LaTiO2N/In2O3 photoanodes with improved performance for solar water splitting

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Measurement-system design for structural identification

Numa Joy Bertola

In developed countries, the management of existing civil infrastructure is challenging due to evolving functional requirements, aging and climate change. Due to conservative approaches in construction design and practice, infrastructure often has hidden re ...

EPFL2020

Solar Water Splitting with Perovskite/Silicon Tandem Cell and TiC-Supported Pt Nanocluster Electrocatalyst

Michael Graetzel, Shaik Mohammed Zakeeruddin, Christophe Ballif, Quentin Thomas Jeangros, Jingshan Luo, Dan Ren, Jing Gao, Florent Sahli, Jérémie Werner

Developing efficient, stable, and cost-effective photosystems to split water into hydrogen and oxygen using sunlight is of paramount importance for future production of fuels and chemicals from renewable sources. However, the high cost of current systems l ...

2019

Rapid Performance Optimization Method for Photoelectrodes

Sophia Haussener, Yannick Kenneth Gaudy

We report the development of a rapid method for the performance optimization of photoelectrodes. The method requires as an input incident photon-to-current efficiency (IPCE) measurements of a material at two or more wavelengths, an estimation of the comple ...

2019

Investigations into Nanostructured Materials for Water Splitting and Direct Solar Energy Harvesting

Filip Mateusz Podjaski

This thesis deals with different aspects of renewable energy transformation and storage concepts and connects them. Although renewable energy installations are growing worldwide, their use is limited by storage technologies. As such, water splitting for hy ...

EPFL2019

Dye sensitized photoelectrolysis cells

Ulf Anders Hagfeldt, Nikolaos Vlachopoulos

To advance the progress of photoelectrolysis, various promising devices integrated with p- and n-type photocatalysts and dye sensitized photoelectrodes have been systematically studied. This review discusses, from theory to practice, an integration strateg ...

Royal Society of Chemistry2019

Hematite Photoanodes for Solar Water Splitting: A Detailed Spectroelectrochemical Analysis on the pH-Dependent Performance

Nestor Guijarro Carratala, Florian Le Formal, Yongpeng Liu, Florent Alexandre Boudoire

The effect of the electrolyte pH on the performance of metal oxide photoanodes for solar water oxidation has not been fully resolved, and contrasting views have been presented in recent reports. Herein, a comprehensive set of spectroelectrochemical techniq ...

AMER CHEMICAL SOC2019

A Step toward Economically Viable Solar Fuel Production

Kevin Sivula

Recently in Joule, Zhang, Li, and colleagues reported a new benchmark in photocatalytic overall water splitting. By optimizing the co-catalysts and redox mediator between the light absorbers in a two-step heterogeneous photosystem, the authors reached an a ...

CELL PRESS2018

Yttrium Tantalum Oxynitride Multiphases as Photoanodes for Water Oxidation

Nicola Marzari

The perovskite yttrium tantalum oxynitride is theoretically proposed as a promising semiconductor for solar water splitting because of the predicted band gap and energy positions of band edges. In experiments, however, we show here that depending on the pr ...

AMER CHEMICAL SOC2019

Organic Semiconductor Based Devices for Solar Water Splitting

Kevin Sivula, Liang Yao, Nestor Guijarro Carratala, Muhammad Aiman Bin Rahmanudin Hamdan

Solution processable organic semiconductors are well-established as high-performance materials for inexpensive and scalable solar energy conversion in organic photovoltaic (OPV) devices, but their promise in the economic conversion of solar energy into che ...

2018

Insights into the interfacial carrier behaviour of copper ferrite ( CuFe2O4) photoanodes for solar water oxidation

Kevin Sivula, Liang Yao, Nestor Guijarro Carratala, Florian Le Formal, Yongpeng Liu, Florent Alexandre Boudoire

Designing efficient yet robust photoanodes for water oxidation stands out as a major bottleneck in the realization of a feasible photoelectrochemical tandem cell for solar water splitting. Spinel copper ferrite (CuFe2O4) has been recently reported as a pot ...

Royal Society of Chemistry2019

Amorphous Cobalt Vanadium Oxide as a Highly Active Electrocatalyst for Oxygen Evolution

Xile Hu, Laurent Liardet

The water-splitting reaction provides a promising mechanism to store renewable energies in the form of hydrogen fuel. The oxidation half-reaction, the oxygen evolution reaction (OER), is a complex four-electron process that constitutes an efficiency bottle ...

2018

Solar-Electrochemical Devices for Water Splitting and Chlorine Generation

Enrico Chinello

Solar technologies hold the potential to ultimately counteract the effects of climate change. Nevertheless, the intermittency of sunlight poses technical challenges regarding the storage of the surplus production and the supply of the deficit. The generat ...

EPFL2019