A PCP-Pincer RuII-Terpyridine Building Block as a Potential "Antenna Unit" for Intramolecular Sensitization

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Sensing the Spin of an Individual Ce Adatom

Wolf-Dieter Schneider, Markus Ternes

The magnetic moment of rare earth elements originates from electrons in the partially filled 4f orbitals. Accessing this moment electrically by scanning tunneling spectroscopy is hampered by shielding of outerlying orbitals. Here, we show that we can detec ...

AMER PHYSICAL SOC2020

Delivery of a Masked Uranium(II) by an Oxide-Bridged Diuranium(III) Complex

Marinella Mazzanti, Farzaneh Fadaei Tirani, Chad Thomas Palumbo, Dieuwertje Katelijn Modder

Oxide is an attractive linker for building polymetallic complexes that provide molecular models for metal oxide activity, but studies of these systems are limited to metals in high oxidation states. Herein, we synthesized and characterized the molecular an ...

Wiley-VCH Verlag GmbH2021

Molecular Engineering of Electrode Surfaces for Electrocatalysis

Patrick Eduard Alexa

Electrocatalysts play an important part on the route towards environmental friendly energy sources. They support modern technologies like fuel cells to move further away from the utilization of fossil fuels and the resulting CO2 emission into our atmospher ...

EPFL2020

Bi-stable spin-crossover in charge-neutral [Fe(R-ptp)(2)] (ptp=2-(1H-pyrazol-1-yl)-6-(1H-tetrazol-5-yl)pyridine) complexes

Sergio Vela Llausi

Bi-stable charge-neutral iron(II) spin-crossover (SCO) complexes are a class of switchable molecular materials proposed for molecule-based switching and memory applications. In this study, we report on the SCO behavior of a series of iron(II) complexes com ...

2020

Wideband Multiport Antennas

Anja Skrivervik, Mirmehdi Seyyedesfahlan

In this paper, a wideband four port 2-6 GHz antenna is proposed. One-, two-, and four-port antennas are implemented and characterized between 2 and 6 GHz. The isolation between the ports is improved by connecting and optimizing the ground plane sections. T ...

2020

Orientation, rotation and solvation of ions in helium nanodroplets

Verónica Oliver Álvarez de Lara

Helium nanodroplets are liquid, finite size, nanoscale helium clusters that have been employed since the 1990s as a matrix for high-resolution spectroscopy of molecules. Spectroscopic studies of ionic species inside helium droplets were not however realise ...

EPFL2019

Highly stable enzyme-mimicking nanocomposite of antioxidant activity

Bálint Náfrádi

A highly stable nanocomposite of antioxidant activity was developed by immobilization of a superoxide dismutase-mimicking metal complex on copolymer-functionalized nanoclay. The layered double hydroxide (LDH) nanoclays were synthesized and surface modifica ...

2019

RF sheath modeling of experimentally observed plasma surface interactions with the JET ITER-Like Antenna

Olivier Sauter, Richard Pitts, Ambrogio Fasoli, Stefano Coda, Basil Duval, Henri Weisen, Yves Martin, Yann Camenen, Jan Horacek, Javier García Hernández, Duccio Testa, Marco Wischmeier, Nicola Vianello, Mikhail Maslov, Patrick Blanchard, Alessandro Pau, Davide Galassi, Antonio José Pereira de Figueiredo, Liang Yao, Dalziel Joseph Wilson, Cristian Sommariva, Jonathan Graves, Federico Nespoli, Hamish William Patten, Samuel Lanthaler, David Pfefferlé, Jonathan Marc Philippe Faustin

Waves in the Ion Cyclotron Range of Frequencies (ICRF) enhance local Plasma-Surface Interactions (PSI) near the wave launchers and magnetically-connected objects via Radio-Frequency (RF) sheath rectification. ITER will use 20MW of ICRF power over long puls ...

Elsevier2019

From structure to application: studies on adenine-, pyrene- and lanthanide-based metal-organic frameworks

Andrzej Gladysiak

Metal-organic frameworks (MOFs) are coordination polymer materials in which inorganic metal ions or clusters are linked with multitopic organic ligands by means of coordination bonds. Their structural versatility allows for design of materials based on pre ...

EPFL2019

Progress on an ion cyclotron range of frequency system for DEMO

Minh Quang Tran

An Ion Cyclotron Range of Frequency (ICRF) system can provide power for a number of tasks, experimentally verified on present machines: heating and current drive, first wall conditioning, plasma startup, removing central impurities, controlling sawteeth an ...

2019