Publication

Increased nickel exsolution from LaFe0.8Ni0.2O3 perovskite-derived CO2 methanation catalysts through strontium doping

Oliver Kröcher, Davide Ferri, Patrick Simon Steiger
2020
Journal Articles

Abstract

Perovskite-derived Ni catalysts offer the remarkable benefit of redox stability that allows their regeneration after deactivation through poisoning or Ni particle growth. Here, the catalytic activity of LaFe0.8Ni0.2O3 towards CO2 methanation was improved by increasing Ni reducibility and segregation to the perovskite surface through partial substitution of La by Sr (La1-xSrxFe0.8Ni0.2O3-delta, 0

Official source

https://infoscience.epfl.ch/entities/publication/cfa5883d-fe23-4426-bd02-684296443758

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Oliver Kröcher, Davide Ferri, Patrick Simon Steiger
2020
Journal Articles

Abstract

Official source

https://infoscience.epfl.ch/entities/publication/cfa5883d-fe23-4426-bd02-684296443758

About this result

Related concepts (32)

Perovskite (structure)

A perovskite is any material with a crystal structure following the formula ABX3, which was first discovered as the mineral called perovskite, which consists of calcium titanium oxide (CaTiO3). The mineral was first discovered in the Ural mountains of Russia by Gustav Rose in 1839 and named after Russian mineralogist L. A. Perovski (1792–1856). 'A' and 'B' are two positively charged ions (i.e. cations), often of very different sizes, and X is a negatively charged ion (an anion, frequently oxide) that bonds to both cations.

Selective catalytic reduction

Selective catalytic reduction (SCR) means of converting nitrogen oxides, also referred to as NOxNOx with the aid of a catalyst into diatomic nitrogen (N2), and water (H2O). A reductant, typically anhydrous ammonia (NH3), aqueous ammonia (NH4OH), or a urea (CO(NH2)2) solution, is added to a stream of flue or exhaust gas and is reacted onto a catalyst. As the reaction drives toward completion, nitrogen (N2), and carbon dioxide (CO2), in the case of urea use, are produced.

High-temperature superconductivity

High-temperature superconductors (abbreviated high-Tc or HTS) are defined as materials with critical temperature (the temperature below which the material behaves as a superconductor) above , the boiling point of liquid nitrogen. They are only "high-temperature" relative to previously known superconductors, which function at even colder temperatures, close to absolute zero. The "high temperatures" are still far below ambient (room temperature), and therefore require cooling.

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Increased nickel exsolution from LaFe0.8Ni0.2O3 perovskite-derived CO2 methanation catalysts through strontium doping

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