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The matching pursuit algorithm and its variants are among the most commonly used methods for greedy optimization. In this paper, we present the first explicit convergence rates of matching pursuit methods in an optimization sense, for general sets of atoms. We present sublinear O(1/t) convergence on general smooth objectives, and linear convergence on strongly convex objectives. Our algorithm variants and rates do not need any incoherence or sparsity assumptions. Direct applications of the presented algorithms are structured matrix and tensor factorization problems.