Direct evidence for charge stripes in a layered cobalt oxide

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Small-angle neutron scattering study of mesoscale magnetic disordering and skyrmion phase suppression in the frustrated chiral magnet Co6.75Zn6.75Mn6.51

Henrik Moodysson Rønnow, Jonathan White

Co-Zn-Mn chiral cubic magnets display versatile magnetic skyrmion phases, including equilibrium phases stable far above and far below room temperature, and the facile creation of robust far-from-equilibrium skyrmion states. In this system, compositional di ...

INT UNION CRYSTALLOGRAPHY2022

Solar reduction of carbon dioxide on copper-tin electrocatalysts with energy conversion efficiency near 20%

Michael Graetzel, Shaik Mohammed Zakeeruddin, Yuhang Liu, Dan Ren, Jing Gao, Jun Li, Meng Xia

Solar-driven carbon dioxide reduction has witnessed a renaissance in the past decades, but the system suffers from low reaction rates. Here the authors develop a copper/tin-oxide electrocatalyst, achieving a new benchmark solar-to-CO energy conversion effi ...

Nature Portfolio2022

Active sites on copper-based catalysts for electrochemical CO2 reduction selectively to C2+ products

Jie Zhang

Electrochemical CO2 reduction (eCO2RR) towards value-added chemicals, powered by renewable electricity, is a promising technology for storing the intermittent renewable energy in the form of chemical bonds. Among the various products of eCO2RR, multi-carbo ...

EPFL2022

Magnetotransport signatures of antiferromagnetism coexisting with charge order in the trilayer cuprate HgBa2Ca2Cu3O8+delta

Siham Benhabib

Multilayered cuprates possess not only the highest superconducting temperature transition but also offer a unique platform to study disorder-free CuO2 planes and the interplay between competing orders with superconductivity. Here, we study the underdoped t ...

Nature Research2022

Investigating field-induced magnetic order in Han purple by neutron scattering up to 25.9 T

Frédéric Mila, Philippe Heller, Bruce Normand

BaCuSi2O6 is a quasi-two-dimensional (2D) quantum antiferromagnet containing three different types of stacked, square-lattice bilayer hosting spin-1/2 dimers. Although this compound has been studied extensively over the last two decades, the critical appli ...

2022

Real space and reciprocal space investigations of the spin dynamics in skyrmion-hosting materials

Le Yu

Magnetic skyrmions are whirl-like spin configurations with particle-like properties protected by non-trivial topology. Due to their unique spin structures and dynamical properties, they have attracted tremendous interests over the past decade, from fundame ...

EPFL2022

Enhanced radio-frequency performance of niobium films on copper substrates deposited by high power impulse magnetron sputtering

Fabio Avino

We present a study of radio frequency properties of niobium films deposited on copper by two different approaches based on High Power Impulse Magnetron Sputtering, namely with a DC voltage biased substrate and with bipolar target voltage. Such approaches e ...

IOP Publishing Ltd2022

Magnetic structure of the topological semimetal Co3Sn2S2

Henrik Moodysson Rønnow, Ivica Zivkovic, Jian Rui Soh

Co3Sn2S2 has recently been predicted to be a Weyl semimetal in which magnetic order is key to its behavior as a topological material. Here, we report unpolarized neutron diffraction and spherical neutron polarimetry measurements, supported by magnetization ...

AMER PHYSICAL SOC2022

Magneto-optical study of metamagnetic transitions in the antiferromagnetic phase of alpha-RuCl3

Zhe Wang

alpha-RuCl3 is a promising candidate material to realize the so far elusive quantum spin liquid ground state. However, at low temperatures, the coexistence of different exchange interactions couple the effective pseudospins into an antiferromagnetically zi ...

NATURE PORTFOLIO2022

Disorder-induced electronic, magnetic, and optoelectronic properties of two-dimensional materials

Cheol Yeon Cheon

Technological advancement has been in cadence with material development by improving the purity of single crystals and, at the same time, controlling their imperfections. These capabilities have been especially vital for developing new technolo-gies based ...

EPFL2022

Randomness and frustration in a S = (1/)(2) square-lattice Heisenberg antiferromagnet

Henrik Moodysson Rønnow, Peter Babkevich, Bruce Normand, Ellen Fogh

We explore the interplay between randomness and magnetic frustration in the series of S = 12 Heisenberg square-lattice compounds Sr2CuTe1???xWxO6. Substituting W for Te alters the magnetic interactions dramatically, from strongly nearest-neighbor to next-n ...

2022