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We present a model and protocol that enable the generation of extremely stable computer glasses at minimal computational cost. The protocol consists of an instantaneous quench in an augmented potential energy landscape, with particle radii as additional degrees of freedom. We demonstrate how our glasses' mechanical stability, which is readily tunable in our approach, is reflected in both microscopic and macroscopic observables. Our observations indicate that the stability of our computer glasses is at least comparable to that of computer glasses generated by the celebrated Swap Monte Carlo algorithm Strikingly, some key properties support even qualitatively enhanced stability in our scheme: the density of quasilocalized excitations displays a gap in our most stable computer glasses, whose magnitude scales with the polydispersity of the particles. We explain this observation, which is consistent with the lack of plasticity we observe at small stress. It also suggests that these glasses are depleted from two-level systems, similarly to experimental vapor-deposited ultrastable glasses.
Olivier Schneider, Aurelio Bay, Guido Haefeli, Tatsuya Nakada, Frédéric Blanc, Lesya Shchutska, Elena Graverini, Donal Patrick Hill, Marie Theres Christin Bachmayer, Sebastian Schulte, Aravindhan Venkateswaran, Luis Miguel Garcia Martin, Vitalii Lisovskyi, Serhii Cholak, Federico Ronchetti, Anni Matilda Kauniskangas, Raphaël van Laak, Ettore Zaffaroni, Elisabeth Maria Niel, Pierre Paul Louis Mayencourt, Brianna Leililani Thielen, Arnaud Merlin Gauthey, Gianluca Zunica, Abdul-Kerim Guseinov, Esteban Curras Rivera, Yifei Song, Radoslav Marchevski, Roberto Ribatti, Alexandre Brea Rodriguez, Dimitrios Kaminaris, Rita De Sousa Ataíde Da Silva
Esther Amstad, Ran Zhao, Alexandra Thoma
Laurent Villard, Stephan Brunner, Moahan Murugappan