Publication

Surface screening of written ferroelectric domains in ambient conditions

2013
Conference Papers

Abstract

We have combined Piezoresponse Force Microscopy and Kelvin Probe Force Microscopy (KPFM) to study screening charge dynamics in written domains on PbZr0.2Ti0.8O3 (PZT) thin film surfaces under a controlled environment and at variable temperature. The screening dynamics decayed exponentially on a timescale of tens of minutes, consistently with what we expected for water-mediated surface diffusion of ionic species. Variable-temperature KPFM measurements showed variations in surface potential due to temporary unbalanced surface screening charges. Low humidity experiments revealed gradual incorporation of positive charges onto the surface, even in a non-reactive environment (N-2), as well as deceleration of the screening dynamics upon reversal of the temperature variation. Our work may serve as a guide for future studies on the dynamics and nature of adsorbates on polarized PZT thin films. (C) 2013 AIP Publishing LLC

Official source

https://infoscience.epfl.ch/entities/publication/a483a376-ae4c-4532-9fd0-77da3c00da42

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2013
Conference Papers

Abstract

Official source

https://infoscience.epfl.ch/entities/publication/a483a376-ae4c-4532-9fd0-77da3c00da42

About this result

Related concepts (32)

Scanning probe microscopy

Scanning probe microscopy (SPM) is a branch of microscopy that forms images of surfaces using a physical probe that scans the specimen. SPM was founded in 1981, with the invention of the scanning tunneling microscope, an instrument for imaging surfaces at the atomic level. The first successful scanning tunneling microscope experiment was done by Gerd Binnig and Heinrich Rohrer. The key to their success was using a feedback loop to regulate gap distance between the sample and the probe.

Scanning electron microscope

A scanning electron microscope (SEM) is a type of electron microscope that produces images of a sample by scanning the surface with a focused beam of electrons. The electrons interact with atoms in the sample, producing various signals that contain information about the surface topography and composition of the sample. The electron beam is scanned in a raster scan pattern, and the position of the beam is combined with the intensity of the detected signal to produce an image.

Surface charge

A surface charge is an electric charge present on a two-dimensional surface. These electric charges are constrained on this 2-D surface, and surface charge density, measured in coulombs per square meter (C•m−2), is used to describe the charge distribution on the surface. The electric potential is continuous across a surface charge and the electric field is discontinuous, but not infinite; this is unless the surface charge consists of a dipole layer. In comparison, the potential and electric field both diverge at any point charge or linear charge.

Related publications (32)

Surface screening of written ferroelectric domains in ambient conditions

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