graphene's unparalleled strength, chemical stability, ultimate surface-to-volume ratio and excellent electronic properties make it an ideal candidate as a material for membranes in micro- and nanoelectromechanical systems (MEMS and NEMS). However, the inte ...

2020

Synergistic CO2-Sieving from Polymer with Intrinsic Microporosity Masking Nanoporous Single-Layer Graphene

Kumar Varoon Agrawal, Mounir Driss Mensi, Luis Francisco Villalobos Vazquez de la Parra, Shiqi Huang, Guangwei He, Wan-Chi Lee, Jing Zhao

High-flux nanoporous single-layer graphene membranes are highly promising for energy-efficient gas separation. Herein, in the context of carbon capture, a remarkable enhancement in the CO(2)selectivity is demonstrated by uniquely masking nanoporous single- ...

WILEY-V C H VERLAG GMBH2020

Centimeter-scale gas-sieving nanoporous single-layer graphene membrane

Kumar Varoon Agrawal, Shiqi Huang, Mostapha Dakhchoune, Guangwei He, Luc Sébastien Bondaz, Wan-Chi Lee

High-permeance, molecular-sieving, nanoporous single-layer graphene (NSLG) membranes are highly promising for gas separation. However, the formation of cracks during the transfer of NSLG to a low-cost porous support is difficult to avoid. These cracks are ...

2020

Nanosecond pulsed laser-processing of CVD diamond

Patrik Willi Hoffmann, Marco Cantoni, Sébastien Equis

This work considers the resulting material structural effects of laser-processing chemical vapor deposited (CVD) diamond. The utilized 532 nm wavelength laser had a pulse duration of 40 ns together with a spot diameter of ca. 40 mu m. The effect of cutting ...

ELSEVIER SCI LTD2020

Adsorption-induced spontaneous curvature and superflexibility in monolayer graphene

Hervé Stéphane Elettro

Graphene is considered an enabling material for next generation sensors, due to the remarkable properties derived from its atomic thickness. However, these promises come with acute sensitivity to parasite adsorbates, that may hinder reaching the full poten ...

AMER PHYSICAL SOC2020

Hydrogen storage material

Andreas Züttel, Heena Yang

The present relates to a carbon material having a 3D structure and made of graphene oxide and carbon nanotubes, characterized in that the 3D structure consists in that the carbon nanotubes are located with some agglomeration between the graphene oxide laye ...

2019

Characterizing the maximum number of layers in chemically exfoliated graphene

László Forró, Bálint Náfrádi, Péter Szirmai, Ferenc Simon

An efficient route to synthesize macroscopic amounts of graphene is highly desired and bulk characterization of such samples, in terms of the number of layers, is equally important. We present a Raman spectroscopy-based method to determine the typical uppe ...

Springer Nature2019

Crystallization of gas-selective nanoporous graphene by competitive etching and growth: a modeling study

Kumar Varoon Agrawal, Mojtaba Chevalier

A robust synthesis methodology for crystallizing nanoporous single-layer graphene hosting a high density of size-selective nanopores is urgently needed to realize the true potential of two-dimensional membranes for gas separation. Currently, there are no c ...

Nature Research2019

Single-layer graphene membranes by crack-free transfer for gas mixture separation

Andreas Züttel, Emad Oveisi, Kumar Varoon Agrawal, Duncan Thomas Lindsay Alexander, Wen Luo, Shiqi Huang, Mostapha Dakhchoune, Guangwei He, Mojtaba Chevalier, Jing Zhao

The single-layer graphene film, when incorporated with molecular-sized pores, is predicted to be the ultimate membrane. However, the major bottlenecks have been the crack-free transfer of large-area graphene on a porous support, and the incorporation of mo ...

Nature Publishing Group2018

Theory, design and measurement of near-optimal graphene reconfigurable and non-reciprocal devices at terahertz frequencies

Michele Tamagnone

This thesis explores the applications of graphene for terahertz and far infrared optical components and antennas, with particular emphasis on tunable and non-reciprocal devices. Both terahertz technologies and graphene are emerging fields which hold many p ...

EPFL2016

Polymer - Carbon Nanostructures Composites : from Chemistry to Physics, to Material Science

Maryam Majidian

Synthesis and characterization of polymer-based composites containing carbon nanostructures is the focus of this dissertation. The main polymer which has been used for this research is SU8. The motivation of the work is to overcome the drawbacks of SU8 e.g ...

EPFL2016

Low-temperature Fabrication of Highly-Efficient, Optically-Transparent (FTO-free) Graphene Cathode for Co-Mediated Dye-Sensitized Solar Cells with Acetonitrile-free Electrolyte Solution

Michael Graetzel, Shaik Mohammed Zakeeruddin, Paul Liska, Ladislav Kavan

Propionitrile electrolyte solutions mixed with sulfolane or with 1-ethyl 3-methyl imidazolium tetracyanoborate (ionic liquid) are optimized for Co(bpy)(3)(3+)/Co(bpy)(3)(2+)-tmediated DSCs working at low illumination intensity. Highly-active cathode cataly ...

Elsevier2016

On the optical properties of carbon nanotubes. Part I. A general formula for the dynamical optical conductivity

Benjamin Ricaud

This paper is the first one in a series of two articles in which we revisit the optical properties of single-walled carbon nanotubes (SWNTs). Produced by rolling up a graphene sheet, SWNTs owe their intriguing properties to their cylindrical quasi-one-dime ...

Amer Inst Physics2016